Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)

Lactic acid recovery and reusability for hydrolysis of cellulose offers an economical method and produces fewer waste streams. Successful lactic acid recovery up to three recycle times efficiently hydrolyzed NCs with rod-shape morphology. However, after four cycles, the nanocrystalline cellulose yie...

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Main Authors: Holilah Holilah, Lisman Suryanegara, Hasliza Bahruji, Zuratul Ain Abdul Hamid, Muhammad Sapto Wahyudi, Nanang Masruchin, Asranudin Asranudin, RH. Fitri Faradilla, Edi Syafri, Alvina Tata Melenia, Stella Jovita, Reva Edra Nugraha, Didik Prasetyoko
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Case Studies in Chemical and Environmental Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2666016424003165
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author Holilah Holilah
Lisman Suryanegara
Hasliza Bahruji
Zuratul Ain Abdul Hamid
Muhammad Sapto Wahyudi
Nanang Masruchin
Asranudin Asranudin
RH. Fitri Faradilla
Edi Syafri
Alvina Tata Melenia
Stella Jovita
Reva Edra Nugraha
Didik Prasetyoko
author_facet Holilah Holilah
Lisman Suryanegara
Hasliza Bahruji
Zuratul Ain Abdul Hamid
Muhammad Sapto Wahyudi
Nanang Masruchin
Asranudin Asranudin
RH. Fitri Faradilla
Edi Syafri
Alvina Tata Melenia
Stella Jovita
Reva Edra Nugraha
Didik Prasetyoko
author_sort Holilah Holilah
collection DOAJ
description Lactic acid recovery and reusability for hydrolysis of cellulose offers an economical method and produces fewer waste streams. Successful lactic acid recovery up to three recycle times efficiently hydrolyzed NCs with rod-shape morphology. However, after four cycles, the nanocrystalline cellulose yield reduced from 72.3 % to 48.2 %, forming large nanocelluloses with high crystalline index. Large-size nanocellulose with high zeta potential and thermal stability were obtained with increasing cycles due to inefficient acid diffusion into the rigid crystalline network compared to amorphous cellulose. This study offers a green pathway for hydrolysis nanocellulose using a less corrosive and low toxicity lactic acid than inorganic acids.
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institution Kabale University
issn 2666-0164
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publishDate 2024-12-01
publisher Elsevier
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series Case Studies in Chemical and Environmental Engineering
spelling doaj-art-d44b9e1c07ea498bb69b2c3aed2587072024-12-02T05:06:11ZengElsevierCase Studies in Chemical and Environmental Engineering2666-01642024-12-0110100922Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)Holilah Holilah0Lisman Suryanegara1Hasliza Bahruji2Zuratul Ain Abdul Hamid3Muhammad Sapto Wahyudi4Nanang Masruchin5Asranudin Asranudin6RH. Fitri Faradilla7Edi Syafri8Alvina Tata Melenia9Stella Jovita10Reva Edra Nugraha11Didik Prasetyoko12Research Center for Biomass and Bioproducts, National Research and Innovation Agency of Indonesia (BRIN), Cibinong, 16911, Indonesia; Research Collaboration Center for Nanocellulose, BRIN-Andalas University, Padang, 25163, Indonesia; Corresponding author. Research Center for Biomass and Bioproducts, National Research and Innovation Agency of Indonesia (BRIN), Cibinong, 16911, Indonesia.Research Center for Biomass and Bioproducts, National Research and Innovation Agency of Indonesia (BRIN), Cibinong, 16911, IndonesiaCentre of Advanced Material and Energy Sciences, Universiti Brunei Darussalam, Jl. Tungku Link, BE 1410, BruneiSchool of Materials & Mineral Resources Engineering, Universiti Sains Malaysia, 14300, Nibong Tebal Pulau Pinang, MalaysiaResearch Center for Biomass and Bioproducts, National Research and Innovation Agency of Indonesia (BRIN), Cibinong, 16911, IndonesiaResearch Center for Biomass and Bioproducts, National Research and Innovation Agency of Indonesia (BRIN), Cibinong, 16911, IndonesiaResearch Center for Biomass and Bioproducts, National Research and Innovation Agency of Indonesia (BRIN), Cibinong, 16911, IndonesiaDepartment of Food Science and Technology, Faculty of Agriculture, Halu Oleo University, Kendari, Southeast Sulawesi, IndonesiaDepartment of Agricultural Technology, Politeknik Pertanian Negeri Payakumbuh, West Sumatra, 26271, IndonesiaDepartment of Chemistry, Faculty of Science and Data Analytics, Institut Teknologi Sepuluh Nopember, Surabaya, IndonesiaDepartment of Chemistry, Faculty of Science and Data Analytics, Institut Teknologi Sepuluh Nopember, Surabaya, IndonesiaDepartment of Chemical Engineering, Faculty of Engineering, Universitas Pembangunan Nasional “Veteran” Jawa Timur, Surabaya, 60294, IndonesiaDepartment of Chemistry, Faculty of Science and Data Analytics, Institut Teknologi Sepuluh Nopember, Surabaya, Indonesia; Corresponding author.Lactic acid recovery and reusability for hydrolysis of cellulose offers an economical method and produces fewer waste streams. Successful lactic acid recovery up to three recycle times efficiently hydrolyzed NCs with rod-shape morphology. However, after four cycles, the nanocrystalline cellulose yield reduced from 72.3 % to 48.2 %, forming large nanocelluloses with high crystalline index. Large-size nanocellulose with high zeta potential and thermal stability were obtained with increasing cycles due to inefficient acid diffusion into the rigid crystalline network compared to amorphous cellulose. This study offers a green pathway for hydrolysis nanocellulose using a less corrosive and low toxicity lactic acid than inorganic acids.http://www.sciencedirect.com/science/article/pii/S2666016424003165acid recoverylactic acidNanocrystalline celluloseorganic acidhydrolysis
spellingShingle Holilah Holilah
Lisman Suryanegara
Hasliza Bahruji
Zuratul Ain Abdul Hamid
Muhammad Sapto Wahyudi
Nanang Masruchin
Asranudin Asranudin
RH. Fitri Faradilla
Edi Syafri
Alvina Tata Melenia
Stella Jovita
Reva Edra Nugraha
Didik Prasetyoko
Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)
Case Studies in Chemical and Environmental Engineering
acid recovery
lactic acid
Nanocrystalline cellulose
organic acid
hydrolysis
title Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)
title_full Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)
title_fullStr Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)
title_full_unstemmed Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)
title_short Reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste (piper nigrum L.)
title_sort reusability of lactic acid on hydrolysis of nanocrystalline cellulose from pepper waste piper nigrum l
topic acid recovery
lactic acid
Nanocrystalline cellulose
organic acid
hydrolysis
url http://www.sciencedirect.com/science/article/pii/S2666016424003165
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