Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and Hydroxyapatite

Ultrahigh-molecular-weight polyethylene/high-density polyethylene (UHMWPE/HDPE) blends prepared using polyethylene glycol PEG as the processing aid and hydroxyapatite (HA) as the reinforcing filler were found to be highly processable using conventional melt blending technique. It was demonstrated th...

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Main Authors: Mazatusziha Ahmad, Mat Uzir Wahit, Mohammed Rafiq Abdul Kadir, Khairul Zaman Mohd Dahlan
Format: Article
Language:English
Published: Wiley 2012-01-01
Series:The Scientific World Journal
Online Access:http://dx.doi.org/10.1100/2012/474851
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author Mazatusziha Ahmad
Mat Uzir Wahit
Mohammed Rafiq Abdul Kadir
Khairul Zaman Mohd Dahlan
author_facet Mazatusziha Ahmad
Mat Uzir Wahit
Mohammed Rafiq Abdul Kadir
Khairul Zaman Mohd Dahlan
author_sort Mazatusziha Ahmad
collection DOAJ
description Ultrahigh-molecular-weight polyethylene/high-density polyethylene (UHMWPE/HDPE) blends prepared using polyethylene glycol PEG as the processing aid and hydroxyapatite (HA) as the reinforcing filler were found to be highly processable using conventional melt blending technique. It was demonstrated that PEG reduced the melt viscosity of UHMWPE/HDPE blend significantly, thus improving the extrudability. The mechanical and bioactive properties were improved with incorporation of HA. Inclusion of HA from 10 to 50 phr resulted in a progressive increase in flexural strength and modulus of the composites. The strength increment is due to the improvement on surface contact between the irregular shape of HA and polymer matrix by formation of mechanical interlock. The HA particles were homogenously distributed even at higher percentage showed improvement in wetting ability between the polymer matrix and HA. The inclusion of HA enhanced the bioactivity properties of the composite by the formation of calcium phosphate (Ca-P) precipitates on the composite surface as proven from SEM and XRD analysis.
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publishDate 2012-01-01
publisher Wiley
record_format Article
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spelling doaj-art-d009148111d144aa948b160194d6a2a52025-08-20T03:19:43ZengWileyThe Scientific World Journal1537-744X2012-01-01201210.1100/2012/474851474851Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and HydroxyapatiteMazatusziha Ahmad0Mat Uzir Wahit1Mohammed Rafiq Abdul Kadir2Khairul Zaman Mohd Dahlan3Department of Polymer Engineering, Faculty of Chemical Engineering, Universiti Teknologi Malaysia, Johor, 81310 Skudai, MalaysiaDepartment of Polymer Engineering, Faculty of Chemical Engineering, Universiti Teknologi Malaysia, Johor, 81310 Skudai, MalaysiaDepartment of Biomechanics and Biomedical Materials, Faculty of Biomedical Engineering and Health Science, Universiti Teknologi Malaysia, Johor, 81310 Skudai, MalaysiaDivision of Radiation Processing Technology, Malaysian Nuclear Agency, Selangor, Bangi, 43000 Kajang, MalaysiaUltrahigh-molecular-weight polyethylene/high-density polyethylene (UHMWPE/HDPE) blends prepared using polyethylene glycol PEG as the processing aid and hydroxyapatite (HA) as the reinforcing filler were found to be highly processable using conventional melt blending technique. It was demonstrated that PEG reduced the melt viscosity of UHMWPE/HDPE blend significantly, thus improving the extrudability. The mechanical and bioactive properties were improved with incorporation of HA. Inclusion of HA from 10 to 50 phr resulted in a progressive increase in flexural strength and modulus of the composites. The strength increment is due to the improvement on surface contact between the irregular shape of HA and polymer matrix by formation of mechanical interlock. The HA particles were homogenously distributed even at higher percentage showed improvement in wetting ability between the polymer matrix and HA. The inclusion of HA enhanced the bioactivity properties of the composite by the formation of calcium phosphate (Ca-P) precipitates on the composite surface as proven from SEM and XRD analysis.http://dx.doi.org/10.1100/2012/474851
spellingShingle Mazatusziha Ahmad
Mat Uzir Wahit
Mohammed Rafiq Abdul Kadir
Khairul Zaman Mohd Dahlan
Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and Hydroxyapatite
The Scientific World Journal
title Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and Hydroxyapatite
title_full Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and Hydroxyapatite
title_fullStr Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and Hydroxyapatite
title_full_unstemmed Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and Hydroxyapatite
title_short Mechanical, Rheological, and Bioactivity Properties of Ultra High-Molecular-Weight Polyethylene Bioactive Composites Containing Polyethylene Glycol and Hydroxyapatite
title_sort mechanical rheological and bioactivity properties of ultra high molecular weight polyethylene bioactive composites containing polyethylene glycol and hydroxyapatite
url http://dx.doi.org/10.1100/2012/474851
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