Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health Risk

Abstract In this study, 75 congeners of polychlorinated naphthalenes (PCNs - the new persistent organic pollutants under the Stockholm Convention) were firstly analyzed in ambient air samples collected at five sites in Vietnam. Results indicated that the concentration of total PCNs ranged from 56.8...

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Main Authors: Ngo Thi Thuan, Nguyen Duy Dat, Nguyen Minh Ngoc, Nhung Thi-Tuyet Hoang, To Thi Hien, Moo Been Chang
Format: Article
Language:English
Published: Springer 2024-06-01
Series:Aerosol and Air Quality Research
Subjects:
Online Access:https://doi.org/10.4209/aaqr.240047
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author Ngo Thi Thuan
Nguyen Duy Dat
Nguyen Minh Ngoc
Nhung Thi-Tuyet Hoang
To Thi Hien
Moo Been Chang
author_facet Ngo Thi Thuan
Nguyen Duy Dat
Nguyen Minh Ngoc
Nhung Thi-Tuyet Hoang
To Thi Hien
Moo Been Chang
author_sort Ngo Thi Thuan
collection DOAJ
description Abstract In this study, 75 congeners of polychlorinated naphthalenes (PCNs - the new persistent organic pollutants under the Stockholm Convention) were firstly analyzed in ambient air samples collected at five sites in Vietnam. Results indicated that the concentration of total PCNs ranged from 56.8 to 263 (pg m–3) in the dry season and 12.9 to 208 (pg m–3) in the rainy season. Gaseous PCNs dominated in both seasons, however, the contribution of particulate PCNs increased in the rainy season. Two typical homologue profiles were found in ambient air samples, including low-chlorinated PCNs (monoCNs > diCNs > triCNs) and medium-chlorinated PCNs (tetraCNs > triCNs). Principal component analysis indicated that atmospheric PCNs might be derived from three typical sources including evaporation from products containing PCNs (42.7%), primary emission from combustion-related sources (20.8%), and flue gas after treatment (11.9%). Cluster analysis and diagnostic ratios of typical PCNs indicated that PCNs in each sample might be contributed by different sources with varying magnitudes. The results of the health risk assessment reveal that low risk is associated with atmospheric PCNs in Ho Chi Minh City, Vietnam. This study provides useful information on the characteristics of PCNs in Vietnam, thereby bridging the knowledge divide regarding the pollution of new POPs in developing countries.
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spelling doaj-art-d544ebc823854074a34139309ea8c2cd2025-02-09T12:24:26ZengSpringerAerosol and Air Quality Research1680-85842071-14092024-06-0124811710.4209/aaqr.240047Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health RiskNgo Thi Thuan0Nguyen Duy Dat1Nguyen Minh Ngoc2Nhung Thi-Tuyet Hoang3To Thi Hien4Moo Been Chang5School of Chemical and Environmental Engineering, International UniversityFaculty of Chemical and Food Technology, Ho Chi Minh City University of Technology and EducationVietnam National UniversityFaculty of Chemical and Food Technology, Ho Chi Minh City University of Technology and EducationVietnam National UniversityGraduate Institute of Environmental Engineering, National Central University (NCU)Abstract In this study, 75 congeners of polychlorinated naphthalenes (PCNs - the new persistent organic pollutants under the Stockholm Convention) were firstly analyzed in ambient air samples collected at five sites in Vietnam. Results indicated that the concentration of total PCNs ranged from 56.8 to 263 (pg m–3) in the dry season and 12.9 to 208 (pg m–3) in the rainy season. Gaseous PCNs dominated in both seasons, however, the contribution of particulate PCNs increased in the rainy season. Two typical homologue profiles were found in ambient air samples, including low-chlorinated PCNs (monoCNs > diCNs > triCNs) and medium-chlorinated PCNs (tetraCNs > triCNs). Principal component analysis indicated that atmospheric PCNs might be derived from three typical sources including evaporation from products containing PCNs (42.7%), primary emission from combustion-related sources (20.8%), and flue gas after treatment (11.9%). Cluster analysis and diagnostic ratios of typical PCNs indicated that PCNs in each sample might be contributed by different sources with varying magnitudes. The results of the health risk assessment reveal that low risk is associated with atmospheric PCNs in Ho Chi Minh City, Vietnam. This study provides useful information on the characteristics of PCNs in Vietnam, thereby bridging the knowledge divide regarding the pollution of new POPs in developing countries.https://doi.org/10.4209/aaqr.240047Air pollutionDioxin-like compoundsHealth risk assessmentHo Chi Minh CityPCNs
spellingShingle Ngo Thi Thuan
Nguyen Duy Dat
Nguyen Minh Ngoc
Nhung Thi-Tuyet Hoang
To Thi Hien
Moo Been Chang
Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health Risk
Aerosol and Air Quality Research
Air pollution
Dioxin-like compounds
Health risk assessment
Ho Chi Minh City
PCNs
title Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health Risk
title_full Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health Risk
title_fullStr Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health Risk
title_full_unstemmed Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health Risk
title_short Atmospheric Polychlorinated Naphthalenes in a Tropical Megalopolis of Vietnam: Concentrations, Potential Sources, and Health Risk
title_sort atmospheric polychlorinated naphthalenes in a tropical megalopolis of vietnam concentrations potential sources and health risk
topic Air pollution
Dioxin-like compounds
Health risk assessment
Ho Chi Minh City
PCNs
url https://doi.org/10.4209/aaqr.240047
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