Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorption

Abstract Developing intelligent electromagnetic wave (EMW) absorption materials with real‐time response‐ability is of great significance in complex application environments. Herein, highly compressible Fe@CNFs@Co/C elastic aerogels were assembled through the electrospinning method, achieving EMW abs...

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Main Authors: Hongwei Zhou, Ying Lin, Yongzhen Ma, Luyao Han, Zhixin Cai, Yan Cheng, Qibin Yuan, Wenhuan Huang, Haibo Yang, Renchao Che
Format: Article
Language:English
Published: Wiley 2025-01-01
Series:InfoMat
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Online Access:https://doi.org/10.1002/inf2.12630
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author Hongwei Zhou
Ying Lin
Yongzhen Ma
Luyao Han
Zhixin Cai
Yan Cheng
Qibin Yuan
Wenhuan Huang
Haibo Yang
Renchao Che
author_facet Hongwei Zhou
Ying Lin
Yongzhen Ma
Luyao Han
Zhixin Cai
Yan Cheng
Qibin Yuan
Wenhuan Huang
Haibo Yang
Renchao Che
author_sort Hongwei Zhou
collection DOAJ
description Abstract Developing intelligent electromagnetic wave (EMW) absorption materials with real‐time response‐ability is of great significance in complex application environments. Herein, highly compressible Fe@CNFs@Co/C elastic aerogels were assembled through the electrospinning method, achieving EMW absorption through pressure changes. By varying the pressure, the effective absorption bandwidth (EAB) of Fe@CNFs@Co/C elastic aerogels shows continuous changes from low frequency to high frequency. The EAB of Fe@CNFs@Co/C elastic aerogels is 14.4 GHz (3.36–17.76 GHz), which covers 90% of the range of S/C/X/Ku bands. The theoretical simulation indicates that the external pressure prompts a reduction in the spacing between the fiber layers in the aerogels and facilitates the formation of a 3D conductive network with enhanced attenuation ability of EMW. The uniform distribution of metal particles and appropriate layer spacing can effectively optimize the impedance matching to achieve the best EMW absorption performance. This work state clearly that the hierarchically assembled elastic aerogels composed of metal–organic frameworks (MOFs) derivatives and carbon fibers are ideal dynamic EMW absorption materials for intelligent EMW response.
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institution Kabale University
issn 2567-3165
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publishDate 2025-01-01
publisher Wiley
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spelling doaj-art-c985e3e01c8443b3b00cc9bf7bdfcaea2025-01-17T04:48:29ZengWileyInfoMat2567-31652025-01-0171n/an/a10.1002/inf2.12630Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorptionHongwei Zhou0Ying Lin1Yongzhen Ma2Luyao Han3Zhixin Cai4Yan Cheng5Qibin Yuan6Wenhuan Huang7Haibo Yang8Renchao Che9Shaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Materials Science and Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaShaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Materials Science and Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaShaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Materials Science and Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaShaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Materials Science and Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaShaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Materials Science and Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaShaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Materials Science and Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaSchool of Electronic Information & Artificial Intelligence, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaSchool of Chemistry and Chemical Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaShaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Materials Science and Engineering, Shaanxi University of Science and Technology Xi'an People's Republic of ChinaDepartment of Materials Science and Collaborative Innovation Center of Chemistry for Energy Materials, Laboratory of Advanced Materials Fudan University Shanghai People's Republic of ChinaAbstract Developing intelligent electromagnetic wave (EMW) absorption materials with real‐time response‐ability is of great significance in complex application environments. Herein, highly compressible Fe@CNFs@Co/C elastic aerogels were assembled through the electrospinning method, achieving EMW absorption through pressure changes. By varying the pressure, the effective absorption bandwidth (EAB) of Fe@CNFs@Co/C elastic aerogels shows continuous changes from low frequency to high frequency. The EAB of Fe@CNFs@Co/C elastic aerogels is 14.4 GHz (3.36–17.76 GHz), which covers 90% of the range of S/C/X/Ku bands. The theoretical simulation indicates that the external pressure prompts a reduction in the spacing between the fiber layers in the aerogels and facilitates the formation of a 3D conductive network with enhanced attenuation ability of EMW. The uniform distribution of metal particles and appropriate layer spacing can effectively optimize the impedance matching to achieve the best EMW absorption performance. This work state clearly that the hierarchically assembled elastic aerogels composed of metal–organic frameworks (MOFs) derivatives and carbon fibers are ideal dynamic EMW absorption materials for intelligent EMW response.https://doi.org/10.1002/inf2.12630elastic aerogelselectrospinningheterogeneous interfacehierarchical structureintelligent electromagnetic wave absorption materialsmetal–organic frameworks
spellingShingle Hongwei Zhou
Ying Lin
Yongzhen Ma
Luyao Han
Zhixin Cai
Yan Cheng
Qibin Yuan
Wenhuan Huang
Haibo Yang
Renchao Che
Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorption
InfoMat
elastic aerogels
electrospinning
heterogeneous interface
hierarchical structure
intelligent electromagnetic wave absorption materials
metal–organic frameworks
title Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorption
title_full Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorption
title_fullStr Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorption
title_full_unstemmed Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorption
title_short Hierarchical structure Fe@CNFs@Co/C elastic aerogels with intelligent electromagnetic wave absorption
title_sort hierarchical structure fe cnfs co c elastic aerogels with intelligent electromagnetic wave absorption
topic elastic aerogels
electrospinning
heterogeneous interface
hierarchical structure
intelligent electromagnetic wave absorption materials
metal–organic frameworks
url https://doi.org/10.1002/inf2.12630
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