Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate

Objectives. To study the patterns of behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate.Methods. The study employed infrared and nuclear magnetic resonance spectroscopy, as well as elemental analysis.Results. The formation of mixtures of tautomeric f...

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Main Authors: L. O. Belova, N. A. Golub, M. V. Pletneva, N. I. Kirilina, A. D. Kirilin
Format: Article
Language:Russian
Published: MIREA - Russian Technological University 2022-11-01
Series:Тонкие химические технологии
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Online Access:https://www.finechem-mirea.ru/jour/article/view/1879
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author L. O. Belova
N. A. Golub
M. V. Pletneva
N. I. Kirilina
A. D. Kirilin
author_facet L. O. Belova
N. A. Golub
M. V. Pletneva
N. I. Kirilina
A. D. Kirilin
author_sort L. O. Belova
collection DOAJ
description Objectives. To study the patterns of behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate.Methods. The study employed infrared and nuclear magnetic resonance spectroscopy, as well as elemental analysis.Results. The formation of mixtures of tautomeric forms of silicon-containing urea—N-(trimethylsilyl) morpholine-4-carboxamide and trimethylsilylmorpholine-4-carboximidoate—was established.Conclusions. It is shown that the composition and structure of the resulting products are determined both by the presence of a morpholine substituent at the nitrogen atom and by the type of isocyanate used. Unlike the trimethylsilyl derivative of morpholine, morpholine itself reacts with trimethylsilyl isocyanate to form a mixture of tautomeric forms.
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publisher MIREA - Russian Technological University
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series Тонкие химические технологии
spelling doaj-art-cc3c327b2e9744dd9ecd13163e6e21e32025-08-20T02:59:43ZrusMIREA - Russian Technological UniversityТонкие химические технологии2410-65932686-75752022-11-0117537738310.32362/2410-6593-2022-17-5-377-3831691Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanateL. O. Belova0N. A. Golub1M. V. Pletneva2N. I. Kirilina3A. D. Kirilin4MIREA – Russian Technological University (M.V. Lomonosov Institute of Fine Chemical Technologies)MIREA – Russian Technological University (M.V. Lomonosov Institute of Fine Chemical Technologies)MIREA – Russian Technological University (M.V. Lomonosov Institute of Fine Chemical Technologies)State Research Institute of Chemistry and Technology of Organoelement CompoundsMIREA – Russian Technological University (M.V. Lomonosov Institute of Fine Chemical Technologies)Objectives. To study the patterns of behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate.Methods. The study employed infrared and nuclear magnetic resonance spectroscopy, as well as elemental analysis.Results. The formation of mixtures of tautomeric forms of silicon-containing urea—N-(trimethylsilyl) morpholine-4-carboxamide and trimethylsilylmorpholine-4-carboximidoate—was established.Conclusions. It is shown that the composition and structure of the resulting products are determined both by the presence of a morpholine substituent at the nitrogen atom and by the type of isocyanate used. Unlike the trimethylsilyl derivative of morpholine, morpholine itself reacts with trimethylsilyl isocyanate to form a mixture of tautomeric forms.https://www.finechem-mirea.ru/jour/article/view/1879morpholinetrimethylsilyl isocyanatesilicon-containing ureastautomerismamideisoamide tautomerismn-(trimethylsilyl)morpholine-4-carboxamidetrimethylsilylmorpholine-4-carboxyimidoate
spellingShingle L. O. Belova
N. A. Golub
M. V. Pletneva
N. I. Kirilina
A. D. Kirilin
Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate
Тонкие химические технологии
morpholine
trimethylsilyl isocyanate
silicon-containing ureas
tautomerism
amideisoamide tautomerism
n-(trimethylsilyl)morpholine-4-carboxamide
trimethylsilylmorpholine-4-carboxyimidoate
title Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate
title_full Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate
title_fullStr Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate
title_full_unstemmed Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate
title_short Behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate
title_sort behavior of morpholine and its trimethylsilyl derivative in reactions with trimethylsilyl isocyanate
topic morpholine
trimethylsilyl isocyanate
silicon-containing ureas
tautomerism
amideisoamide tautomerism
n-(trimethylsilyl)morpholine-4-carboxamide
trimethylsilylmorpholine-4-carboxyimidoate
url https://www.finechem-mirea.ru/jour/article/view/1879
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