Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-Substituted

A series of new 1,4-naphtho- and benzoquinone derivatives possessing N-, S-, O-substituted groups which has not been reported yet has been synthesized from 2,3-dichloro-1,4-naphthoquinone 1 and 2,3,5,6-tetrachlorocyclohexa-2,5-diene-1,4-dione 15 involving a Michael addition. In the synthesized compo...

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Main Authors: Semih Kurban, Nahide Gulsah Deniz, Cigdem Sayil, Mustafa Ozyurek, Kubilay Guclu, Maryna Stasevych, Viktor Zvarych, Olena Komarovska-Porokhnyavet, Volodymyr Novikov
Format: Article
Language:English
Published: Wiley 2019-01-01
Series:Heteroatom Chemistry
Online Access:http://dx.doi.org/10.1155/2019/1658417
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author Semih Kurban
Nahide Gulsah Deniz
Cigdem Sayil
Mustafa Ozyurek
Kubilay Guclu
Maryna Stasevych
Viktor Zvarych
Olena Komarovska-Porokhnyavet
Volodymyr Novikov
author_facet Semih Kurban
Nahide Gulsah Deniz
Cigdem Sayil
Mustafa Ozyurek
Kubilay Guclu
Maryna Stasevych
Viktor Zvarych
Olena Komarovska-Porokhnyavet
Volodymyr Novikov
author_sort Semih Kurban
collection DOAJ
description A series of new 1,4-naphtho- and benzoquinone derivatives possessing N-, S-, O-substituted groups which has not been reported yet has been synthesized from 2,3-dichloro-1,4-naphthoquinone 1 and 2,3,5,6-tetrachlorocyclohexa-2,5-diene-1,4-dione 15 involving a Michael addition. In the synthesized compounds, antimicrobial activity at low concentrations against Escherichia coli B-906, Staphylococcus aureus 209-P, and Mycobacterium luteum B-917 bacteria and Candida tenuis VKM Y-70 and Aspergillus niger F-1119 fungi in comparison with controls was identified. 2-Chloro-3-((2-(piperidin-1-yl)ethyl)amino)naphthalene-1,4-dione 3g and 2,5-dichloro-3-ethoxy-6-((2,4,6-trifluorophenyl)amino)cyclohexa-2,5-diene-1,4-dione 17 were the most potent, with a minimum inhibitory concentration value of 15.6 μg/mL against test-culture M. luteum and S. aureus, respectively. Furthermore, in this work, a catalase activity of benzo- and naphthoquinone derivatives was examined for the first time. The catalase activity of benzo- and naphthoquinone derivatives was determined, showing that compound 3g had significant inhibition activity for catalase enzyme.
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spelling doaj-art-d02e5e9e329f4595a8517d746d8be8482025-08-20T02:20:03ZengWileyHeteroatom Chemistry1042-71631098-10712019-01-01201910.1155/2019/16584171658417Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-SubstitutedSemih Kurban0Nahide Gulsah Deniz1Cigdem Sayil2Mustafa Ozyurek3Kubilay Guclu4Maryna Stasevych5Viktor Zvarych6Olena Komarovska-Porokhnyavet7Volodymyr Novikov8Division of Organic Chemistry, Department of Chemistry, Engineering Faculty, Istanbul University-Cerrahpasa, Istanbul, TurkeyDivision of Organic Chemistry, Department of Chemistry, Engineering Faculty, Istanbul University-Cerrahpasa, Istanbul, TurkeyDivision of Organic Chemistry, Department of Chemistry, Engineering Faculty, Istanbul University-Cerrahpasa, Istanbul, TurkeyDivision of Analytical Chemistry, Department of Chemistry, Engineering Faculty, Istanbul University-Cerrahpasa, Istanbul, TurkeyFaculty of Arts and Sciences, Department of Chemistry, Aydın Adnan Menderes University, Aydın, TurkeyDepartment of Technology of Biologically Active Substances, Pharmacy and Biotechnology, Lviv Polytechnic National University, Lviv, UkraineDepartment of Technology of Biologically Active Substances, Pharmacy and Biotechnology, Lviv Polytechnic National University, Lviv, UkraineDepartment of Technology of Biologically Active Substances, Pharmacy and Biotechnology, Lviv Polytechnic National University, Lviv, UkraineDepartment of Technology of Biologically Active Substances, Pharmacy and Biotechnology, Lviv Polytechnic National University, Lviv, UkraineA series of new 1,4-naphtho- and benzoquinone derivatives possessing N-, S-, O-substituted groups which has not been reported yet has been synthesized from 2,3-dichloro-1,4-naphthoquinone 1 and 2,3,5,6-tetrachlorocyclohexa-2,5-diene-1,4-dione 15 involving a Michael addition. In the synthesized compounds, antimicrobial activity at low concentrations against Escherichia coli B-906, Staphylococcus aureus 209-P, and Mycobacterium luteum B-917 bacteria and Candida tenuis VKM Y-70 and Aspergillus niger F-1119 fungi in comparison with controls was identified. 2-Chloro-3-((2-(piperidin-1-yl)ethyl)amino)naphthalene-1,4-dione 3g and 2,5-dichloro-3-ethoxy-6-((2,4,6-trifluorophenyl)amino)cyclohexa-2,5-diene-1,4-dione 17 were the most potent, with a minimum inhibitory concentration value of 15.6 μg/mL against test-culture M. luteum and S. aureus, respectively. Furthermore, in this work, a catalase activity of benzo- and naphthoquinone derivatives was examined for the first time. The catalase activity of benzo- and naphthoquinone derivatives was determined, showing that compound 3g had significant inhibition activity for catalase enzyme.http://dx.doi.org/10.1155/2019/1658417
spellingShingle Semih Kurban
Nahide Gulsah Deniz
Cigdem Sayil
Mustafa Ozyurek
Kubilay Guclu
Maryna Stasevych
Viktor Zvarych
Olena Komarovska-Porokhnyavet
Volodymyr Novikov
Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-Substituted
Heteroatom Chemistry
title Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-Substituted
title_full Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-Substituted
title_fullStr Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-Substituted
title_full_unstemmed Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-Substituted
title_short Synthesis, Antimicrobial Properties, and Inhibition of Catalase Activity of 1,4-Naphtho- and Benzoquinone Derivatives Containing N-, S-, O-Substituted
title_sort synthesis antimicrobial properties and inhibition of catalase activity of 1 4 naphtho and benzoquinone derivatives containing n s o substituted
url http://dx.doi.org/10.1155/2019/1658417
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