Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism study

Magnetic tunnel junctions (MTJs), consisting of two ferromagnetic electrodes separated by an insulating layer, have been foundational in spintronics. This study expands the traditional MTJ framework by incorporating an antiferromagnetic electrode alongside a ferromagnetic one to elucidate the interp...

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Main Authors: Ritika Charak, Sanjeev Gautam, Shaffy Garg, Pardeep K. Thakur, Navdeep Goyal, Younghak Kim, Keun Hwa Chae
Format: Article
Language:English
Published: AIP Publishing LLC 2025-03-01
Series:AIP Advances
Online Access:http://dx.doi.org/10.1063/9.0000908
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author Ritika Charak
Sanjeev Gautam
Shaffy Garg
Pardeep K. Thakur
Navdeep Goyal
Younghak Kim
Keun Hwa Chae
author_facet Ritika Charak
Sanjeev Gautam
Shaffy Garg
Pardeep K. Thakur
Navdeep Goyal
Younghak Kim
Keun Hwa Chae
author_sort Ritika Charak
collection DOAJ
description Magnetic tunnel junctions (MTJs), consisting of two ferromagnetic electrodes separated by an insulating layer, have been foundational in spintronics. This study expands the traditional MTJ framework by incorporating an antiferromagnetic electrode alongside a ferromagnetic one to elucidate the interplay between perpendicular magnetic anisotropy (PMA) and tunnel magnetoresistance (TMR). Specifically, we investigate the relationship among spin-orbital magnetic moments, PMA, and TMR in pristine and Ag-irradiated (200 MeV) thin films of CoFe2O4 (40 nm)/MgO (20 nm)/ZnFe2O4 (40 nm). Angle-dependent soft X-ray magnetic circular dichroism (XMCD), together with element-specific hysteresis loops at the Fe L-edge, reveals that both the pristine and swift heavy ion (SHI)-multilayer stacks display magnetic anisotropy, characterized by a decreased XMCD intensity from out-of-plane (perpendicular) to in-plane (parallel) geometry. This reduction in the XMCD intensity correlates with spin polarization, establishing a direct relationship with the TMR of the MTJ. Furthermore, the analysis confirms that TMR decreases as the measurement angle decreases. Therefore, this investigation underscores the pivotal role of spin-orbital magnetic moments in influencing the PMA and TMR properties of CoFe2O4/MgO/ZnFe2O4 MTJs.
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spelling doaj-art-d0111c07b1fd475ca5d26c543fdd2d6f2025-08-20T03:06:18ZengAIP Publishing LLCAIP Advances2158-32262025-03-01153035314035314-610.1063/9.0000908Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism studyRitika Charak0Sanjeev Gautam1Shaffy Garg2Pardeep K. Thakur3Navdeep Goyal4Younghak Kim5Keun Hwa Chae6Energy Research Centre, Panjab University, Chandigarh 160014, IndiaAdvanced Functional Materials Lab., Dr. S. S. Bhatnagar University Institute of Chemical Engineering and Technology, Panjab University, Chandigarh 160014, IndiaDepartment of Physics, Panjab University Chandigarh, Chandigarh 160014, IndiaBeamline Division, Diamond Light Source Ltd., Oxfordshire, United KingdomDepartment of Physics, Panjab University Chandigarh, Chandigarh 160014, IndiaPohang Accelerator Laboratory, Pohang University of Science and Technology, Pohang 37673, Republic of KoreaAdvanced Analysis and Data Center, Korea Institute of Science and Technology, Seoul 02792, Republic of KoreaMagnetic tunnel junctions (MTJs), consisting of two ferromagnetic electrodes separated by an insulating layer, have been foundational in spintronics. This study expands the traditional MTJ framework by incorporating an antiferromagnetic electrode alongside a ferromagnetic one to elucidate the interplay between perpendicular magnetic anisotropy (PMA) and tunnel magnetoresistance (TMR). Specifically, we investigate the relationship among spin-orbital magnetic moments, PMA, and TMR in pristine and Ag-irradiated (200 MeV) thin films of CoFe2O4 (40 nm)/MgO (20 nm)/ZnFe2O4 (40 nm). Angle-dependent soft X-ray magnetic circular dichroism (XMCD), together with element-specific hysteresis loops at the Fe L-edge, reveals that both the pristine and swift heavy ion (SHI)-multilayer stacks display magnetic anisotropy, characterized by a decreased XMCD intensity from out-of-plane (perpendicular) to in-plane (parallel) geometry. This reduction in the XMCD intensity correlates with spin polarization, establishing a direct relationship with the TMR of the MTJ. Furthermore, the analysis confirms that TMR decreases as the measurement angle decreases. Therefore, this investigation underscores the pivotal role of spin-orbital magnetic moments in influencing the PMA and TMR properties of CoFe2O4/MgO/ZnFe2O4 MTJs.http://dx.doi.org/10.1063/9.0000908
spellingShingle Ritika Charak
Sanjeev Gautam
Shaffy Garg
Pardeep K. Thakur
Navdeep Goyal
Younghak Kim
Keun Hwa Chae
Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism study
AIP Advances
title Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism study
title_full Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism study
title_fullStr Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism study
title_full_unstemmed Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism study
title_short Exploring swift heavy ion-induced perpendicular magnetic anisotropy and tunnel magnetoresistance in CoFe2O4/MgO/ZnFe2O4 multilayers: X-ray magnetic circular dichroism study
title_sort exploring swift heavy ion induced perpendicular magnetic anisotropy and tunnel magnetoresistance in cofe2o4 mgo znfe2o4 multilayers x ray magnetic circular dichroism study
url http://dx.doi.org/10.1063/9.0000908
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