Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteries

Abstract To drive electronic devices for a long range, the energy density of Li‐ion batteries must be further enhanced, and high‐energy cathode materials are required. Among the cathode materials, LiCoO2 (LCO) is one of the most promising candidates when charged to higher voltages over 4.3 V. Howeve...

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Main Authors: Xiaoshuang Ma, Jinkun Wang, Zehua Wang, Li Wang, Hong Xu, Xiangming He
Format: Article
Language:English
Published: Wiley 2024-08-01
Series:Electron
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Online Access:https://doi.org/10.1002/elt2.33
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author Xiaoshuang Ma
Jinkun Wang
Zehua Wang
Li Wang
Hong Xu
Xiangming He
author_facet Xiaoshuang Ma
Jinkun Wang
Zehua Wang
Li Wang
Hong Xu
Xiangming He
author_sort Xiaoshuang Ma
collection DOAJ
description Abstract To drive electronic devices for a long range, the energy density of Li‐ion batteries must be further enhanced, and high‐energy cathode materials are required. Among the cathode materials, LiCoO2 (LCO) is one of the most promising candidates when charged to higher voltages over 4.3 V. However, high‐voltage LCO materials are confronted with severe surface and bulk issues inducing poor cyclic stability. To completely unleash the potential of LCO cathodes, a more comprehensive theoretical understanding of the underlying issues is necessary, along with active exploration of previous modifications. This paper mainly presents the degradation mechanisms of LCO under high voltage, the formation and evolution mechanisms of the cathode electrolyte interface, and the surface engineering strategies employed to enhance the cell performance. By organizing and summarizing these modifications, this work aims to establish associations among common research issues and to suggest future research priorities, thus facilitating the rapid development of high‐voltage LCO.
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spelling doaj-art-d9a43b9bc99741089efd7c8cb2bd150e2025-08-20T03:22:15ZengWileyElectron2751-26062751-26142024-08-0123n/an/a10.1002/elt2.33Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteriesXiaoshuang Ma0Jinkun Wang1Zehua Wang2Li Wang3Hong Xu4Xiangming He5School of Chemistry and Chemical Engineering Southeast University Nanjing ChinaInstitute of Nuclear and New Energy Technology Tsinghua University Beijing ChinaInstitute of Nuclear and New Energy Technology Tsinghua University Beijing ChinaInstitute of Nuclear and New Energy Technology Tsinghua University Beijing ChinaInstitute of Nuclear and New Energy Technology Tsinghua University Beijing ChinaInstitute of Nuclear and New Energy Technology Tsinghua University Beijing ChinaAbstract To drive electronic devices for a long range, the energy density of Li‐ion batteries must be further enhanced, and high‐energy cathode materials are required. Among the cathode materials, LiCoO2 (LCO) is one of the most promising candidates when charged to higher voltages over 4.3 V. However, high‐voltage LCO materials are confronted with severe surface and bulk issues inducing poor cyclic stability. To completely unleash the potential of LCO cathodes, a more comprehensive theoretical understanding of the underlying issues is necessary, along with active exploration of previous modifications. This paper mainly presents the degradation mechanisms of LCO under high voltage, the formation and evolution mechanisms of the cathode electrolyte interface, and the surface engineering strategies employed to enhance the cell performance. By organizing and summarizing these modifications, this work aims to establish associations among common research issues and to suggest future research priorities, thus facilitating the rapid development of high‐voltage LCO.https://doi.org/10.1002/elt2.33coatingdopingelectrolyte additiveshigh‐voltage LiCoO2lithium‐ion batteries
spellingShingle Xiaoshuang Ma
Jinkun Wang
Zehua Wang
Li Wang
Hong Xu
Xiangming He
Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteries
Electron
coating
doping
electrolyte additives
high‐voltage LiCoO2
lithium‐ion batteries
title Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteries
title_full Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteries
title_fullStr Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteries
title_full_unstemmed Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteries
title_short Engineering strategies for high‐voltage LiCoO2 based high‐energy Li‐ion batteries
title_sort engineering strategies for high voltage licoo2 based high energy li ion batteries
topic coating
doping
electrolyte additives
high‐voltage LiCoO2
lithium‐ion batteries
url https://doi.org/10.1002/elt2.33
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AT zehuawang engineeringstrategiesforhighvoltagelicoo2basedhighenergyliionbatteries
AT liwang engineeringstrategiesforhighvoltagelicoo2basedhighenergyliionbatteries
AT hongxu engineeringstrategiesforhighvoltagelicoo2basedhighenergyliionbatteries
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