Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displays

Thanks to their tunable luminescence, narrow emission range, and superior color fidelity, perovskite quantum dots (PeQDs) are widely considered as promising materials for next-generation backlight displays. However, the susceptibility to degradation and failure when exposed to ambient environment si...

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Main Authors: Jie Gao, Yu Ren, Qi Ding, Peng Yan, Yongping Liu, Yunfeng Hu, Jihu Chen, Zhi Cheng, Yuchi Fan, Wan Jiang
Format: Article
Language:English
Published: Elsevier 2025-07-01
Series:Journal of Materiomics
Online Access:http://www.sciencedirect.com/science/article/pii/S2352847824001722
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author Jie Gao
Yu Ren
Qi Ding
Peng Yan
Yongping Liu
Yunfeng Hu
Jihu Chen
Zhi Cheng
Yuchi Fan
Wan Jiang
author_facet Jie Gao
Yu Ren
Qi Ding
Peng Yan
Yongping Liu
Yunfeng Hu
Jihu Chen
Zhi Cheng
Yuchi Fan
Wan Jiang
author_sort Jie Gao
collection DOAJ
description Thanks to their tunable luminescence, narrow emission range, and superior color fidelity, perovskite quantum dots (PeQDs) are widely considered as promising materials for next-generation backlight displays. However, the susceptibility to degradation and failure when exposed to ambient environment significantly hampers their widespread applications. Herein, we reported an effective strategy to encapsulate CsPbBr3 nanocrystals into robust KBr matrix via cold sintering process at 120 °C. The well prepared translucent CsPbBr3@KBr ceramic displays a narrow green photoluminescence (with a full-width at half-maximum of ∼22 nm) and an quantum yield of 73.6% with remarkable thermal stability. By incorporating red emitting K2SiF4:Mn4+ phosphor into the KBr matrix, the color gamut of the constructed white LED improves to 118% of the National Television System Committee (NTSC) standard, suggesting that the thermally robust and narrow-band green emitter holds significant promise for wide-color-gamut liquid crystal displays.
format Article
id doaj-art-cbb0e1a040ff48a3b3d2fb979ffee910
institution DOAJ
issn 2352-8478
language English
publishDate 2025-07-01
publisher Elsevier
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series Journal of Materiomics
spelling doaj-art-cbb0e1a040ff48a3b3d2fb979ffee9102025-08-20T02:54:22ZengElsevierJournal of Materiomics2352-84782025-07-0111410093310.1016/j.jmat.2024.100933Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displaysJie Gao0Yu Ren1Qi Ding2Peng Yan3Yongping Liu4Yunfeng Hu5Jihu Chen6Zhi Cheng7Yuchi Fan8Wan Jiang9State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaCorresponding author.; State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Institute of Functional Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, ChinaThanks to their tunable luminescence, narrow emission range, and superior color fidelity, perovskite quantum dots (PeQDs) are widely considered as promising materials for next-generation backlight displays. However, the susceptibility to degradation and failure when exposed to ambient environment significantly hampers their widespread applications. Herein, we reported an effective strategy to encapsulate CsPbBr3 nanocrystals into robust KBr matrix via cold sintering process at 120 °C. The well prepared translucent CsPbBr3@KBr ceramic displays a narrow green photoluminescence (with a full-width at half-maximum of ∼22 nm) and an quantum yield of 73.6% with remarkable thermal stability. By incorporating red emitting K2SiF4:Mn4+ phosphor into the KBr matrix, the color gamut of the constructed white LED improves to 118% of the National Television System Committee (NTSC) standard, suggesting that the thermally robust and narrow-band green emitter holds significant promise for wide-color-gamut liquid crystal displays.http://www.sciencedirect.com/science/article/pii/S2352847824001722
spellingShingle Jie Gao
Yu Ren
Qi Ding
Peng Yan
Yongping Liu
Yunfeng Hu
Jihu Chen
Zhi Cheng
Yuchi Fan
Wan Jiang
Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displays
Journal of Materiomics
title Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displays
title_full Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displays
title_fullStr Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displays
title_full_unstemmed Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displays
title_short Cold sintering of CsPbBr3 quantum dots embedded KBr ceramics for LED displays
title_sort cold sintering of cspbbr3 quantum dots embedded kbr ceramics for led displays
url http://www.sciencedirect.com/science/article/pii/S2352847824001722
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