Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass Models

Glass curators often question how their treatments affect the long-term stability of historical glass. While damp cotton swabs are commonly used to remove surface salts and dust, the use of water remains controversial, particularly for heavily altered glass, due to concerns about worsening hydration...

Full description

Saved in:
Bibliographic Details
Main Authors: Thalie Law, Odile Majérus, Marie Godet, Mélanie Moskura, Thibault Charpentier, Antoine Seyeux, Daniel Caurant
Format: Article
Language:English
Published: MDPI AG 2025-07-01
Series:Heritage
Subjects:
Online Access:https://www.mdpi.com/2571-9408/8/7/276
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849407066053017600
author Thalie Law
Odile Majérus
Marie Godet
Mélanie Moskura
Thibault Charpentier
Antoine Seyeux
Daniel Caurant
author_facet Thalie Law
Odile Majérus
Marie Godet
Mélanie Moskura
Thibault Charpentier
Antoine Seyeux
Daniel Caurant
author_sort Thalie Law
collection DOAJ
description Glass curators often question how their treatments affect the long-term stability of historical glass. While damp cotton swabs are commonly used to remove surface salts and dust, the use of water remains controversial, particularly for heavily altered glass, due to concerns about worsening hydration. This study investigates the effect of water rinsing on an unstable soda-lime glass altered for six months (monoliths) and fifteen months (powders) at 35 °C and 85% relative humidity. Samples were then rinsed with Milli-Q water at 20 °C or 50 °C, and the monolithic glass was subsequently subjected to an additional 15 months of alteration under the same conditions. The glass surface was characterized by optical and scanning electron microscopy (SEM) as well as Raman spectroscopy to identify the nature of the salts. The evolution of the hydrated layer was assessed using transmission FTIR, Raman and solid-state NMR spectroscopies, ToF-SIMS, and thermogravimetric analysis (TGA). The results show that rinsing effectively removes surface salts—primarily sodium carbonate—and induces structural changes in the hydrated layer, promoting silicate network polymerization. Upon resuming alteration, rinsed monolithic samples exhibit no further degradation after the additional 15 months of alteration. These findings offer promising insights for conservation practices and may help curators refining their treatment strategies for altered glass.
format Article
id doaj-art-d796dcd9d71d4328bd18fe0ec9d15711
institution Kabale University
issn 2571-9408
language English
publishDate 2025-07-01
publisher MDPI AG
record_format Article
series Heritage
spelling doaj-art-d796dcd9d71d4328bd18fe0ec9d157112025-08-20T03:36:11ZengMDPI AGHeritage2571-94082025-07-018727610.3390/heritage8070276Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass ModelsThalie Law0Odile Majérus1Marie Godet2Mélanie Moskura3Thibault Charpentier4Antoine Seyeux5Daniel Caurant6Institut de Recherche de Chimie Paris (IRCP), Chimie ParisTech, Université PSL, CNRS, F-75005 Paris, FranceInstitut de Recherche de Chimie Paris (IRCP), Chimie ParisTech, Université PSL, CNRS, F-75005 Paris, FranceInstitut de Recherche de Chimie Paris (IRCP), Chimie ParisTech, Université PSL, CNRS, F-75005 Paris, FranceNIMBE, CEA Saclay, Université Paris-Saclay, CEA, CNRS, F-91191 Gif-sur-Yvette, FranceNIMBE, CEA Saclay, Université Paris-Saclay, CEA, CNRS, F-91191 Gif-sur-Yvette, FranceInstitut de Recherche de Chimie Paris (IRCP), Chimie ParisTech, Université PSL, CNRS, F-75005 Paris, FranceInstitut de Recherche de Chimie Paris (IRCP), Chimie ParisTech, Université PSL, CNRS, F-75005 Paris, FranceGlass curators often question how their treatments affect the long-term stability of historical glass. While damp cotton swabs are commonly used to remove surface salts and dust, the use of water remains controversial, particularly for heavily altered glass, due to concerns about worsening hydration. This study investigates the effect of water rinsing on an unstable soda-lime glass altered for six months (monoliths) and fifteen months (powders) at 35 °C and 85% relative humidity. Samples were then rinsed with Milli-Q water at 20 °C or 50 °C, and the monolithic glass was subsequently subjected to an additional 15 months of alteration under the same conditions. The glass surface was characterized by optical and scanning electron microscopy (SEM) as well as Raman spectroscopy to identify the nature of the salts. The evolution of the hydrated layer was assessed using transmission FTIR, Raman and solid-state NMR spectroscopies, ToF-SIMS, and thermogravimetric analysis (TGA). The results show that rinsing effectively removes surface salts—primarily sodium carbonate—and induces structural changes in the hydrated layer, promoting silicate network polymerization. Upon resuming alteration, rinsed monolithic samples exhibit no further degradation after the additional 15 months of alteration. These findings offer promising insights for conservation practices and may help curators refining their treatment strategies for altered glass.https://www.mdpi.com/2571-9408/8/7/276glassatmospheric alterationdegradationweatheringglass corrosionwater cleaning
spellingShingle Thalie Law
Odile Majérus
Marie Godet
Mélanie Moskura
Thibault Charpentier
Antoine Seyeux
Daniel Caurant
Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass Models
Heritage
glass
atmospheric alteration
degradation
weathering
glass corrosion
water cleaning
title Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass Models
title_full Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass Models
title_fullStr Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass Models
title_full_unstemmed Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass Models
title_short Does Water Cleaning Mitigate Atmospheric Degradation of Unstable Heritage Glass? An Experimental Study on Glass Models
title_sort does water cleaning mitigate atmospheric degradation of unstable heritage glass an experimental study on glass models
topic glass
atmospheric alteration
degradation
weathering
glass corrosion
water cleaning
url https://www.mdpi.com/2571-9408/8/7/276
work_keys_str_mv AT thalielaw doeswatercleaningmitigateatmosphericdegradationofunstableheritageglassanexperimentalstudyonglassmodels
AT odilemajerus doeswatercleaningmitigateatmosphericdegradationofunstableheritageglassanexperimentalstudyonglassmodels
AT mariegodet doeswatercleaningmitigateatmosphericdegradationofunstableheritageglassanexperimentalstudyonglassmodels
AT melaniemoskura doeswatercleaningmitigateatmosphericdegradationofunstableheritageglassanexperimentalstudyonglassmodels
AT thibaultcharpentier doeswatercleaningmitigateatmosphericdegradationofunstableheritageglassanexperimentalstudyonglassmodels
AT antoineseyeux doeswatercleaningmitigateatmosphericdegradationofunstableheritageglassanexperimentalstudyonglassmodels
AT danielcaurant doeswatercleaningmitigateatmosphericdegradationofunstableheritageglassanexperimentalstudyonglassmodels