Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in rats

Abstract Schizophrenia is a neuropsychiatric disorder with limited treatment options that have unwanted side effects. Clozapine, an atypical antipsychotic, has been used for resistant schizophrenia. This study investigated the effect of anthocyanin-rich extract from Rubus fruticosus (RFE) loaded int...

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Main Authors: Mina Y. George, Nermeen Farag, Esther T. Menze, Reham S. Elezaby, Nayera A. Salem, Shereen K. Elrahmany, Nahed Adel, Rana M. ElKhatib, Menna Galal, Hams Assem, Radwa Elkhouly, Mariam Alkess Wesa, Noha Hesham, Nouran Hossam, Iriny M. Ayoub
Format: Article
Language:English
Published: Nature Portfolio 2025-05-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-025-00918-2
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author Mina Y. George
Nermeen Farag
Esther T. Menze
Reham S. Elezaby
Nayera A. Salem
Shereen K. Elrahmany
Nahed Adel
Rana M. ElKhatib
Menna Galal
Hams Assem
Radwa Elkhouly
Mariam Alkess Wesa
Noha Hesham
Nouran Hossam
Iriny M. Ayoub
author_facet Mina Y. George
Nermeen Farag
Esther T. Menze
Reham S. Elezaby
Nayera A. Salem
Shereen K. Elrahmany
Nahed Adel
Rana M. ElKhatib
Menna Galal
Hams Assem
Radwa Elkhouly
Mariam Alkess Wesa
Noha Hesham
Nouran Hossam
Iriny M. Ayoub
author_sort Mina Y. George
collection DOAJ
description Abstract Schizophrenia is a neuropsychiatric disorder with limited treatment options that have unwanted side effects. Clozapine, an atypical antipsychotic, has been used for resistant schizophrenia. This study investigated the effect of anthocyanin-rich extract from Rubus fruticosus (RFE) loaded into chitosan nanoparticles against ketamine-induced schizophrenia in rats. The extract’s phenolic and flavonoid content was measured using UPLC-ESI-MS/MS, revealing 9.42 ± 0.5 mg of gallic acid equivalent and 2.54 ± 0.02 mg of quercetin equivalent per g of extract, with 19 identified compounds, predominantly anthocyanin glycosides. Chitosan nanoparticles were prepared with chitosan and sodium tripolyphosphate at a ratio of 3:1 with particle size 194.49 ± 5.69 nm and encapsulation efficiency of 64.6 ± 1.12%. Rats were treated with ketamine to induce schizophrenia-like symptoms, and various groups received different treatments, including control, ketamine, ketamine + clozapine, ketamine + RFE, and a combination of clozapine/RFE. Clozapine and RFE treatments were initiated from day 8 to day 14. RFE treatment ameliorated positive, negative, and cognitive symptoms of schizophrenia while mitigating clozapine-induced side effects such as weight gain, hyperglycemia, hyperlipidemia, agranulocytosis, and liver dysfunction. RFE corrected oxidative stress as evidenced by its effect on catalase activity and reduced glutathione level. Additionally, RFE hindered neuroinflammation induced by ketamine and reduced the levels of Tumor Necrosis Factor-α. RFE also increased BDNF levels. This study demonstrates that RFE-loaded chitosan nanoparticles exhibit potent antipsychotic properties and enhance clozapine’s therapeutic efficacy while minimizing its adverse effects. This could shed light on the integration of the use of natural products and advanced nano-based formulations to manage schizophrenia patients worldwide.
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spelling doaj-art-cdeb49b776954761b2eaa0b47d18a58c2025-08-20T01:51:39ZengNature PortfolioScientific Reports2045-23222025-05-0115112110.1038/s41598-025-00918-2Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in ratsMina Y. George0Nermeen Farag1Esther T. Menze2Reham S. Elezaby3Nayera A. Salem4Shereen K. Elrahmany5Nahed Adel6Rana M. ElKhatib7Menna Galal8Hams Assem9Radwa Elkhouly10Mariam Alkess Wesa11Noha Hesham12Nouran Hossam13Iriny M. Ayoub14Department of Pharmacology & Toxicology, Faculty of Pharmacy, Ain Shams UniversityDepartment of Pharmacognosy, Faculty of Pharmacy, Cairo UniversityDepartment of Pharmacology & Toxicology, Faculty of Pharmacy, Ain Shams UniversityDepartment of Pharmaceutics, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDrug Design Program Graduates, Faculty of Pharmacy, Ain Shams UniversityDepartment of Pharmacognosy, Faculty of Pharmacy, Ain Shams UniversityAbstract Schizophrenia is a neuropsychiatric disorder with limited treatment options that have unwanted side effects. Clozapine, an atypical antipsychotic, has been used for resistant schizophrenia. This study investigated the effect of anthocyanin-rich extract from Rubus fruticosus (RFE) loaded into chitosan nanoparticles against ketamine-induced schizophrenia in rats. The extract’s phenolic and flavonoid content was measured using UPLC-ESI-MS/MS, revealing 9.42 ± 0.5 mg of gallic acid equivalent and 2.54 ± 0.02 mg of quercetin equivalent per g of extract, with 19 identified compounds, predominantly anthocyanin glycosides. Chitosan nanoparticles were prepared with chitosan and sodium tripolyphosphate at a ratio of 3:1 with particle size 194.49 ± 5.69 nm and encapsulation efficiency of 64.6 ± 1.12%. Rats were treated with ketamine to induce schizophrenia-like symptoms, and various groups received different treatments, including control, ketamine, ketamine + clozapine, ketamine + RFE, and a combination of clozapine/RFE. Clozapine and RFE treatments were initiated from day 8 to day 14. RFE treatment ameliorated positive, negative, and cognitive symptoms of schizophrenia while mitigating clozapine-induced side effects such as weight gain, hyperglycemia, hyperlipidemia, agranulocytosis, and liver dysfunction. RFE corrected oxidative stress as evidenced by its effect on catalase activity and reduced glutathione level. Additionally, RFE hindered neuroinflammation induced by ketamine and reduced the levels of Tumor Necrosis Factor-α. RFE also increased BDNF levels. This study demonstrates that RFE-loaded chitosan nanoparticles exhibit potent antipsychotic properties and enhance clozapine’s therapeutic efficacy while minimizing its adverse effects. This could shed light on the integration of the use of natural products and advanced nano-based formulations to manage schizophrenia patients worldwide.https://doi.org/10.1038/s41598-025-00918-2Rubus fruticosusAnthocyaninsUPLC-ESI-MS/MSChitosanSchizophreniaClozapine
spellingShingle Mina Y. George
Nermeen Farag
Esther T. Menze
Reham S. Elezaby
Nayera A. Salem
Shereen K. Elrahmany
Nahed Adel
Rana M. ElKhatib
Menna Galal
Hams Assem
Radwa Elkhouly
Mariam Alkess Wesa
Noha Hesham
Nouran Hossam
Iriny M. Ayoub
Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in rats
Scientific Reports
Rubus fruticosus
Anthocyanins
UPLC-ESI-MS/MS
Chitosan
Schizophrenia
Clozapine
title Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in rats
title_full Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in rats
title_fullStr Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in rats
title_full_unstemmed Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in rats
title_short Intranasal delivery of blackberry-loaded Chitosan nanoparticles for antipsychotic potential in Ketamine-induced schizophrenia in rats
title_sort intranasal delivery of blackberry loaded chitosan nanoparticles for antipsychotic potential in ketamine induced schizophrenia in rats
topic Rubus fruticosus
Anthocyanins
UPLC-ESI-MS/MS
Chitosan
Schizophrenia
Clozapine
url https://doi.org/10.1038/s41598-025-00918-2
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