Second harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arrays

The solid solution of BaTiO _3 –BiFeO _3 (BTO–BFO) exhibits enhanced magneto-electric coupling compared to the widely explored BiFeO _3 . In this study, we examined BTO–BFO nanorod arrays (and films) ranging from 200 to 600 nm in height (and thickness) by employing second harmonic emission (SHE) and...

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Main Authors: Nicholas W G Smith, Rathsara R H H Mudiyanselage, Shuang Wu, Satoru Emori, Brenden A Magill, Shashank Priya, Giti A Khodaparast
Format: Article
Language:English
Published: IOP Publishing 2025-01-01
Series:JPhys Materials
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Online Access:https://doi.org/10.1088/2515-7639/adeaee
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author Nicholas W G Smith
Rathsara R H H Mudiyanselage
Shuang Wu
Satoru Emori
Brenden A Magill
Shashank Priya
Giti A Khodaparast
author_facet Nicholas W G Smith
Rathsara R H H Mudiyanselage
Shuang Wu
Satoru Emori
Brenden A Magill
Shashank Priya
Giti A Khodaparast
author_sort Nicholas W G Smith
collection DOAJ
description The solid solution of BaTiO _3 –BiFeO _3 (BTO–BFO) exhibits enhanced magneto-electric coupling compared to the widely explored BiFeO _3 . In this study, we examined BTO–BFO nanorod arrays (and films) ranging from 200 to 600 nm in height (and thickness) by employing second harmonic emission (SHE) and ferromagnetic resonance (FMR) measurements. We demonstrated a large enhancement in SHE in nanorod arrays compared to the films, which can be attributed to the high surface-to-volume ratio in the nanorod arrays. Our FMR measurements showed low effective damping parameters of (4–8) $\times{}$ 10 ^−3 in both nanorods and film structures. These observations are promising for future nonlinear optoelectronics and spintronics applications.
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spelling doaj-art-c73558ae54144f00a9d34f42d61151d72025-08-20T02:41:42ZengIOP PublishingJPhys Materials2515-76392025-01-018303500910.1088/2515-7639/adeaeeSecond harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arraysNicholas W G Smith0Rathsara R H H Mudiyanselage1Shuang Wu2Satoru Emori3https://orcid.org/0000-0001-8035-317XBrenden A Magill4https://orcid.org/0000-0001-7378-4713Shashank Priya5https://orcid.org/0000-0003-1367-3434Giti A Khodaparast6https://orcid.org/0000-0002-1597-6538Department of Physics, Virginia Tech , Blacksburg, VA 24061, United States of AmericaDepartment of Physics, Virginia Tech , Blacksburg, VA 24061, United States of AmericaDepartment of Physics, Virginia Tech , Blacksburg, VA 24061, United States of AmericaDepartment of Physics, Virginia Tech , Blacksburg, VA 24061, United States of AmericaDepartment of Physics, Virginia Tech , Blacksburg, VA 24061, United States of AmericaMaterials Research Institute, Penn State , University Park, PA 16802, United States of AmericaDepartment of Physics, Virginia Tech , Blacksburg, VA 24061, United States of AmericaThe solid solution of BaTiO _3 –BiFeO _3 (BTO–BFO) exhibits enhanced magneto-electric coupling compared to the widely explored BiFeO _3 . In this study, we examined BTO–BFO nanorod arrays (and films) ranging from 200 to 600 nm in height (and thickness) by employing second harmonic emission (SHE) and ferromagnetic resonance (FMR) measurements. We demonstrated a large enhancement in SHE in nanorod arrays compared to the films, which can be attributed to the high surface-to-volume ratio in the nanorod arrays. Our FMR measurements showed low effective damping parameters of (4–8) $\times{}$ 10 ^−3 in both nanorods and film structures. These observations are promising for future nonlinear optoelectronics and spintronics applications.https://doi.org/10.1088/2515-7639/adeaeesecond harmonic generationmagneto-electricferromagnetic resonancemultiferroicsspintronicsnonlinear optics
spellingShingle Nicholas W G Smith
Rathsara R H H Mudiyanselage
Shuang Wu
Satoru Emori
Brenden A Magill
Shashank Priya
Giti A Khodaparast
Second harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arrays
JPhys Materials
second harmonic generation
magneto-electric
ferromagnetic resonance
multiferroics
spintronics
nonlinear optics
title Second harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arrays
title_full Second harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arrays
title_fullStr Second harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arrays
title_full_unstemmed Second harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arrays
title_short Second harmonic generation and ferromagnetic resonance of BaTiO3–BiFeO3 films and nanorod arrays
title_sort second harmonic generation and ferromagnetic resonance of batio3 bifeo3 films and nanorod arrays
topic second harmonic generation
magneto-electric
ferromagnetic resonance
multiferroics
spintronics
nonlinear optics
url https://doi.org/10.1088/2515-7639/adeaee
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AT shuangwu secondharmonicgenerationandferromagneticresonanceofbatio3bifeo3filmsandnanorodarrays
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