Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reduction

Photocatalysis presents a promising pathway for clean energy generation by leveraging solar energy under environmentally benign conditions with minimal pollutant emissions. However, its widespread application is hindered by low catalytic efficiency, stemming from limited light absorption, rapid reco...

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Main Authors: Chan Woo Lee, Jeong Hyun Kim, Megalamane S. Bootharaju, Taeghwan Hyeon, Byoung-Hoon Lee
Format: Article
Language:English
Published: Tsinghua University Press 2024-12-01
Series:Carbon Future
Subjects:
Online Access:https://www.sciopen.com/article/10.26599/CF.2024.9200025
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author Chan Woo Lee
Jeong Hyun Kim
Megalamane S. Bootharaju
Taeghwan Hyeon
Byoung-Hoon Lee
author_facet Chan Woo Lee
Jeong Hyun Kim
Megalamane S. Bootharaju
Taeghwan Hyeon
Byoung-Hoon Lee
author_sort Chan Woo Lee
collection DOAJ
description Photocatalysis presents a promising pathway for clean energy generation by leveraging solar energy under environmentally benign conditions with minimal pollutant emissions. However, its widespread application is hindered by low catalytic efficiency, stemming from limited light absorption, rapid recombination of photo-excited electrons, and suboptimal charge carrier potential for target reactions. This review discusses advanced strategies to enhance photocatalytic performance by modulating photocatalytic supports and refining co-catalysts. Techniques such as hydrogenation and extrinsic doping of photocatalytic supports are highlighted for their ability to broaden light absorption and prolong electron lifetimes. Additionally, the strategic design of co-catalysts, including the use of nanoclusters and atomically dispersed catalysts, is emphasized for optimizing charge carrier potential and improving atomic utilization efficiency. This review aims to guide researchers in developing high-performance photocatalysts for clean energy applications, including CO2 reduction and plastic waste photoreforming, thereby contributing to the advancement of sustainable energy technologies.
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institution DOAJ
issn 2960-0561
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language English
publishDate 2024-12-01
publisher Tsinghua University Press
record_format Article
series Carbon Future
spelling doaj-art-d1fbc93e118c48668c471cf3c5e6c5842025-08-20T02:40:33ZengTsinghua University PressCarbon Future2960-05612960-04212024-12-0114920002510.26599/CF.2024.9200025Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reductionChan Woo Lee0https://orcid.org/0000-0002-9358-6893Jeong Hyun Kim1Megalamane S. Bootharaju2Taeghwan Hyeon3https://orcid.org/0000-0001-5959-6257Byoung-Hoon Lee4https://orcid.org/0000-0002-0482-2859Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of KoreaCenter for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of KoreaCenter for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of KoreaCenter for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of KoreaCenter for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of KoreaPhotocatalysis presents a promising pathway for clean energy generation by leveraging solar energy under environmentally benign conditions with minimal pollutant emissions. However, its widespread application is hindered by low catalytic efficiency, stemming from limited light absorption, rapid recombination of photo-excited electrons, and suboptimal charge carrier potential for target reactions. This review discusses advanced strategies to enhance photocatalytic performance by modulating photocatalytic supports and refining co-catalysts. Techniques such as hydrogenation and extrinsic doping of photocatalytic supports are highlighted for their ability to broaden light absorption and prolong electron lifetimes. Additionally, the strategic design of co-catalysts, including the use of nanoclusters and atomically dispersed catalysts, is emphasized for optimizing charge carrier potential and improving atomic utilization efficiency. This review aims to guide researchers in developing high-performance photocatalysts for clean energy applications, including CO2 reduction and plastic waste photoreforming, thereby contributing to the advancement of sustainable energy technologies.https://www.sciopen.com/article/10.26599/CF.2024.9200025photocatalystsclean energy productionphotocatalytic co2 reductionphotoreforming of plastic wastes
spellingShingle Chan Woo Lee
Jeong Hyun Kim
Megalamane S. Bootharaju
Taeghwan Hyeon
Byoung-Hoon Lee
Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reduction
Carbon Future
photocatalysts
clean energy production
photocatalytic co2 reduction
photoreforming of plastic wastes
title Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reduction
title_full Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reduction
title_fullStr Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reduction
title_full_unstemmed Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reduction
title_short Synthesis of high-performance photocatalysts for solar-driven hydrogen production and carbon dioxide reduction
title_sort synthesis of high performance photocatalysts for solar driven hydrogen production and carbon dioxide reduction
topic photocatalysts
clean energy production
photocatalytic co2 reduction
photoreforming of plastic wastes
url https://www.sciopen.com/article/10.26599/CF.2024.9200025
work_keys_str_mv AT chanwoolee synthesisofhighperformancephotocatalystsforsolardrivenhydrogenproductionandcarbondioxidereduction
AT jeonghyunkim synthesisofhighperformancephotocatalystsforsolardrivenhydrogenproductionandcarbondioxidereduction
AT megalamanesbootharaju synthesisofhighperformancephotocatalystsforsolardrivenhydrogenproductionandcarbondioxidereduction
AT taeghwanhyeon synthesisofhighperformancephotocatalystsforsolardrivenhydrogenproductionandcarbondioxidereduction
AT byounghoonlee synthesisofhighperformancephotocatalystsforsolardrivenhydrogenproductionandcarbondioxidereduction