Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion Complexes

Pterostilbene (PTS) has multiple benefits, but poor water solubility and bioavailability limit its application. PTS/β-CD inclusion complexes were synthesized through the phase solubility method to enhance their water solubility. The inclusion complexes were characterized through Fourier transform in...

Full description

Saved in:
Bibliographic Details
Main Authors: Chuan-Chao Wu, Long Qian, Zhen Rong, Yu-Qi Li, Hui-Min Zhang, Rui-Yu He, Guo-Qiang Zhang
Format: Article
Language:English
Published: MDPI AG 2025-03-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/30/6/1363
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849341693127557120
author Chuan-Chao Wu
Long Qian
Zhen Rong
Yu-Qi Li
Hui-Min Zhang
Rui-Yu He
Guo-Qiang Zhang
author_facet Chuan-Chao Wu
Long Qian
Zhen Rong
Yu-Qi Li
Hui-Min Zhang
Rui-Yu He
Guo-Qiang Zhang
author_sort Chuan-Chao Wu
collection DOAJ
description Pterostilbene (PTS) has multiple benefits, but poor water solubility and bioavailability limit its application. PTS/β-CD inclusion complexes were synthesized through the phase solubility method to enhance their water solubility. The inclusion complexes were characterized through Fourier transform infrared spectroscopy, scanning electron microscopy, X-ray diffraction, nuclear magnetic resonance, and molecular docking techniques. The results demonstrated that PTS and β-CD successfully created inclusion complexes with a host–guest ratio of 1:1 and a stability constant of 166.7 M<sup>−1</sup>. To further investigate its prebiotic function, simulated digestion experiments revealed that β-CD exhibited resistance to digestion, allowing it to reach the colon intact. During gastrointestinal digestion, PTS in the PTS/β-CD inclusion complexes was gradually released. Following digestion, the in vitro fermentation of healthy human feces further confirmed the probiotic properties. Compared to the β-CD and fructooligosaccharide (FOS) groups, the PTS/β-CD group significantly increased the production of acetic acid, butyric acid, and lactic acid, respectively. Additionally, beneficial bacteria, such as <i>Bifidobacterium</i> and <i>Lactobacillus</i>, proliferated in the PTS/β-CD group, while the relative abundance of potential pathogenic bacteria, such as <i>Lactococcus</i>, <i>Streptococcus</i>, and <i>Klebsiella</i>, was significantly reduced. Compared to the blank group, propionic acid and butyric acid concentrations in the β-CD group were significantly higher. The abundance of <i>Lactobacillus</i> and other key bacterial species in the β-CD group increased, while the relative abundance of <i>Klebsiella</i> and other pathogens decreased significantly. In conclusion, PTS/β-CD inclusion complexes altered the composition of intestinal flora, promoting the proliferation of beneficial bacteria and inhibiting the growth of harmful bacteria, thereby demonstrating dual probiotic functionality.
format Article
id doaj-art-c3eb7229ee3046939d5289f8d6704baa
institution Kabale University
issn 1420-3049
language English
publishDate 2025-03-01
publisher MDPI AG
record_format Article
series Molecules
spelling doaj-art-c3eb7229ee3046939d5289f8d6704baa2025-08-20T03:43:34ZengMDPI AGMolecules1420-30492025-03-01306136310.3390/molecules30061363Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion ComplexesChuan-Chao Wu0Long Qian1Zhen Rong2Yu-Qi Li3Hui-Min Zhang4Rui-Yu He5Guo-Qiang Zhang6College of Biology and Food Engineering, Anhui Polytechnic University, Wuhu 241000, ChinaCollege of Biology and Food Engineering, Anhui Polytechnic University, Wuhu 241000, ChinaCollege of Biology and Food Engineering, Anhui Polytechnic University, Wuhu 241000, ChinaCollege of Biology and Food Engineering, Anhui Polytechnic University, Wuhu 241000, ChinaCollege of Biology and Food Engineering, Anhui Polytechnic University, Wuhu 241000, ChinaCollege of Biology and Food Engineering, Anhui Polytechnic University, Wuhu 241000, ChinaCollege of Biology and Food Engineering, Anhui Polytechnic University, Wuhu 241000, ChinaPterostilbene (PTS) has multiple benefits, but poor water solubility and bioavailability limit its application. PTS/β-CD inclusion complexes were synthesized through the phase solubility method to enhance their water solubility. The inclusion complexes were characterized through Fourier transform infrared spectroscopy, scanning electron microscopy, X-ray diffraction, nuclear magnetic resonance, and molecular docking techniques. The results demonstrated that PTS and β-CD successfully created inclusion complexes with a host–guest ratio of 1:1 and a stability constant of 166.7 M<sup>−1</sup>. To further investigate its prebiotic function, simulated digestion experiments revealed that β-CD exhibited resistance to digestion, allowing it to reach the colon intact. During gastrointestinal digestion, PTS in the PTS/β-CD inclusion complexes was gradually released. Following digestion, the in vitro fermentation of healthy human feces further confirmed the probiotic properties. Compared to the β-CD and fructooligosaccharide (FOS) groups, the PTS/β-CD group significantly increased the production of acetic acid, butyric acid, and lactic acid, respectively. Additionally, beneficial bacteria, such as <i>Bifidobacterium</i> and <i>Lactobacillus</i>, proliferated in the PTS/β-CD group, while the relative abundance of potential pathogenic bacteria, such as <i>Lactococcus</i>, <i>Streptococcus</i>, and <i>Klebsiella</i>, was significantly reduced. Compared to the blank group, propionic acid and butyric acid concentrations in the β-CD group were significantly higher. The abundance of <i>Lactobacillus</i> and other key bacterial species in the β-CD group increased, while the relative abundance of <i>Klebsiella</i> and other pathogens decreased significantly. In conclusion, PTS/β-CD inclusion complexes altered the composition of intestinal flora, promoting the proliferation of beneficial bacteria and inhibiting the growth of harmful bacteria, thereby demonstrating dual probiotic functionality.https://www.mdpi.com/1420-3049/30/6/1363pterostilbeneβ-cyclodextrininclusion complexesprebioticshort chain fatty acidsgut microbiota
spellingShingle Chuan-Chao Wu
Long Qian
Zhen Rong
Yu-Qi Li
Hui-Min Zhang
Rui-Yu He
Guo-Qiang Zhang
Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion Complexes
Molecules
pterostilbene
β-cyclodextrin
inclusion complexes
prebiotic
short chain fatty acids
gut microbiota
title Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion Complexes
title_full Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion Complexes
title_fullStr Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion Complexes
title_full_unstemmed Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion Complexes
title_short Characterization and In Vitro Prebiotic Activity of Pterostilbene/β-Cyclodextrin Inclusion Complexes
title_sort characterization and in vitro prebiotic activity of pterostilbene β cyclodextrin inclusion complexes
topic pterostilbene
β-cyclodextrin
inclusion complexes
prebiotic
short chain fatty acids
gut microbiota
url https://www.mdpi.com/1420-3049/30/6/1363
work_keys_str_mv AT chuanchaowu characterizationandinvitroprebioticactivityofpterostilbenebcyclodextrininclusioncomplexes
AT longqian characterizationandinvitroprebioticactivityofpterostilbenebcyclodextrininclusioncomplexes
AT zhenrong characterizationandinvitroprebioticactivityofpterostilbenebcyclodextrininclusioncomplexes
AT yuqili characterizationandinvitroprebioticactivityofpterostilbenebcyclodextrininclusioncomplexes
AT huiminzhang characterizationandinvitroprebioticactivityofpterostilbenebcyclodextrininclusioncomplexes
AT ruiyuhe characterizationandinvitroprebioticactivityofpterostilbenebcyclodextrininclusioncomplexes
AT guoqiangzhang characterizationandinvitroprebioticactivityofpterostilbenebcyclodextrininclusioncomplexes