Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric Detection

A simple and accurate ion chromatography (IC) method with pulsed amperometric detection (PAD) was proposed for the determination of cyanide ion in urine, sweat, and saliva samples. The sample pretreatment relies on alkaline digestion and application of Dionex OnGuard II H cartridge. Under the optimi...

Full description

Saved in:
Bibliographic Details
Main Authors: Ewa Jaszczak, Marek Ruman, Sylwia Narkowicz, Jacek Namieśnik, Żaneta Polkowska
Format: Article
Language:English
Published: Wiley 2017-01-01
Series:Journal of Analytical Methods in Chemistry
Online Access:http://dx.doi.org/10.1155/2017/7157953
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849473472144605184
author Ewa Jaszczak
Marek Ruman
Sylwia Narkowicz
Jacek Namieśnik
Żaneta Polkowska
author_facet Ewa Jaszczak
Marek Ruman
Sylwia Narkowicz
Jacek Namieśnik
Żaneta Polkowska
author_sort Ewa Jaszczak
collection DOAJ
description A simple and accurate ion chromatography (IC) method with pulsed amperometric detection (PAD) was proposed for the determination of cyanide ion in urine, sweat, and saliva samples. The sample pretreatment relies on alkaline digestion and application of Dionex OnGuard II H cartridge. Under the optimized conditions, the method showed good linearity in the range of 1–100 μg/L for urine, 5–100 μg/L for saliva, and 3–100 μg/L for sweat samples with determination coefficients (R)>0.992. Low detection limits (LODs) in the range of 1.8 μg/L, 5.1 μg/L, and 5.8 μg/L for urine, saliva, and sweat samples, respectively, and good repeatability (CV < 3%, n=3) were obtained. The proposed method has been successfully applied to the analysis of human biological samples.
format Article
id doaj-art-d2bcfdc0387844298fd74c9b5f4efce5
institution Kabale University
issn 2090-8865
2090-8873
language English
publishDate 2017-01-01
publisher Wiley
record_format Article
series Journal of Analytical Methods in Chemistry
spelling doaj-art-d2bcfdc0387844298fd74c9b5f4efce52025-08-20T03:24:07ZengWileyJournal of Analytical Methods in Chemistry2090-88652090-88732017-01-01201710.1155/2017/71579537157953Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric DetectionEwa Jaszczak0Marek Ruman1Sylwia Narkowicz2Jacek Namieśnik3Żaneta Polkowska4Department of Analytical Chemistry, Faculty of Chemistry, Gdańsk University of Technology, Narutowicza Str. 11/12, 80-233 Gdańsk, PolandFaculty of Earth Sciences, University of Silesia, Będzińska 60, 41-200 Sosnowiec, PolandDepartment of Analytical Chemistry, Faculty of Chemistry, Gdańsk University of Technology, Narutowicza Str. 11/12, 80-233 Gdańsk, PolandDepartment of Analytical Chemistry, Faculty of Chemistry, Gdańsk University of Technology, Narutowicza Str. 11/12, 80-233 Gdańsk, PolandDepartment of Analytical Chemistry, Faculty of Chemistry, Gdańsk University of Technology, Narutowicza Str. 11/12, 80-233 Gdańsk, PolandA simple and accurate ion chromatography (IC) method with pulsed amperometric detection (PAD) was proposed for the determination of cyanide ion in urine, sweat, and saliva samples. The sample pretreatment relies on alkaline digestion and application of Dionex OnGuard II H cartridge. Under the optimized conditions, the method showed good linearity in the range of 1–100 μg/L for urine, 5–100 μg/L for saliva, and 3–100 μg/L for sweat samples with determination coefficients (R)>0.992. Low detection limits (LODs) in the range of 1.8 μg/L, 5.1 μg/L, and 5.8 μg/L for urine, saliva, and sweat samples, respectively, and good repeatability (CV < 3%, n=3) were obtained. The proposed method has been successfully applied to the analysis of human biological samples.http://dx.doi.org/10.1155/2017/7157953
spellingShingle Ewa Jaszczak
Marek Ruman
Sylwia Narkowicz
Jacek Namieśnik
Żaneta Polkowska
Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric Detection
Journal of Analytical Methods in Chemistry
title Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric Detection
title_full Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric Detection
title_fullStr Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric Detection
title_full_unstemmed Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric Detection
title_short Development of an Analytical Protocol for Determination of Cyanide in Human Biological Samples Based on Application of Ion Chromatography with Pulsed Amperometric Detection
title_sort development of an analytical protocol for determination of cyanide in human biological samples based on application of ion chromatography with pulsed amperometric detection
url http://dx.doi.org/10.1155/2017/7157953
work_keys_str_mv AT ewajaszczak developmentofananalyticalprotocolfordeterminationofcyanideinhumanbiologicalsamplesbasedonapplicationofionchromatographywithpulsedamperometricdetection
AT marekruman developmentofananalyticalprotocolfordeterminationofcyanideinhumanbiologicalsamplesbasedonapplicationofionchromatographywithpulsedamperometricdetection
AT sylwianarkowicz developmentofananalyticalprotocolfordeterminationofcyanideinhumanbiologicalsamplesbasedonapplicationofionchromatographywithpulsedamperometricdetection
AT jaceknamiesnik developmentofananalyticalprotocolfordeterminationofcyanideinhumanbiologicalsamplesbasedonapplicationofionchromatographywithpulsedamperometricdetection
AT zanetapolkowska developmentofananalyticalprotocolfordeterminationofcyanideinhumanbiologicalsamplesbasedonapplicationofionchromatographywithpulsedamperometricdetection