Skeletal isomerization of heptanes over superacid catalysts of different nature

The sequence of the formation of multi-branched heptane isomers was studied in liquid and gaseous phases over different liquid and solid superacid catalysts. It was found that this sequence does not depend on the phase state, catalyst nature, and conditions, evidencing in favor of common reaction me...

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Main Authors: A. S. Berenblum, E. A. Katsman, V. Ya. Danyushevskiy, B. P. Krymov
Format: Article
Language:Russian
Published: MIREA - Russian Technological University 2011-06-01
Series:Тонкие химические технологии
Subjects:
Online Access:https://www.finechem-mirea.ru/jour/article/view/836
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author A. S. Berenblum
E. A. Katsman
V. Ya. Danyushevskiy
B. P. Krymov
author_facet A. S. Berenblum
E. A. Katsman
V. Ya. Danyushevskiy
B. P. Krymov
author_sort A. S. Berenblum
collection DOAJ
description The sequence of the formation of multi-branched heptane isomers was studied in liquid and gaseous phases over different liquid and solid superacid catalysts. It was found that this sequence does not depend on the phase state, catalyst nature, and conditions, evidencing in favor of common reaction mechanism. The 2,4-dimethylpentane transformation into 2,2-dimethylpentane can be explained by the intermediate formation of cyclobutyl carbocation.
format Article
id doaj-art-ca0ee993bd434234bd2c86fb4d2c7919
institution Kabale University
issn 2410-6593
2686-7575
language Russian
publishDate 2011-06-01
publisher MIREA - Russian Technological University
record_format Article
series Тонкие химические технологии
spelling doaj-art-ca0ee993bd434234bd2c86fb4d2c79192025-08-20T03:56:24ZrusMIREA - Russian Technological UniversityТонкие химические технологии2410-65932686-75752011-06-01634043830Skeletal isomerization of heptanes over superacid catalysts of different natureA. S. Berenblum0E. A. Katsman1V. Ya. Danyushevskiy2B. P. Krymov3МИТХТ им. М.В. Ломоносова, 119571, Москва, пр-т Вернадского, д. 86МИТХТ им. М.В. Ломоносова, 119571, Москва, пр-т Вернадского, д. 86ООО «ВНИИОС-Наука»ООО «ВНИИОС-Наука»The sequence of the formation of multi-branched heptane isomers was studied in liquid and gaseous phases over different liquid and solid superacid catalysts. It was found that this sequence does not depend on the phase state, catalyst nature, and conditions, evidencing in favor of common reaction mechanism. The 2,4-dimethylpentane transformation into 2,2-dimethylpentane can be explained by the intermediate formation of cyclobutyl carbocation.https://www.finechem-mirea.ru/jour/article/view/836paraffinisomerizationreaction mechanismcatalysissuperacids
spellingShingle A. S. Berenblum
E. A. Katsman
V. Ya. Danyushevskiy
B. P. Krymov
Skeletal isomerization of heptanes over superacid catalysts of different nature
Тонкие химические технологии
paraffin
isomerization
reaction mechanism
catalysis
superacids
title Skeletal isomerization of heptanes over superacid catalysts of different nature
title_full Skeletal isomerization of heptanes over superacid catalysts of different nature
title_fullStr Skeletal isomerization of heptanes over superacid catalysts of different nature
title_full_unstemmed Skeletal isomerization of heptanes over superacid catalysts of different nature
title_short Skeletal isomerization of heptanes over superacid catalysts of different nature
title_sort skeletal isomerization of heptanes over superacid catalysts of different nature
topic paraffin
isomerization
reaction mechanism
catalysis
superacids
url https://www.finechem-mirea.ru/jour/article/view/836
work_keys_str_mv AT asberenblum skeletalisomerizationofheptanesoversuperacidcatalystsofdifferentnature
AT eakatsman skeletalisomerizationofheptanesoversuperacidcatalystsofdifferentnature
AT vyadanyushevskiy skeletalisomerizationofheptanesoversuperacidcatalystsofdifferentnature
AT bpkrymov skeletalisomerizationofheptanesoversuperacidcatalystsofdifferentnature