PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃO

This study investigated the preparation of a thermoplastic starch-based (ATP) biocomposite reinforced with eucalyptus fibers (FE), focusing on how fiber size affects the properties. The natural fibers were chemically processed using alkaline and bleaching treatments of eucalyptus bark. Subsequently,...

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Main Authors: Luisa B. dos Santos, Tonny A. Moreira, Cleocir J. Dalmaschio, Marta A. Machado
Format: Article
Language:English
Published: Sociedade Brasileira de Química 2024-11-01
Series:Química Nova
Online Access:http://www.scielo.br/scielo.php?script=sci_arttext&pid=S0100-40422024001000209&lng=pt&tlng=pt
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author Luisa B. dos Santos
Tonny A. Moreira
Cleocir J. Dalmaschio
Marta A. Machado
author_facet Luisa B. dos Santos
Tonny A. Moreira
Cleocir J. Dalmaschio
Marta A. Machado
author_sort Luisa B. dos Santos
collection DOAJ
description This study investigated the preparation of a thermoplastic starch-based (ATP) biocomposite reinforced with eucalyptus fibers (FE), focusing on how fiber size affects the properties. The natural fibers were chemically processed using alkaline and bleaching treatments of eucalyptus bark. Subsequently, they were characterized by infrared spectroscopy (FTIR) and X-ray diffraction (XRD) to evaluate alterations in fiber composition and crystalline structure. Samples of biocomposites were prepared with a fixed fiber content (20 wt.%) and variations in particle size (dp): ATP/FE600 (600 μm ≤ dp < 1180 μm), ATP/FE250 (250 μm ≤ dp < 600 μm), and ATP/FE75 (75 μm ≤ dp < 250 μm). The samples were characterized by optical and scanning electron microscopy, mechanical tests, moisture absorption, and swelling analysis. Results indicated significant effects of fiber size on the biocomposite properties. Notably, the larger fibers present in ATP/FE600 exhibited superior tensile strength and elastic modulus, while this sample demonstrated reduced moisture absorption and swelling tendencies. Microscopic images revealed enhanced matrix-fiber adhesion in ATP/FE600, highlighting the importance of proper fiber size. The optimization of fiber size emerges as a relevant strategy for improving the mechanical attributes and mitigating moisture/water absorption tendencies in starch-based thermoplastic biocomposites, contributing to sustainable and high-performance materials.
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spelling doaj-art-cd66f337cce947c8bce359b0fae4779d2025-08-20T02:27:32ZengSociedade Brasileira de QuímicaQuímica Nova1678-70642024-11-01471010.21577/0100-4042.20240074PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃOLuisa B. dos Santoshttps://orcid.org/0009-0001-9653-5186Tonny A. Moreirahttps://orcid.org/0009-0007-3482-0735Cleocir J. Dalmaschiohttps://orcid.org/0000-0002-3773-5786Marta A. Machadohttps://orcid.org/0000-0001-8335-3351This study investigated the preparation of a thermoplastic starch-based (ATP) biocomposite reinforced with eucalyptus fibers (FE), focusing on how fiber size affects the properties. The natural fibers were chemically processed using alkaline and bleaching treatments of eucalyptus bark. Subsequently, they were characterized by infrared spectroscopy (FTIR) and X-ray diffraction (XRD) to evaluate alterations in fiber composition and crystalline structure. Samples of biocomposites were prepared with a fixed fiber content (20 wt.%) and variations in particle size (dp): ATP/FE600 (600 μm ≤ dp < 1180 μm), ATP/FE250 (250 μm ≤ dp < 600 μm), and ATP/FE75 (75 μm ≤ dp < 250 μm). The samples were characterized by optical and scanning electron microscopy, mechanical tests, moisture absorption, and swelling analysis. Results indicated significant effects of fiber size on the biocomposite properties. Notably, the larger fibers present in ATP/FE600 exhibited superior tensile strength and elastic modulus, while this sample demonstrated reduced moisture absorption and swelling tendencies. Microscopic images revealed enhanced matrix-fiber adhesion in ATP/FE600, highlighting the importance of proper fiber size. The optimization of fiber size emerges as a relevant strategy for improving the mechanical attributes and mitigating moisture/water absorption tendencies in starch-based thermoplastic biocomposites, contributing to sustainable and high-performance materials.http://www.scielo.br/scielo.php?script=sci_arttext&pid=S0100-40422024001000209&lng=pt&tlng=pt
spellingShingle Luisa B. dos Santos
Tonny A. Moreira
Cleocir J. Dalmaschio
Marta A. Machado
PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃO
Química Nova
title PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃO
title_full PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃO
title_fullStr PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃO
title_full_unstemmed PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃO
title_short PREPARAÇÃO DE BIOCOMPÓSITO À BASE DE AMIDO TERMOPLÁSTICO REFORÇADO COM FIBRAS DE EUCALIPTO: AVALIAÇÃO DO EFEITO DO TAMANHO DAS FIBRAS NAS PROPRIEDADES MECÂNICAS E DE SORÇÃO
title_sort preparacao de biocomposito a base de amido termoplastico reforcado com fibras de eucalipto avaliacao do efeito do tamanho das fibras nas propriedades mecanicas e de sorcao
url http://www.scielo.br/scielo.php?script=sci_arttext&pid=S0100-40422024001000209&lng=pt&tlng=pt
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