Degradation Mechanisms of Cellulose-Based Transformer Insulation: The Role of Dissolved Gases and Macromolecular Characterisation

The ageing of cellulose paper-based transformer insulation is a critical factor influencing the reliability and lifespan of power transformers, as insulating paper is not easily replaced or repaired. Therefore, this review explores the degradation mechanisms of insulating paper, emphasising the role...

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Bibliographic Details
Main Authors: Andrew Adewunmi Adekunle, Samson Okikiola Oparanti, Issouf Fofana, Patrick Picher, Esperanza Mariela Rodriguez-Celis, Oscar Henry Arroyo-Fernandez, Fethi Meghnefi
Format: Article
Language:English
Published: MDPI AG 2025-05-01
Series:Macromol
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Online Access:https://www.mdpi.com/2673-6209/5/2/20
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Summary:The ageing of cellulose paper-based transformer insulation is a critical factor influencing the reliability and lifespan of power transformers, as insulating paper is not easily replaced or repaired. Therefore, this review explores the degradation mechanisms of insulating paper, emphasising the roles of dissolved gases, chemical markers, and macromolecular characterisation in assessing paper deterioration. Likewise, the impact of moisture and thermal stress on the breakdown of cellulose fibres are discussed, especially acid hydrolysis, which serves as the main degradation mechanism in cellulose insulating paper. Advanced diagnostic techniques for insulation condition monitoring, such as molecular simulations, glass transition temperature analysis, and DP estimation models, are highlighted. Furthermore, special attention is given to natural esters as alternative insulating liquids, demonstrating their ability to slow cellulose ageing through moisture absorption, hydrogen bonding stabilisation, and transesterification reactions. This paper also evaluates key chemical markers, including 2FAL and methanol, for estimating paper degradation. A comprehensive understanding of these mechanisms and diagnostic approaches can enhance predictive maintenance strategies and improve transformer longevity.
ISSN:2673-6209