Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicing
This study of manganese (Mn, Z = 25) introduces a novel combination of extended-range high energy resolution fluorescence detection (XR-HERFD), multiple-crystal spectrometers and advanced binary data splicing techniques to address challenges in X-ray emission spectroscopy. XR-HERFD enhances spectral...
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| Format: | Article |
| Language: | English |
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International Union of Crystallography
2025-07-01
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| Series: | Journal of Synchrotron Radiation |
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| Online Access: | https://journals.iucr.org/paper?S1600577525004084 |
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| author | Ramesh Rijal Jack Stephens Daniel Sier Nicholas T. T. Tran Truong V. B. Nguyen Jonathan W. Dean Pierce Bowman Minh Dao Paul Di Pasquale Tony Kirk Chanh Q. Tran Shusaku Hayama Matteo Aramini Nitya Ramanan Sofia Diaz-Moreno Christopher T. Chantler |
| author_facet | Ramesh Rijal Jack Stephens Daniel Sier Nicholas T. T. Tran Truong V. B. Nguyen Jonathan W. Dean Pierce Bowman Minh Dao Paul Di Pasquale Tony Kirk Chanh Q. Tran Shusaku Hayama Matteo Aramini Nitya Ramanan Sofia Diaz-Moreno Christopher T. Chantler |
| author_sort | Ramesh Rijal |
| collection | DOAJ |
| description | This study of manganese (Mn, Z = 25) introduces a novel combination of extended-range high energy resolution fluorescence detection (XR-HERFD), multiple-crystal spectrometers and advanced binary data splicing techniques to address challenges in X-ray emission spectroscopy. XR-HERFD enhances spectral precision by utilizing high-resolution crystal analysers and optimized detector configurations. The systematic application of these methods using multiple Bragg crystal analysers at Diamond Light Source has led to substantial improvements in data quality. Simultaneously, advanced binary data splicing integrates multiple datasets to correct distortions and improve resolution, resulting in sharper spectral features. Our results show a significant increase in peak counts and a notable reduction in full width at half-maximum (FWHM), with peak amplitudes increasing by 83% and resolution improving by 46%. These developments provide greater detail for X-ray absorption or emission spectra, offering valuable insights into complex materials, and permitting advances and breakthroughs in atomic relativistic quantum mechanics, chemical sensitivity of atomic transitions and modelling of solid-state effects. |
| format | Article |
| id | doaj-art-d873d1358d5746ee95062c63af2a536a |
| institution | DOAJ |
| issn | 1600-5775 |
| language | English |
| publishDate | 2025-07-01 |
| publisher | International Union of Crystallography |
| record_format | Article |
| series | Journal of Synchrotron Radiation |
| spelling | doaj-art-d873d1358d5746ee95062c63af2a536a2025-08-20T03:17:39ZengInternational Union of CrystallographyJournal of Synchrotron Radiation1600-57752025-07-01324994100910.1107/S1600577525004084rv5191Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicingRamesh Rijal0Jack Stephens1Daniel Sier2Nicholas T. T. Tran3Truong V. B. Nguyen4Jonathan W. Dean5Pierce Bowman6Minh Dao7Paul Di Pasquale8Tony Kirk9Chanh Q. Tran10Shusaku Hayama11Matteo Aramini12Nitya Ramanan13Sofia Diaz-Moreno14Christopher T. Chantler15School of Physics, University of Melbourne, Melbourne, Victoria, AustraliaSchool of Physics, University of Melbourne, Melbourne, Victoria, AustraliaSchool of Physics, University of Melbourne, Melbourne, Victoria, AustraliaSchool of Physics, University of Melbourne, Melbourne, Victoria, AustraliaSchool of Physics, University of Melbourne, Melbourne, Victoria, AustraliaSchool of Physics, University of Melbourne, Melbourne, Victoria, AustraliaDepartment of Chemistry and Physics, La Trobe University, Melbourne, Victoria, AustraliaDepartment of Chemistry and Physics, La Trobe University, Melbourne, Victoria, AustraliaDepartment of Chemistry and Physics, La Trobe University, Melbourne, Victoria, AustraliaDepartment of Chemistry and Physics, La Trobe University, Melbourne, Victoria, AustraliaDepartment of Chemistry and Physics, La Trobe University, Melbourne, Victoria, AustraliaDiamond Light Source, Harwell Science and Innovation Campus, Didcot OX11 0DE, United KingdomDiamond Light Source, Harwell Science and Innovation Campus, Didcot OX11 0DE, United KingdomDiamond Light Source, Harwell Science and Innovation Campus, Didcot OX11 0DE, United KingdomDiamond Light Source, Harwell Science and Innovation Campus, Didcot OX11 0DE, United KingdomSchool of Physics, University of Melbourne, Melbourne, Victoria, AustraliaThis study of manganese (Mn, Z = 25) introduces a novel combination of extended-range high energy resolution fluorescence detection (XR-HERFD), multiple-crystal spectrometers and advanced binary data splicing techniques to address challenges in X-ray emission spectroscopy. XR-HERFD enhances spectral precision by utilizing high-resolution crystal analysers and optimized detector configurations. The systematic application of these methods using multiple Bragg crystal analysers at Diamond Light Source has led to substantial improvements in data quality. Simultaneously, advanced binary data splicing integrates multiple datasets to correct distortions and improve resolution, resulting in sharper spectral features. Our results show a significant increase in peak counts and a notable reduction in full width at half-maximum (FWHM), with peak amplitudes increasing by 83% and resolution improving by 46%. These developments provide greater detail for X-ray absorption or emission spectra, offering valuable insights into complex materials, and permitting advances and breakthroughs in atomic relativistic quantum mechanics, chemical sensitivity of atomic transitions and modelling of solid-state effects.https://journals.iucr.org/paper?S1600577525004084xr-herfdextended-range high energy resolution fluorescence detectionmultiple-crystal spectrometersadvanced binary data splicingmanganese |
| spellingShingle | Ramesh Rijal Jack Stephens Daniel Sier Nicholas T. T. Tran Truong V. B. Nguyen Jonathan W. Dean Pierce Bowman Minh Dao Paul Di Pasquale Tony Kirk Chanh Q. Tran Shusaku Hayama Matteo Aramini Nitya Ramanan Sofia Diaz-Moreno Christopher T. Chantler Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicing Journal of Synchrotron Radiation xr-herfd extended-range high energy resolution fluorescence detection multiple-crystal spectrometers advanced binary data splicing manganese |
| title | Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicing |
| title_full | Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicing |
| title_fullStr | Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicing |
| title_full_unstemmed | Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicing |
| title_short | Hyper-resolution in X-ray emission spectroscopy: integrating extended-range high energy resolution fluorescence detection and multiple-crystal spectrometry with advanced binary data splicing |
| title_sort | hyper resolution in x ray emission spectroscopy integrating extended range high energy resolution fluorescence detection and multiple crystal spectrometry with advanced binary data splicing |
| topic | xr-herfd extended-range high energy resolution fluorescence detection multiple-crystal spectrometers advanced binary data splicing manganese |
| url | https://journals.iucr.org/paper?S1600577525004084 |
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