Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination Temperature

The electrical properties of tin dioxide (SnO2) nanoparticles induced by low calcination temperature were systematically investigated for gas sensing applications. The precipitation method was used to prepare SnO2 powders, while the sol-gel method was adopted to prepare SnO2 thin films at different...

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Main Authors: Panya Khaenamkaew, Dhonluck Manop, Chaileok Tanghengjaroen, Worasit Palakawong Na Ayuthaya
Format: Article
Language:English
Published: Wiley 2020-01-01
Series:Advances in Materials Science and Engineering
Online Access:http://dx.doi.org/10.1155/2020/3852421
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author Panya Khaenamkaew
Dhonluck Manop
Chaileok Tanghengjaroen
Worasit Palakawong Na Ayuthaya
author_facet Panya Khaenamkaew
Dhonluck Manop
Chaileok Tanghengjaroen
Worasit Palakawong Na Ayuthaya
author_sort Panya Khaenamkaew
collection DOAJ
description The electrical properties of tin dioxide (SnO2) nanoparticles induced by low calcination temperature were systematically investigated for gas sensing applications. The precipitation method was used to prepare SnO2 powders, while the sol-gel method was adopted to prepare SnO2 thin films at different calcination temperatures. The characterization was done by X-ray diffraction, scanning electron microscopy (SEM), and atomic force microscopy (AFM). The samples were perfectly matched with the rutile tetragonal structure. The average crystallite sizes of SnO2 powders were 45 ± 2, 50 ± 2, 62 ± 2, and 65 ± 2 nm at calcination temperatures of 300, 350, 400, and 450°C, respectively. SEM images and AFM topographies showed an increase in particle size and roughness with the rise in calcination temperature. The dielectric constant decreased with the increase in the frequency of the applied signals but increased on increasing calcination temperature. By using the UV-Vis spectrum, the direct energy bandgaps of SnO2 thin films were found as 4.85, 4.80, 4.75, and 4.10 eV for 300, 350, 400, and 450°C, respectively. Low calcination temperature as 300°C allows smaller crystallite sizes and lower dielectric constants but increases the surface roughness of SnO2, while lattice strain remains independent. Thus, low calcination temperatures of SnO2 are promising for electronic devices like gas sensors.
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spelling doaj-art-c752edbb124d494d8fe150d5f30a48132025-08-20T03:22:55ZengWileyAdvances in Materials Science and Engineering1687-84341687-84422020-01-01202010.1155/2020/38524213852421Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination TemperaturePanya Khaenamkaew0Dhonluck Manop1Chaileok Tanghengjaroen2Worasit Palakawong Na Ayuthaya3Department of Basic Science and Physical Education, Faculty of Science at Si Racha, Kasetsart University, Sriracha Campus, Chonburi 20230, ThailandDepartment of Basic Science and Physical Education, Faculty of Science at Si Racha, Kasetsart University, Sriracha Campus, Chonburi 20230, ThailandDepartment of Basic Science and Physical Education, Faculty of Science at Si Racha, Kasetsart University, Sriracha Campus, Chonburi 20230, ThailandDepartment of Resources and Environment, Faculty of Science at Si Racha, Kasetsart University, Sriracha Campus, Chonburi 20230, ThailandThe electrical properties of tin dioxide (SnO2) nanoparticles induced by low calcination temperature were systematically investigated for gas sensing applications. The precipitation method was used to prepare SnO2 powders, while the sol-gel method was adopted to prepare SnO2 thin films at different calcination temperatures. The characterization was done by X-ray diffraction, scanning electron microscopy (SEM), and atomic force microscopy (AFM). The samples were perfectly matched with the rutile tetragonal structure. The average crystallite sizes of SnO2 powders were 45 ± 2, 50 ± 2, 62 ± 2, and 65 ± 2 nm at calcination temperatures of 300, 350, 400, and 450°C, respectively. SEM images and AFM topographies showed an increase in particle size and roughness with the rise in calcination temperature. The dielectric constant decreased with the increase in the frequency of the applied signals but increased on increasing calcination temperature. By using the UV-Vis spectrum, the direct energy bandgaps of SnO2 thin films were found as 4.85, 4.80, 4.75, and 4.10 eV for 300, 350, 400, and 450°C, respectively. Low calcination temperature as 300°C allows smaller crystallite sizes and lower dielectric constants but increases the surface roughness of SnO2, while lattice strain remains independent. Thus, low calcination temperatures of SnO2 are promising for electronic devices like gas sensors.http://dx.doi.org/10.1155/2020/3852421
spellingShingle Panya Khaenamkaew
Dhonluck Manop
Chaileok Tanghengjaroen
Worasit Palakawong Na Ayuthaya
Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination Temperature
Advances in Materials Science and Engineering
title Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination Temperature
title_full Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination Temperature
title_fullStr Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination Temperature
title_full_unstemmed Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination Temperature
title_short Crystal Structure, Lattice Strain, Morphology, and Electrical Properties of SnO2 Nanoparticles Induced by Low Calcination Temperature
title_sort crystal structure lattice strain morphology and electrical properties of sno2 nanoparticles induced by low calcination temperature
url http://dx.doi.org/10.1155/2020/3852421
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AT chaileoktanghengjaroen crystalstructurelatticestrainmorphologyandelectricalpropertiesofsno2nanoparticlesinducedbylowcalcinationtemperature
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