Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change Memory

Abstract Chalcogenide phase change memory, a next‐generation non‐volatile memory technology, holds significant promise in neuromorphic computing, leading to an urgent demand for high‐performance phase change materials. However, in the realm of phase change materials, there appears to be an inherent...

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Main Authors: Ke Gao, Ruizhe Zhao, Xin Li, Jingwei Cai, Hao Tong, Xiangshui Miao
Format: Article
Language:English
Published: Wiley-VCH 2025-08-01
Series:Advanced Electronic Materials
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Online Access:https://doi.org/10.1002/aelm.202500032
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author Ke Gao
Ruizhe Zhao
Xin Li
Jingwei Cai
Hao Tong
Xiangshui Miao
author_facet Ke Gao
Ruizhe Zhao
Xin Li
Jingwei Cai
Hao Tong
Xiangshui Miao
author_sort Ke Gao
collection DOAJ
description Abstract Chalcogenide phase change memory, a next‐generation non‐volatile memory technology, holds significant promise in neuromorphic computing, leading to an urgent demand for high‐performance phase change materials. However, in the realm of phase change materials, there appears to be an inherent contradiction between enhancing crystallization speed and bolstering amorphous stability. In this work, the formation of Ga─Ge bonds associated with Ga single doping are effectively addressed through the deliberate incorporation of GaSb co‐doping. This strategic approach to bonding variety has significantly improved operational speed to a remarkable 8 ns, the crystallization temperature is elevated to 196 °C, and multilevel phase change performance is retained. First‐principles calculations and material characterization is conducted to elucidate the underlying mechanisms responsible for the observed enhancements in both thermal stability and operation speed. This investigation provides valuable insights for optimizing the performance of phase change materials and addresses the pressing challenge of integrating phase change materials into a neuromorphic computing system.
format Article
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institution Kabale University
issn 2199-160X
language English
publishDate 2025-08-01
publisher Wiley-VCH
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series Advanced Electronic Materials
spelling doaj-art-d9d8909b41c34594bf13be7fd48234182025-08-20T03:59:22ZengWiley-VCHAdvanced Electronic Materials2199-160X2025-08-011112n/an/a10.1002/aelm.202500032Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change MemoryKe Gao0Ruizhe Zhao1Xin Li2Jingwei Cai3Hao Tong4Xiangshui Miao5School of Integrated Circuits Huazhong University of Science & Technology Wuhan 430074 ChinaSchool of Integrated Circuits Huazhong University of Science & Technology Wuhan 430074 ChinaSchool of Integrated Circuits Huazhong University of Science & Technology Wuhan 430074 ChinaSchool of Integrated Circuits Huazhong University of Science & Technology Wuhan 430074 ChinaSchool of Integrated Circuits Huazhong University of Science & Technology Wuhan 430074 ChinaSchool of Integrated Circuits Huazhong University of Science & Technology Wuhan 430074 ChinaAbstract Chalcogenide phase change memory, a next‐generation non‐volatile memory technology, holds significant promise in neuromorphic computing, leading to an urgent demand for high‐performance phase change materials. However, in the realm of phase change materials, there appears to be an inherent contradiction between enhancing crystallization speed and bolstering amorphous stability. In this work, the formation of Ga─Ge bonds associated with Ga single doping are effectively addressed through the deliberate incorporation of GaSb co‐doping. This strategic approach to bonding variety has significantly improved operational speed to a remarkable 8 ns, the crystallization temperature is elevated to 196 °C, and multilevel phase change performance is retained. First‐principles calculations and material characterization is conducted to elucidate the underlying mechanisms responsible for the observed enhancements in both thermal stability and operation speed. This investigation provides valuable insights for optimizing the performance of phase change materials and addresses the pressing challenge of integrating phase change materials into a neuromorphic computing system.https://doi.org/10.1002/aelm.202500032Ga─Sb bondhigh speedhigh thermal stabilitylinear and symmetric resistancephase change memory
spellingShingle Ke Gao
Ruizhe Zhao
Xin Li
Jingwei Cai
Hao Tong
Xiangshui Miao
Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change Memory
Advanced Electronic Materials
Ga─Sb bond
high speed
high thermal stability
linear and symmetric resistance
phase change memory
title Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change Memory
title_full Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change Memory
title_fullStr Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change Memory
title_full_unstemmed Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change Memory
title_short Enhancing Ga─Sb Bonds by GaSb Co‐Doping Ge2Sb2Te5 for High Speed and Thermal Stability Phase Change Memory
title_sort enhancing ga─sb bonds by gasb co doping ge2sb2te5 for high speed and thermal stability phase change memory
topic Ga─Sb bond
high speed
high thermal stability
linear and symmetric resistance
phase change memory
url https://doi.org/10.1002/aelm.202500032
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