Dehydration of Natural Gas Using Synthesized Chabazite Zeolite Membranes

ine"> Chabazite zeolite membranes were synthesized for their potential application in dehydration of natural gas. The membranes were prepared using secondary growth method on porous ·-alumina substrates. Hydrothermal treatment was applied for the synthesis of chabazite seeds. The membranes w...

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Bibliographic Details
Main Authors: S. Shirazian, S. N. Ashrafizadeh
Format: Article
Language:English
Published: Iranian Association of Chemical Engineering (IAChE) 2015-01-01
Series:Iranian Journal of Chemical Engineering
Subjects:
Online Access:https://www.ijche.com/article_11223_5a8e90d9a66d583c719471c768e3edaa.pdf
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Summary:ine"> Chabazite zeolite membranes were synthesized for their potential application in dehydration of natural gas. The membranes were prepared using secondary growth method on porous ·-alumina substrates. Hydrothermal treatment was applied for the synthesis of chabazite seeds. The membranes were synthesized at four temperatures of 100, 120, 140, and 160°C; and duration of 20 h. Separation performance of assynthesized membranes was evaluated through permeation ofwater vapor and methane as single gas. Moreover, the structure and morphology ofas-synthesized chabazite zeolite membranes as well as seeds were characterized using scanning electron microscopy (SEM), X-ray diffraction (XRD), and dynamic light scattering (DLS). The results revealed that the optimum temperature for the synthesis ofchabazite membranes is 140°C while at lower and higher temperatures, lower separation performances were observed. At the optimum synthesis temperature, an ideal selectivity of 23 was obtained for water vapor/methane, while a thin and integrated chabazite zeolite layer of about 5 m in thickness was synthesized over the surface ofalumina substrate.
ISSN:1735-5397
2008-2355