A novel reversible thermo-swelling hydrogel

A novel reversible thermo-swelling gel was prepared from poly(vinyl alcohol)-trimellitate (PVA-T) by crosslinking with ethylene glycol diglycidyl ether (EGDGE). Only in the presence of sulfate anion, this polymer gel showed a significant and reversible swelling behavior with increasing the temperatu...

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Format: Article
Language:English
Published: Budapest University of Technology and Economics 2010-07-01
Series:eXPRESS Polymer Letters
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Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0001502&mi=cd
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description A novel reversible thermo-swelling gel was prepared from poly(vinyl alcohol)-trimellitate (PVA-T) by crosslinking with ethylene glycol diglycidyl ether (EGDGE). Only in the presence of sulfate anion, this polymer gel showed a significant and reversible swelling behavior with increasing the temperature from 5 to 40°C, and vice versa, probably due to the scission and formation of the inter- and/or intramolecular hydrogen-bondings (HBs) between the carboxyls on the side groups. The involvement of inter- and/or intramolecular HBs for the thermo-swelling behavior was also suggested by a significant dependence on HCl concentration of the swelling degree. In addition, the swelling reversibility and reproducibility were confirmed via the temperature jump between 5 and 40°C, well satisfying for a candidate as a thermosensitive material.
format Article
id doaj-art-cef85c4360ca445aa21503bd35fbdf52
institution Kabale University
issn 1788-618X
language English
publishDate 2010-07-01
publisher Budapest University of Technology and Economics
record_format Article
series eXPRESS Polymer Letters
spelling doaj-art-cef85c4360ca445aa21503bd35fbdf522025-08-20T03:57:44ZengBudapest University of Technology and EconomicseXPRESS Polymer Letters1788-618X2010-07-014745045410.3144/expresspolymlett.2010.56A novel reversible thermo-swelling hydrogelA novel reversible thermo-swelling gel was prepared from poly(vinyl alcohol)-trimellitate (PVA-T) by crosslinking with ethylene glycol diglycidyl ether (EGDGE). Only in the presence of sulfate anion, this polymer gel showed a significant and reversible swelling behavior with increasing the temperature from 5 to 40°C, and vice versa, probably due to the scission and formation of the inter- and/or intramolecular hydrogen-bondings (HBs) between the carboxyls on the side groups. The involvement of inter- and/or intramolecular HBs for the thermo-swelling behavior was also suggested by a significant dependence on HCl concentration of the swelling degree. In addition, the swelling reversibility and reproducibility were confirmed via the temperature jump between 5 and 40°C, well satisfying for a candidate as a thermosensitive material.http://www.expresspolymlett.com/letolt.php?file=EPL-0001502&mi=cdPolymer gelsReversible thermo-swellingHofmeister Series
spellingShingle A novel reversible thermo-swelling hydrogel
eXPRESS Polymer Letters
Polymer gels
Reversible thermo-swelling
Hofmeister Series
title A novel reversible thermo-swelling hydrogel
title_full A novel reversible thermo-swelling hydrogel
title_fullStr A novel reversible thermo-swelling hydrogel
title_full_unstemmed A novel reversible thermo-swelling hydrogel
title_short A novel reversible thermo-swelling hydrogel
title_sort novel reversible thermo swelling hydrogel
topic Polymer gels
Reversible thermo-swelling
Hofmeister Series
url http://www.expresspolymlett.com/letolt.php?file=EPL-0001502&mi=cd