Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with Lignosulfonate

3,4-ethylenedioxythiophene (EDOT) was electropolymerized in the presence of sodium lignosulfonate (LS) at constant current density of 0.25 mA cm−2. As a result, a thin composite film consisting of poly(3,4-Ethylenedioxythiophene) and LS (PEDOT/LS) was deposited on the electrode surface. Unlike PEDOT...

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Main Authors: Grzegorz Milczarek, Tomasz Rebis
Format: Article
Language:English
Published: Wiley 2012-01-01
Series:International Journal of Electrochemistry
Online Access:http://dx.doi.org/10.1155/2012/130980
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author Grzegorz Milczarek
Tomasz Rebis
author_facet Grzegorz Milczarek
Tomasz Rebis
author_sort Grzegorz Milczarek
collection DOAJ
description 3,4-ethylenedioxythiophene (EDOT) was electropolymerized in the presence of sodium lignosulfonate (LS) at constant current density of 0.25 mA cm−2. As a result, a thin composite film consisting of poly(3,4-Ethylenedioxythiophene) and LS (PEDOT/LS) was deposited on the electrode surface. Unlike PEDOT, PEDOT/LS shows appreciable redox activity due to LS-derived quinone moieties with diffusion-like charge propagation across the film thickness. The film-modified gold electrodes can be used as voltammetric sensor of uric acid (UA) in the presence of ascorbic acid (AA). Interestingly, the UA response is catalysed by the presence of AA, and for high AA/UA concentration ratios more than 10-fold enhancement of the UA peak currents are apparent.
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series International Journal of Electrochemistry
spelling doaj-art-ced33df2a3154b68bbe4eb089e14903f2025-08-20T03:23:43ZengWileyInternational Journal of Electrochemistry2090-35292090-35372012-01-01201210.1155/2012/130980130980Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with LignosulfonateGrzegorz Milczarek0Tomasz Rebis1Institute of Chemistry and Technical Electrochemistry, Poznan University of Technology, Piotrowo 3, 60-965 Poznan, PolandInstitute of Chemistry and Technical Electrochemistry, Poznan University of Technology, Piotrowo 3, 60-965 Poznan, Poland3,4-ethylenedioxythiophene (EDOT) was electropolymerized in the presence of sodium lignosulfonate (LS) at constant current density of 0.25 mA cm−2. As a result, a thin composite film consisting of poly(3,4-Ethylenedioxythiophene) and LS (PEDOT/LS) was deposited on the electrode surface. Unlike PEDOT, PEDOT/LS shows appreciable redox activity due to LS-derived quinone moieties with diffusion-like charge propagation across the film thickness. The film-modified gold electrodes can be used as voltammetric sensor of uric acid (UA) in the presence of ascorbic acid (AA). Interestingly, the UA response is catalysed by the presence of AA, and for high AA/UA concentration ratios more than 10-fold enhancement of the UA peak currents are apparent.http://dx.doi.org/10.1155/2012/130980
spellingShingle Grzegorz Milczarek
Tomasz Rebis
Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with Lignosulfonate
International Journal of Electrochemistry
title Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with Lignosulfonate
title_full Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with Lignosulfonate
title_fullStr Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with Lignosulfonate
title_full_unstemmed Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with Lignosulfonate
title_short Synthesis and Electroanalytical Performance of a Composite Material Based on Poly(3,4-ethylenedioxythiophene) Doped with Lignosulfonate
title_sort synthesis and electroanalytical performance of a composite material based on poly 3 4 ethylenedioxythiophene doped with lignosulfonate
url http://dx.doi.org/10.1155/2012/130980
work_keys_str_mv AT grzegorzmilczarek synthesisandelectroanalyticalperformanceofacompositematerialbasedonpoly34ethylenedioxythiophenedopedwithlignosulfonate
AT tomaszrebis synthesisandelectroanalyticalperformanceofacompositematerialbasedonpoly34ethylenedioxythiophenedopedwithlignosulfonate