Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.

Depression poses a significant global health challenge, affecting an estimated 300 million people worldwide. While amitriptyline (Ami) remains one of the most effective antidepressants, its numerous side-effects contribute to a high dropout rate among patients. Addressing this issue requires explori...

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Main Authors: Ramón Eduardo Valadez-Lemus, José L Góngora-Alfaro, Juana María Jiménez-Vargas, Javier Alamilla, Néstor Mendoza-Muñoz
Format: Article
Language:English
Published: Public Library of Science (PLoS) 2025-01-01
Series:PLoS ONE
Online Access:https://doi.org/10.1371/journal.pone.0316389
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author Ramón Eduardo Valadez-Lemus
José L Góngora-Alfaro
Juana María Jiménez-Vargas
Javier Alamilla
Néstor Mendoza-Muñoz
author_facet Ramón Eduardo Valadez-Lemus
José L Góngora-Alfaro
Juana María Jiménez-Vargas
Javier Alamilla
Néstor Mendoza-Muñoz
author_sort Ramón Eduardo Valadez-Lemus
collection DOAJ
description Depression poses a significant global health challenge, affecting an estimated 300 million people worldwide. While amitriptyline (Ami) remains one of the most effective antidepressants, its numerous side-effects contribute to a high dropout rate among patients. Addressing this issue requires exploring methods to enhance its bioavailability and reduce dosage. In this study, we describe a technique for producing amitriptyline nanoparticles (Ami-NPs) to improve the drug's efficiency. The effectiveness was assessed by comparing the dose-response curves of Ami-NPs and non-encapsulated Ami in male and female Wistar rats subjected to the forced swimming test (FST). Ami-NPs were fabricated using nanoprecipitation, with a copolymer of poly (methyl vinyl ether/maleic acid) as the encapsulant, and a 3% solution of poloxamer F-127 as surfactant stabilizer. A Box-Behnken design was used to optimize the production of Ami-NPs, resulting in nanoparticles with the following optimal characteristics: a size of 198.6 ±  38.1 nm, a polydispersity index of 0.005 ±  0.03 nm, a zeta potential of -32 ±  6 mV, and encapsulation efficiency of 79.1 ±  7.4%. Ami-NPs showed higher potency and efficacy in reducing immobility during the FST (ED50 =  7.06 mg/kg, Emax =  41.1%), compared to amitriptyline in solution (Ami-S) (ED50 =  11.89 mg/kg, Emax =  33.2%). The Emax of Ami-NPs occurred at 12 mg/kg, while Ami-S peaked at 15.8 mg/kg. In the open field test, only treatment with Ami-NPs (12 mg/kg) and the empty nanoparticles increased immobility. In the elevated plus-maze, treatment with Ami-NPs (12 mg/kg) significantly reduced closed-arm entries (2.1 ±  0.6), compared to control solution (9.5 ±  1.8), control nanoparticles (8 ±  1.0) and Ami-S (11.5 ±  2). In the marble burying test, Ami-NPs (12 mg/kg) significantly reduced buried marbles (2.4 ±  0.4) compared to control nanoparticles (8.7 ±  1.2). These findings suggest that Ami-NPs could be a promising approach to enhance Ami bioavailability, thereby increasing its potency and antidepressant efficacy, while improving anxiolytic-like effects.
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spelling doaj-art-ce511c16274646c89e5be9ea7ea77f422025-08-20T01:50:31ZengPublic Library of Science (PLoS)PLoS ONE1932-62032025-01-01202e031638910.1371/journal.pone.0316389Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.Ramón Eduardo Valadez-LemusJosé L Góngora-AlfaroJuana María Jiménez-VargasJavier AlamillaNéstor Mendoza-MuñozDepression poses a significant global health challenge, affecting an estimated 300 million people worldwide. While amitriptyline (Ami) remains one of the most effective antidepressants, its numerous side-effects contribute to a high dropout rate among patients. Addressing this issue requires exploring methods to enhance its bioavailability and reduce dosage. In this study, we describe a technique for producing amitriptyline nanoparticles (Ami-NPs) to improve the drug's efficiency. The effectiveness was assessed by comparing the dose-response curves of Ami-NPs and non-encapsulated Ami in male and female Wistar rats subjected to the forced swimming test (FST). Ami-NPs were fabricated using nanoprecipitation, with a copolymer of poly (methyl vinyl ether/maleic acid) as the encapsulant, and a 3% solution of poloxamer F-127 as surfactant stabilizer. A Box-Behnken design was used to optimize the production of Ami-NPs, resulting in nanoparticles with the following optimal characteristics: a size of 198.6 ±  38.1 nm, a polydispersity index of 0.005 ±  0.03 nm, a zeta potential of -32 ±  6 mV, and encapsulation efficiency of 79.1 ±  7.4%. Ami-NPs showed higher potency and efficacy in reducing immobility during the FST (ED50 =  7.06 mg/kg, Emax =  41.1%), compared to amitriptyline in solution (Ami-S) (ED50 =  11.89 mg/kg, Emax =  33.2%). The Emax of Ami-NPs occurred at 12 mg/kg, while Ami-S peaked at 15.8 mg/kg. In the open field test, only treatment with Ami-NPs (12 mg/kg) and the empty nanoparticles increased immobility. In the elevated plus-maze, treatment with Ami-NPs (12 mg/kg) significantly reduced closed-arm entries (2.1 ±  0.6), compared to control solution (9.5 ±  1.8), control nanoparticles (8 ±  1.0) and Ami-S (11.5 ±  2). In the marble burying test, Ami-NPs (12 mg/kg) significantly reduced buried marbles (2.4 ±  0.4) compared to control nanoparticles (8.7 ±  1.2). These findings suggest that Ami-NPs could be a promising approach to enhance Ami bioavailability, thereby increasing its potency and antidepressant efficacy, while improving anxiolytic-like effects.https://doi.org/10.1371/journal.pone.0316389
spellingShingle Ramón Eduardo Valadez-Lemus
José L Góngora-Alfaro
Juana María Jiménez-Vargas
Javier Alamilla
Néstor Mendoza-Muñoz
Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.
PLoS ONE
title Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.
title_full Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.
title_fullStr Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.
title_full_unstemmed Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.
title_short Nanoencapsulation of amitriptyline enhances the potency of antidepressant-like effects and exhibits anxiolytic-like effects in Wistar rats.
title_sort nanoencapsulation of amitriptyline enhances the potency of antidepressant like effects and exhibits anxiolytic like effects in wistar rats
url https://doi.org/10.1371/journal.pone.0316389
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