Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic Site

Abstract Positive Matrix Factorization was used for source apportionment of 2-hour online metals (Xact625i; PM2.5) and elemental and organic carbon (EC/OC analyser; PM1) data at an urban traffic site in Prague, Czech Republic, for two month-long periods in spring (February–March) and winter (Novembe...

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Main Authors: Laurence C. Windell, Petra Pokorná, Jaroslav Schwarz, Petr Vodička, Philip K. Hopke, Naděžda Zíková, Radek Lhotka, Jakub Ondráček, Petr Roztočil, Michal Vojtišek, Vladimír Ždímal
Format: Article
Language:English
Published: Springer 2024-05-01
Series:Aerosol and Air Quality Research
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Online Access:https://doi.org/10.4209/aaqr.240058
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author Laurence C. Windell
Petra Pokorná
Jaroslav Schwarz
Petr Vodička
Philip K. Hopke
Naděžda Zíková
Radek Lhotka
Jakub Ondráček
Petr Roztočil
Michal Vojtišek
Vladimír Ždímal
author_facet Laurence C. Windell
Petra Pokorná
Jaroslav Schwarz
Petr Vodička
Philip K. Hopke
Naděžda Zíková
Radek Lhotka
Jakub Ondráček
Petr Roztočil
Michal Vojtišek
Vladimír Ždímal
author_sort Laurence C. Windell
collection DOAJ
description Abstract Positive Matrix Factorization was used for source apportionment of 2-hour online metals (Xact625i; PM2.5) and elemental and organic carbon (EC/OC analyser; PM1) data at an urban traffic site in Prague, Czech Republic, for two month-long periods in spring (February–March) and winter (November–December), 2020 (400 samples). Five factors were obtained for spring: Local heating (39%), Soil/road dust (21%), Secondary inorganic aerosol (20%), Traffic (12%), and Road salt (9%), while four factors were resolved for winter: Local heating (20%), Soil/road dust (31%), Secondary inorganic aerosol (SIA; 36%), and Traffic (13%). Aside from SIA, the sources were of local origins. Air mass back trajectories calculated by HYSPLIT and concentration weighted trajectories (CWT) were used to identify long-distance sources. Greater PM concentrations during winter (~3 times greater) were attributed to both lower boundary layer heights and more abundant air masses from Central Europe, compared to more marine air masses during spring.
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institution Kabale University
issn 1680-8584
2071-1409
language English
publishDate 2024-05-01
publisher Springer
record_format Article
series Aerosol and Air Quality Research
spelling doaj-art-d4e0765e9cdc4e1daa2151ce76e848a92025-02-09T12:24:25ZengSpringerAerosol and Air Quality Research1680-85842071-14092024-05-0124811710.4209/aaqr.240058Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic SiteLaurence C. Windell0Petra Pokorná1Jaroslav Schwarz2Petr Vodička3Philip K. Hopke4Naděžda Zíková5Radek Lhotka6Jakub Ondráček7Petr Roztočil8Michal Vojtišek9Vladimír Ždímal10Aerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesDepartment of Public Health Sciences, University of Rochester School of Medicine and DentistryAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAerosol Chemistry and Physics Research Group, Institute of Chemical Process Fundamentals of the Czech Academy of SciencesAbstract Positive Matrix Factorization was used for source apportionment of 2-hour online metals (Xact625i; PM2.5) and elemental and organic carbon (EC/OC analyser; PM1) data at an urban traffic site in Prague, Czech Republic, for two month-long periods in spring (February–March) and winter (November–December), 2020 (400 samples). Five factors were obtained for spring: Local heating (39%), Soil/road dust (21%), Secondary inorganic aerosol (20%), Traffic (12%), and Road salt (9%), while four factors were resolved for winter: Local heating (20%), Soil/road dust (31%), Secondary inorganic aerosol (SIA; 36%), and Traffic (13%). Aside from SIA, the sources were of local origins. Air mass back trajectories calculated by HYSPLIT and concentration weighted trajectories (CWT) were used to identify long-distance sources. Greater PM concentrations during winter (~3 times greater) were attributed to both lower boundary layer heights and more abundant air masses from Central Europe, compared to more marine air masses during spring.https://doi.org/10.4209/aaqr.240058PMFOnlineXactEC/OC
spellingShingle Laurence C. Windell
Petra Pokorná
Jaroslav Schwarz
Petr Vodička
Philip K. Hopke
Naděžda Zíková
Radek Lhotka
Jakub Ondráček
Petr Roztočil
Michal Vojtišek
Vladimír Ždímal
Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic Site
Aerosol and Air Quality Research
PMF
Online
Xact
EC/OC
title Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic Site
title_full Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic Site
title_fullStr Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic Site
title_full_unstemmed Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic Site
title_short Highly Time-Resolved Elemental Source Apportionment at a Prague Urban Traffic Site
title_sort highly time resolved elemental source apportionment at a prague urban traffic site
topic PMF
Online
Xact
EC/OC
url https://doi.org/10.4209/aaqr.240058
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