Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC Syntheses

Diacetates of meso-2-nitro-1,3-diols, readily available from nitroalkanes and aldehydes, are saponified to crystalline monoacetates of > 97% ee by pig liver esterase (PLE). A general discussion of this type of EPC synthesis (EPC: enantiomerically pure compounds) is given, and a specific example...

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Main Authors: Dieter Seebach, Martin Eberle
Format: Article
Language:deu
Published: Swiss Chemical Society 1986-09-01
Series:CHIMIA
Online Access:https://www.chimia.ch/chimia/article/view/9749
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author Dieter Seebach
Martin Eberle
author_facet Dieter Seebach
Martin Eberle
author_sort Dieter Seebach
collection DOAJ
description Diacetates of meso-2-nitro-1,3-diols, readily available from nitroalkanes and aldehydes, are saponified to crystalline monoacetates of > 97% ee by pig liver esterase (PLE). A general discussion of this type of EPC synthesis (EPC: enantiomerically pure compounds) is given, and a specific example is described in detail: a procedure for the preparation of a very inexpensive PLE concentrate and of a PLE solution from fresh liver, and a procedure for preparing 20 g amounts of enantiomerically pure (1S, 2S, 3R)-3-hydroxy-2-nitro-cyclohexyl acetate.
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publishDate 1986-09-01
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spelling doaj-art-c721dd7d813a443d8900de484b2baba92025-08-20T01:47:43ZdeuSwiss Chemical SocietyCHIMIA0009-42932673-24241986-09-0140910.2533/chimia.1986.315Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC SynthesesDieter Seebach0Martin Eberle1Laboratorium für Organische Chemie Eidgenössische Technische Hochschule Zürich ETH-Zentrum, Universitätstrasse 16 CH-8092 ZürichLaboratorium für Organische Chemie Eidgenössische Technische Hochschule Zürich ETH-Zentrum, Universitätstrasse 16 CH-8092 Zürich Diacetates of meso-2-nitro-1,3-diols, readily available from nitroalkanes and aldehydes, are saponified to crystalline monoacetates of > 97% ee by pig liver esterase (PLE). A general discussion of this type of EPC synthesis (EPC: enantiomerically pure compounds) is given, and a specific example is described in detail: a procedure for the preparation of a very inexpensive PLE concentrate and of a PLE solution from fresh liver, and a procedure for preparing 20 g amounts of enantiomerically pure (1S, 2S, 3R)-3-hydroxy-2-nitro-cyclohexyl acetate. https://www.chimia.ch/chimia/article/view/9749
spellingShingle Dieter Seebach
Martin Eberle
Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC Syntheses
CHIMIA
title Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC Syntheses
title_full Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC Syntheses
title_fullStr Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC Syntheses
title_full_unstemmed Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC Syntheses
title_short Enantioselective Cleavage of meso-Nitrodiol Diacetates by an Esterase Concentrate from Fresh Pig Liver: Preparation of Useful Nitroaliphatic Building Blocks for EPC Syntheses
title_sort enantioselective cleavage of meso nitrodiol diacetates by an esterase concentrate from fresh pig liver preparation of useful nitroaliphatic building blocks for epc syntheses
url https://www.chimia.ch/chimia/article/view/9749
work_keys_str_mv AT dieterseebach enantioselectivecleavageofmesonitrodioldiacetatesbyanesteraseconcentratefromfreshpigliverpreparationofusefulnitroaliphaticbuildingblocksforepcsyntheses
AT martineberle enantioselectivecleavageofmesonitrodioldiacetatesbyanesteraseconcentratefromfreshpigliverpreparationofusefulnitroaliphaticbuildingblocksforepcsyntheses