In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic Acid

This study introduces a novel recombinant humanised collagen (DuCol) developed through codon optimisation and prokaryotic soluble expression, exhibiting exceptional biocompatibility and bioactivity. Structural integrity was confirmed via RP-HPLC, SEM, and CD spectroscopy. In vitro evaluations reveal...

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Main Authors: Mingjie Tong, Xin Zhou, Jiongni Zhong, Dengjian Qu, Wei Chen, Chun Chen, Yiting Wang, Yaoping Liu, Shaochuan Li, Yuan Xiao, Ning Wang, Chaowan Guo, Qiuling Xie, Sheng Xiong
Format: Article
Language:English
Published: MDPI AG 2025-05-01
Series:Bioengineering
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Online Access:https://www.mdpi.com/2306-5354/12/5/510
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author Mingjie Tong
Xin Zhou
Jiongni Zhong
Dengjian Qu
Wei Chen
Chun Chen
Yiting Wang
Yaoping Liu
Shaochuan Li
Yuan Xiao
Ning Wang
Chaowan Guo
Qiuling Xie
Sheng Xiong
author_facet Mingjie Tong
Xin Zhou
Jiongni Zhong
Dengjian Qu
Wei Chen
Chun Chen
Yiting Wang
Yaoping Liu
Shaochuan Li
Yuan Xiao
Ning Wang
Chaowan Guo
Qiuling Xie
Sheng Xiong
author_sort Mingjie Tong
collection DOAJ
description This study introduces a novel recombinant humanised collagen (DuCol) developed through codon optimisation and prokaryotic soluble expression, exhibiting exceptional biocompatibility and bioactivity. Structural integrity was confirmed via RP-HPLC, SEM, and CD spectroscopy. In vitro evaluations revealed DuCol’s dose-dependent enhancement of NIH-3T3 fibroblast proliferation, adhesion, and migration. In a D-galactose-induced ageing rat model, subcutaneous implantation of DuCol showcased time-dependent anti-ageing effects. Early-stage intervention (30 days post-injection) markedly upregulated COL1A1 expression through the TGF-β/Smad3 pathway activation, outperforming poly-<span style="font-variant: small-caps;">l</span>-lactic acid (PLLA) in collagen deposition. Histological analysis revealed 23.4% greater dermal thickness in DuCol-treated groups compared to PLLA at 90 days. While PLLA exhibited sustained collagen stimulation beyond 90 days, DuCol exhibited superior early-phase efficacy (<i>p</i> < 0.001) with comparable safety profiles (no inflammatory response observed through 180-day monitoring). The combinatorial PLLA/DuCol (P&C) formulation synergistically enhanced dermal regeneration, achieving a 31.7% thicker collagen matrix than monotherapy groups. These results underscore the potential of DuCol as a novel implantable filler material for skin repair and regeneration.
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institution Kabale University
issn 2306-5354
language English
publishDate 2025-05-01
publisher MDPI AG
record_format Article
series Bioengineering
spelling doaj-art-d3f7d978f427469da9c1a73d7f943a8a2025-08-20T03:47:53ZengMDPI AGBioengineering2306-53542025-05-0112551010.3390/bioengineering12050510In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic AcidMingjie Tong0Xin Zhou1Jiongni Zhong2Dengjian Qu3Wei Chen4Chun Chen5Yiting Wang6Yaoping Liu7Shaochuan Li8Yuan Xiao9Ning Wang10Chaowan Guo11Qiuling Xie12Sheng Xiong13Institute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaInstitute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaInstitute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaInstitute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaGuangzhou Huike Biotech Co., Ltd., Guangzhou 510530, ChinaInstitute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaInstitute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaGuangzhou Cheer-Derm Biotech Co., Ltd., Guangzhou 510530, ChinaCollege of Veterinary Medicine, South China Agricultural University, Guangzhou 510642, ChinaGuangdong Marubi Biotech Co., Ltd., Guangzhou 510530, ChinaGuangdong Marubi Biotech Co., Ltd., Guangzhou 510530, ChinaGuangdong Marubi Biotech Co., Ltd., Guangzhou 510530, ChinaInstitute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaInstitute of Biomedicine and National Engineering Research Center of Genetic Medicine, College of Life Science and Technology, Jinan University, Guangzhou 510632, ChinaThis study introduces a novel recombinant humanised collagen (DuCol) developed through codon optimisation and prokaryotic soluble expression, exhibiting exceptional biocompatibility and bioactivity. Structural integrity was confirmed via RP-HPLC, SEM, and CD spectroscopy. In vitro evaluations revealed DuCol’s dose-dependent enhancement of NIH-3T3 fibroblast proliferation, adhesion, and migration. In a D-galactose-induced ageing rat model, subcutaneous implantation of DuCol showcased time-dependent anti-ageing effects. Early-stage intervention (30 days post-injection) markedly upregulated COL1A1 expression through the TGF-β/Smad3 pathway activation, outperforming poly-<span style="font-variant: small-caps;">l</span>-lactic acid (PLLA) in collagen deposition. Histological analysis revealed 23.4% greater dermal thickness in DuCol-treated groups compared to PLLA at 90 days. While PLLA exhibited sustained collagen stimulation beyond 90 days, DuCol exhibited superior early-phase efficacy (<i>p</i> < 0.001) with comparable safety profiles (no inflammatory response observed through 180-day monitoring). The combinatorial PLLA/DuCol (P&C) formulation synergistically enhanced dermal regeneration, achieving a 31.7% thicker collagen matrix than monotherapy groups. These results underscore the potential of DuCol as a novel implantable filler material for skin repair and regeneration.https://www.mdpi.com/2306-5354/12/5/510recombinant collagenskin ageingTGF-β signallingPLLAinjectable biomaterials
spellingShingle Mingjie Tong
Xin Zhou
Jiongni Zhong
Dengjian Qu
Wei Chen
Chun Chen
Yiting Wang
Yaoping Liu
Shaochuan Li
Yuan Xiao
Ning Wang
Chaowan Guo
Qiuling Xie
Sheng Xiong
In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic Acid
Bioengineering
recombinant collagen
skin ageing
TGF-β signalling
PLLA
injectable biomaterials
title In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic Acid
title_full In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic Acid
title_fullStr In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic Acid
title_full_unstemmed In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic Acid
title_short In Vivo Evaluation of the Anti-Skin-Ageing Bioactivity of a Recombinant Dual Humanised Collagen and Poly-L-Lactic Acid
title_sort in vivo evaluation of the anti skin ageing bioactivity of a recombinant dual humanised collagen and poly l lactic acid
topic recombinant collagen
skin ageing
TGF-β signalling
PLLA
injectable biomaterials
url https://www.mdpi.com/2306-5354/12/5/510
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