Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic Degradation

The present investigation reports the greener synthesis and characterization of novel acrylic acid grafted amphoteric chitosan/TiO2 (CAT) bionanocomposites using ultrasonic radiations. This was done by grafting of acrylic acid onto chitosan in the presence of potassium persulfate by free radical pol...

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Main Authors: M. Bahal, N. Kaur, Nidhi Sharotri, Dhiraj Sud
Format: Article
Language:English
Published: Wiley 2019-01-01
Series:Advances in Polymer Technology
Online Access:http://dx.doi.org/10.1155/2019/2345631
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author M. Bahal
N. Kaur
Nidhi Sharotri
Dhiraj Sud
author_facet M. Bahal
N. Kaur
Nidhi Sharotri
Dhiraj Sud
author_sort M. Bahal
collection DOAJ
description The present investigation reports the greener synthesis and characterization of novel acrylic acid grafted amphoteric chitosan/TiO2 (CAT) bionanocomposites using ultrasonic radiations. This was done by grafting of acrylic acid onto chitosan in the presence of potassium persulfate by free radical polymerization reaction. The uniform distribution of metal oxide in CA/TiO2 nanocomposites was achieved on grafted acrylic acid/chitosan which contains a weak anionic group (-COOH) using ultrasonication technique. Physiochemical techniques such as X-ray diffraction (XRD), field emission scanning electron microscope (FE-SEM), Fourier Transform Infra-Red spectroscopy (FT-IR), Energy Dispersive X-ray spectroscopy (EDX), and Thermal Gravimetric Analysis (TGA) were employed to characterize synthesized CAT. Nanocomposite CAT was applied for degradation of industrial dye. Malachite green (MG) often presents in the waste waters. The degradation kinetics were studied by monitoring the photocatalytic reaction for degradation of MG under visible light, and the rate constant of the reaction was found to be 7.13x10−3min−1. The current research work opens vistas for the new dimensions in the area of water treatment by solving the issues related to degradation reaction efficiency in visible light and cost effectiveness.
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spelling doaj-art-d46f46e2c5b54552bc2f89438a91900b2025-08-20T03:23:47ZengWileyAdvances in Polymer Technology0730-66791098-23292019-01-01201910.1155/2019/23456312345631Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic DegradationM. Bahal0N. Kaur1Nidhi Sharotri2Dhiraj Sud3Department of Chemistry, Sant Longowal Institute of Engineering and Technology (Deemed University), Longowal 148106, Sangrur, Punjab, IndiaDepartment of Chemical Technology, Sant Longowal Institute of Engineering and Technology (Deemed University), Longowal 148106, Sangrur, Punjab, IndiaDepartment of Chemistry, Sant Longowal Institute of Engineering and Technology (Deemed University), Longowal 148106, Sangrur, Punjab, IndiaDepartment of Chemistry, Sant Longowal Institute of Engineering and Technology (Deemed University), Longowal 148106, Sangrur, Punjab, IndiaThe present investigation reports the greener synthesis and characterization of novel acrylic acid grafted amphoteric chitosan/TiO2 (CAT) bionanocomposites using ultrasonic radiations. This was done by grafting of acrylic acid onto chitosan in the presence of potassium persulfate by free radical polymerization reaction. The uniform distribution of metal oxide in CA/TiO2 nanocomposites was achieved on grafted acrylic acid/chitosan which contains a weak anionic group (-COOH) using ultrasonication technique. Physiochemical techniques such as X-ray diffraction (XRD), field emission scanning electron microscope (FE-SEM), Fourier Transform Infra-Red spectroscopy (FT-IR), Energy Dispersive X-ray spectroscopy (EDX), and Thermal Gravimetric Analysis (TGA) were employed to characterize synthesized CAT. Nanocomposite CAT was applied for degradation of industrial dye. Malachite green (MG) often presents in the waste waters. The degradation kinetics were studied by monitoring the photocatalytic reaction for degradation of MG under visible light, and the rate constant of the reaction was found to be 7.13x10−3min−1. The current research work opens vistas for the new dimensions in the area of water treatment by solving the issues related to degradation reaction efficiency in visible light and cost effectiveness.http://dx.doi.org/10.1155/2019/2345631
spellingShingle M. Bahal
N. Kaur
Nidhi Sharotri
Dhiraj Sud
Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic Degradation
Advances in Polymer Technology
title Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic Degradation
title_full Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic Degradation
title_fullStr Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic Degradation
title_full_unstemmed Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic Degradation
title_short Investigations on Amphoteric Chitosan/TiO2 Bionanocomposites for Application in Visible Light Induced Photocatalytic Degradation
title_sort investigations on amphoteric chitosan tio2 bionanocomposites for application in visible light induced photocatalytic degradation
url http://dx.doi.org/10.1155/2019/2345631
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AT nkaur investigationsonamphotericchitosantio2bionanocompositesforapplicationinvisiblelightinducedphotocatalyticdegradation
AT nidhisharotri investigationsonamphotericchitosantio2bionanocompositesforapplicationinvisiblelightinducedphotocatalyticdegradation
AT dhirajsud investigationsonamphotericchitosantio2bionanocompositesforapplicationinvisiblelightinducedphotocatalyticdegradation