Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxide

Distilled propargyltrichlorosilane with >99% isomeric purity was prepared for the first time, and its asymmetric catalytic regiospecific addition reaction to aldehydes was developed through a systematic catalyst structure–reactivity and selectivity relationship study. The observed catalyst struct...

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Main Authors: Noble Brako, Sreerag Moorkkannur Narayanan, Amber Burns, Layla Auter, Valentino Cesiliano, Rajeev Prabhakar, Norito Takenaka
Format: Article
Language:English
Published: Beilstein-Institut 2024-11-01
Series:Beilstein Journal of Organic Chemistry
Subjects:
Online Access:https://doi.org/10.3762/bjoc.20.255
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author Noble Brako
Sreerag Moorkkannur Narayanan
Amber Burns
Layla Auter
Valentino Cesiliano
Rajeev Prabhakar
Norito Takenaka
author_facet Noble Brako
Sreerag Moorkkannur Narayanan
Amber Burns
Layla Auter
Valentino Cesiliano
Rajeev Prabhakar
Norito Takenaka
author_sort Noble Brako
collection DOAJ
description Distilled propargyltrichlorosilane with >99% isomeric purity was prepared for the first time, and its asymmetric catalytic regiospecific addition reaction to aldehydes was developed through a systematic catalyst structure–reactivity and selectivity relationship study. The observed catalyst structure–enantioselectivity relationship of the present allenylation reaction was found exactly opposite to that of the analogous allylation reaction. The method provided eleven α-allenic alcohols in 22–99% yield with 61:39–92:8 enantiomeric ratios. Furthermore, possible mechanisms of propargyl–allenyl isomerization of propargyltrichlorosilane were computationally investigated.
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issn 1860-5397
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publishDate 2024-11-01
publisher Beilstein-Institut
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series Beilstein Journal of Organic Chemistry
spelling doaj-art-c31569bb2cb64c9b98b4604a81f877c72025-08-20T02:51:15ZengBeilstein-InstitutBeilstein Journal of Organic Chemistry1860-53972024-11-012013069307610.3762/bjoc.20.2551860-5397-20-255Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxideNoble Brako0Sreerag Moorkkannur Narayanan1Amber Burns2Layla Auter3Valentino Cesiliano4Rajeev Prabhakar5Norito Takenaka6Department of Chemistry and Chemical Engineering, Florida Institute of Technology, 150 West University Boulevard, Melbourne, Florida 32901-6975, USA Department of Chemistry, University of Miami, 1301 Memorial Drive, Coral Gables, Florida 33146-0431, USA Department of Chemistry and Chemical Engineering, Florida Institute of Technology, 150 West University Boulevard, Melbourne, Florida 32901-6975, USA Department of Chemistry and Chemical Engineering, Florida Institute of Technology, 150 West University Boulevard, Melbourne, Florida 32901-6975, USA Department of Chemistry, University of Miami, 1301 Memorial Drive, Coral Gables, Florida 33146-0431, USA Department of Chemistry, University of Miami, 1301 Memorial Drive, Coral Gables, Florida 33146-0431, USA Department of Chemistry and Chemical Engineering, Florida Institute of Technology, 150 West University Boulevard, Melbourne, Florida 32901-6975, USA Distilled propargyltrichlorosilane with >99% isomeric purity was prepared for the first time, and its asymmetric catalytic regiospecific addition reaction to aldehydes was developed through a systematic catalyst structure–reactivity and selectivity relationship study. The observed catalyst structure–enantioselectivity relationship of the present allenylation reaction was found exactly opposite to that of the analogous allylation reaction. The method provided eleven α-allenic alcohols in 22–99% yield with 61:39–92:8 enantiomeric ratios. Furthermore, possible mechanisms of propargyl–allenyl isomerization of propargyltrichlorosilane were computationally investigated.https://doi.org/10.3762/bjoc.20.255α-allenic alcoholcomputational chemistrylewis base catalysisorganocatalysispropargyltrichlorosilane
spellingShingle Noble Brako
Sreerag Moorkkannur Narayanan
Amber Burns
Layla Auter
Valentino Cesiliano
Rajeev Prabhakar
Norito Takenaka
Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxide
Beilstein Journal of Organic Chemistry
α-allenic alcohol
computational chemistry
lewis base catalysis
organocatalysis
propargyltrichlorosilane
title Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxide
title_full Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxide
title_fullStr Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxide
title_full_unstemmed Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxide
title_short Enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline N,N’-dioxide
title_sort enantioselective regiospecific addition of propargyltrichlorosilane to aldehydes catalyzed by biisoquinoline n n dioxide
topic α-allenic alcohol
computational chemistry
lewis base catalysis
organocatalysis
propargyltrichlorosilane
url https://doi.org/10.3762/bjoc.20.255
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