The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic Acid

This study investigated the different viscosity effects of natural isoprene rubber (NR) compared to the synthetic one (IR) on toughening of polylactic acid (PLA). Here, 15 wt% rubber was melt blended with PLA in an internal mixer at 180°C and 50 rpm. It was found that the addition of these rubbers l...

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Main Authors: Supanut Phattarateera, Cattaleeya Pattamaprom
Format: Article
Language:English
Published: Wiley 2019-01-01
Series:International Journal of Polymer Science
Online Access:http://dx.doi.org/10.1155/2019/5679871
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author Supanut Phattarateera
Cattaleeya Pattamaprom
author_facet Supanut Phattarateera
Cattaleeya Pattamaprom
author_sort Supanut Phattarateera
collection DOAJ
description This study investigated the different viscosity effects of natural isoprene rubber (NR) compared to the synthetic one (IR) on toughening of polylactic acid (PLA). Here, 15 wt% rubber was melt blended with PLA in an internal mixer at 180°C and 50 rpm. It was found that the addition of these rubbers led to a significant increase in the tensile toughness and impact strength. These rubbers were masticated at 50°C and at 200 rpm for various mastication times to reduce their molecular weights. A too-long mastication time was found to adversely affect the impact strength and tensile toughness due to the fast agglomeration of rubber particles. At a comparable viscosity, it was remarkable that the impact strength of PLA/NR was higher than that of PLA/IR regardless of the similar chemical structures probably because the presence of nonrubber components including proteins and lipids could enhance the interfacial interaction between NR and the PLA matrix.
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issn 1687-9422
1687-9430
language English
publishDate 2019-01-01
publisher Wiley
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series International Journal of Polymer Science
spelling doaj-art-d809c863c2cf4d629fca4a3124a013222025-08-20T02:21:11ZengWileyInternational Journal of Polymer Science1687-94221687-94302019-01-01201910.1155/2019/56798715679871The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic AcidSupanut Phattarateera0Cattaleeya Pattamaprom1Department of Chemical Engineering, Thammasat School of Engineering, Thammasat University, Pathum Thani 12120, ThailandDepartment of Chemical Engineering, Thammasat School of Engineering, Thammasat University, Pathum Thani 12120, ThailandThis study investigated the different viscosity effects of natural isoprene rubber (NR) compared to the synthetic one (IR) on toughening of polylactic acid (PLA). Here, 15 wt% rubber was melt blended with PLA in an internal mixer at 180°C and 50 rpm. It was found that the addition of these rubbers led to a significant increase in the tensile toughness and impact strength. These rubbers were masticated at 50°C and at 200 rpm for various mastication times to reduce their molecular weights. A too-long mastication time was found to adversely affect the impact strength and tensile toughness due to the fast agglomeration of rubber particles. At a comparable viscosity, it was remarkable that the impact strength of PLA/NR was higher than that of PLA/IR regardless of the similar chemical structures probably because the presence of nonrubber components including proteins and lipids could enhance the interfacial interaction between NR and the PLA matrix.http://dx.doi.org/10.1155/2019/5679871
spellingShingle Supanut Phattarateera
Cattaleeya Pattamaprom
The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic Acid
International Journal of Polymer Science
title The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic Acid
title_full The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic Acid
title_fullStr The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic Acid
title_full_unstemmed The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic Acid
title_short The Viscosity Effect of Masticated Natural vs. Synthetic Isoprene Rubber on Toughening of Polylactic Acid
title_sort viscosity effect of masticated natural vs synthetic isoprene rubber on toughening of polylactic acid
url http://dx.doi.org/10.1155/2019/5679871
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