Role of Hornification of Cellulose Rich Biomass for Pellet Production

Hornification of cellulose-rich materials, particularly wood pulps, occurs when chemical bonds form between cellulose surfaces, along with intermolecular forces created during dewatering and drying, preventing the material from reswelling in water to its original structure. Hornification of pulps re...

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Main Authors: Björn Sjöstrand, Gunnar Henriksson, Carl-Anton Karlsson, Jonas Berghel
Format: Article
Language:English
Published: North Carolina State University 2025-07-01
Series:BioResources
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Online Access:https://ojs.bioresources.com/index.php/BRJ/article/view/24793
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author Björn Sjöstrand
Gunnar Henriksson
Carl-Anton Karlsson
Jonas Berghel
author_facet Björn Sjöstrand
Gunnar Henriksson
Carl-Anton Karlsson
Jonas Berghel
author_sort Björn Sjöstrand
collection DOAJ
description Hornification of cellulose-rich materials, particularly wood pulps, occurs when chemical bonds form between cellulose surfaces, along with intermolecular forces created during dewatering and drying, preventing the material from reswelling in water to its original structure. Hornification of pulps results in a reduced ability to form effective fiber networks and therefore weaker paper products. The objective of this work was to investigate the role of hornification in pelletized cellulosic biomass and materials in general to provide more information than can be obtained by measuring standard wet state properties, such as water retention. Pellets were produced from chemical pulps with different degrees of hornification, as indicated by the water retention value (WRV), and their mechanical performance was evaluated. The chemical pulps served as a model material for investigating hornification. Pulps with higher hornification produced pellets with inferior mechanical properties, which has not been shown before by such a test. This effect is attributed to increased fiber stiffness and reduced surface flexibility, which limits fiber-fiber bonding. In addition, high drying temperatures prior to pelletizing, and thus higher hornification, will increase compression energy and friction in the pelletizing process. A novel connection was observed between WRV and mechanical performance, highlighting the impact of hornification on the surface interactions of cellulose-based materials.
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institution Kabale University
issn 1930-2126
language English
publishDate 2025-07-01
publisher North Carolina State University
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series BioResources
spelling doaj-art-d140efa06e7944248fbb9551aec4f08e2025-08-20T03:43:55ZengNorth Carolina State UniversityBioResources1930-21262025-07-01203746374753136Role of Hornification of Cellulose Rich Biomass for Pellet ProductionBjörn Sjöstrand0https://orcid.org/0000-0003-4023-594XGunnar Henriksson1https://orcid.org/0000-0001-8817-2031Carl-Anton Karlsson2Jonas Berghel3https://orcid.org/0000-0002-9707-8896Chemical Engineering, Department of Engineering and Chemical Sciences, Karlstad University, 651 88 Karlstad, SwedenChemical Engineering, Department of Engineering and Chemical Sciences, Karlstad University, 651 88 Karlstad, SwedenChemical Engineering, Department of Engineering and Chemical Sciences, Karlstad University, 651 88 Karlstad, SwedenEnvironmental and Energy Systems, Department of Engineering and Chemical Science, Karlstad University, 651 88 Karlstad, SwedenHornification of cellulose-rich materials, particularly wood pulps, occurs when chemical bonds form between cellulose surfaces, along with intermolecular forces created during dewatering and drying, preventing the material from reswelling in water to its original structure. Hornification of pulps results in a reduced ability to form effective fiber networks and therefore weaker paper products. The objective of this work was to investigate the role of hornification in pelletized cellulosic biomass and materials in general to provide more information than can be obtained by measuring standard wet state properties, such as water retention. Pellets were produced from chemical pulps with different degrees of hornification, as indicated by the water retention value (WRV), and their mechanical performance was evaluated. The chemical pulps served as a model material for investigating hornification. Pulps with higher hornification produced pellets with inferior mechanical properties, which has not been shown before by such a test. This effect is attributed to increased fiber stiffness and reduced surface flexibility, which limits fiber-fiber bonding. In addition, high drying temperatures prior to pelletizing, and thus higher hornification, will increase compression energy and friction in the pelletizing process. A novel connection was observed between WRV and mechanical performance, highlighting the impact of hornification on the surface interactions of cellulose-based materials.https://ojs.bioresources.com/index.php/BRJ/article/view/24793hornificationcellulosehydrogen bondsbiomasspelletspellet production
spellingShingle Björn Sjöstrand
Gunnar Henriksson
Carl-Anton Karlsson
Jonas Berghel
Role of Hornification of Cellulose Rich Biomass for Pellet Production
BioResources
hornification
cellulose
hydrogen bonds
biomass
pellets
pellet production
title Role of Hornification of Cellulose Rich Biomass for Pellet Production
title_full Role of Hornification of Cellulose Rich Biomass for Pellet Production
title_fullStr Role of Hornification of Cellulose Rich Biomass for Pellet Production
title_full_unstemmed Role of Hornification of Cellulose Rich Biomass for Pellet Production
title_short Role of Hornification of Cellulose Rich Biomass for Pellet Production
title_sort role of hornification of cellulose rich biomass for pellet production
topic hornification
cellulose
hydrogen bonds
biomass
pellets
pellet production
url https://ojs.bioresources.com/index.php/BRJ/article/view/24793
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AT gunnarhenriksson roleofhornificationofcelluloserichbiomassforpelletproduction
AT carlantonkarlsson roleofhornificationofcelluloserichbiomassforpelletproduction
AT jonasberghel roleofhornificationofcelluloserichbiomassforpelletproduction