Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater

Summary: Freshwater pearl farming in China generates wastewater high in ammoniacal nitrogen (NH₃-N) posing environmental threats. This study explores the use of coal fly ash (CFA), an industrial waste, to synthesize A-type zeolite for effective NH₃-N removal from pearl farming wastewater. The zeolit...

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Main Authors: Bo Xia, Honghao Chen, Juntao Wang, Xiaocheng Pan
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:iScience
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Online Access:http://www.sciencedirect.com/science/article/pii/S2589004224028724
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author Bo Xia
Honghao Chen
Juntao Wang
Xiaocheng Pan
author_facet Bo Xia
Honghao Chen
Juntao Wang
Xiaocheng Pan
author_sort Bo Xia
collection DOAJ
description Summary: Freshwater pearl farming in China generates wastewater high in ammoniacal nitrogen (NH₃-N) posing environmental threats. This study explores the use of coal fly ash (CFA), an industrial waste, to synthesize A-type zeolite for effective NH₃-N removal from pearl farming wastewater. The zeolite was prepared via pickling pretreatment and hydrothermal methods, resulting in a material with favorable adsorption properties, including cubic and spherical microstructures, a specific surface area of 17.5 m2/g, an average pore size of 10.7 nm, and a pore volume of 0.03 cm³/g. Adsorption experiments showed that NH₃-N removal followed pseudo-first-order kinetics and fit the Dubinin-Radushkevich isotherm model. Applied to actual wastewater, the zeolite achieved a 74% removal efficiency at a dosage of 70 g/L. This approach converts CFA into a valuable adsorbent, reducing its environmental impact, and enhances the sustainability of freshwater pearl farming through effective wastewater treatment, and demonstrates the potential of transforming industrial waste into functional materials for environmental remediation.
format Article
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institution Kabale University
issn 2589-0042
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publishDate 2025-01-01
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spelling doaj-art-c2c177bcbd614abfb9a378aa199f081d2025-01-14T04:12:33ZengElsevieriScience2589-00422025-01-01281111645Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewaterBo Xia0Honghao Chen1Juntao Wang2Xiaocheng Pan3Department of Biological Environment, Jiyang College of Zhejiang A&F University, Zhuji, China; Corresponding authorDepartment of Biological Environment, Jiyang College of Zhejiang A&F University, Zhuji, ChinaDepartment of Biological Environment, Jiyang College of Zhejiang A&F University, Zhuji, ChinaDepartment of Biological Environment, Jiyang College of Zhejiang A&F University, Zhuji, China; Corresponding authorSummary: Freshwater pearl farming in China generates wastewater high in ammoniacal nitrogen (NH₃-N) posing environmental threats. This study explores the use of coal fly ash (CFA), an industrial waste, to synthesize A-type zeolite for effective NH₃-N removal from pearl farming wastewater. The zeolite was prepared via pickling pretreatment and hydrothermal methods, resulting in a material with favorable adsorption properties, including cubic and spherical microstructures, a specific surface area of 17.5 m2/g, an average pore size of 10.7 nm, and a pore volume of 0.03 cm³/g. Adsorption experiments showed that NH₃-N removal followed pseudo-first-order kinetics and fit the Dubinin-Radushkevich isotherm model. Applied to actual wastewater, the zeolite achieved a 74% removal efficiency at a dosage of 70 g/L. This approach converts CFA into a valuable adsorbent, reducing its environmental impact, and enhances the sustainability of freshwater pearl farming through effective wastewater treatment, and demonstrates the potential of transforming industrial waste into functional materials for environmental remediation.http://www.sciencedirect.com/science/article/pii/S2589004224028724Environmental chemistryEnvironmental managementAquatic science
spellingShingle Bo Xia
Honghao Chen
Juntao Wang
Xiaocheng Pan
Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater
iScience
Environmental chemistry
Environmental management
Aquatic science
title Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater
title_full Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater
title_fullStr Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater
title_full_unstemmed Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater
title_short Coal fly ash-derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater
title_sort coal fly ash derived zeolite for efficient ammoniacal nitrogen removal from freshwater pearl farming wastewater
topic Environmental chemistry
Environmental management
Aquatic science
url http://www.sciencedirect.com/science/article/pii/S2589004224028724
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AT juntaowang coalflyashderivedzeoliteforefficientammoniacalnitrogenremovalfromfreshwaterpearlfarmingwastewater
AT xiaochengpan coalflyashderivedzeoliteforefficientammoniacalnitrogenremovalfromfreshwaterpearlfarmingwastewater