Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free system

Abstract Construction of a self-regenerating biochemical system is critical for building a synthetic cell. An essential step in building a self-regenerative system is producing a complete set of tRNAs for translation, which remains a significant challenge. Here, we reconstitute a complete set of 21...

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Main Authors: Fanjun Li, Amogh Kumar Baranwal, Sebastian J. Maerkl
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-61671-8
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author Fanjun Li
Amogh Kumar Baranwal
Sebastian J. Maerkl
author_facet Fanjun Li
Amogh Kumar Baranwal
Sebastian J. Maerkl
author_sort Fanjun Li
collection DOAJ
description Abstract Construction of a self-regenerating biochemical system is critical for building a synthetic cell. An essential step in building a self-regenerative system is producing a complete set of tRNAs for translation, which remains a significant challenge. Here, we reconstitute a complete set of 21 in vitro transcribed tRNAs and optimize their abundance to improve protein yield. Next, we show that protein expression in the PURE transcription-translation system can be achieved by in situ transcribing tRNAs from 21 linear tRNA templates or a single plasmid template. To enable synthesis of mature tRNAs from a circular template, we employ either a nicked plasmid template or T. maritima tRNase Z to post-transcriptionally process the precursor tRNAs. We ultimately achieve continuous in situ synthesis of a complete set of tRNAs capable of supporting sustained, steady-state protein expression in PURE reactions running on microfluidic chemostats. Our findings advance the development of an autopoietic biochemical system.
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issn 2041-1723
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spelling doaj-art-c2af97969fa44521ace34b401a672c2f2025-08-20T03:03:38ZengNature PortfolioNature Communications2041-17232025-07-0116111210.1038/s41467-025-61671-8Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free systemFanjun Li0Amogh Kumar Baranwal1Sebastian J. Maerkl2Institute of Bioengineering, School of Engineering, École Polytechnique Fédérale de LausanneInstitute of Bioengineering, School of Engineering, École Polytechnique Fédérale de LausanneInstitute of Bioengineering, School of Engineering, École Polytechnique Fédérale de LausanneAbstract Construction of a self-regenerating biochemical system is critical for building a synthetic cell. An essential step in building a self-regenerative system is producing a complete set of tRNAs for translation, which remains a significant challenge. Here, we reconstitute a complete set of 21 in vitro transcribed tRNAs and optimize their abundance to improve protein yield. Next, we show that protein expression in the PURE transcription-translation system can be achieved by in situ transcribing tRNAs from 21 linear tRNA templates or a single plasmid template. To enable synthesis of mature tRNAs from a circular template, we employ either a nicked plasmid template or T. maritima tRNase Z to post-transcriptionally process the precursor tRNAs. We ultimately achieve continuous in situ synthesis of a complete set of tRNAs capable of supporting sustained, steady-state protein expression in PURE reactions running on microfluidic chemostats. Our findings advance the development of an autopoietic biochemical system.https://doi.org/10.1038/s41467-025-61671-8
spellingShingle Fanjun Li
Amogh Kumar Baranwal
Sebastian J. Maerkl
Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free system
Nature Communications
title Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free system
title_full Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free system
title_fullStr Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free system
title_full_unstemmed Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free system
title_short Continuous in situ synthesis of a complete set of tRNAs sustains steady-state translation in a recombinant cell-free system
title_sort continuous in situ synthesis of a complete set of trnas sustains steady state translation in a recombinant cell free system
url https://doi.org/10.1038/s41467-025-61671-8
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AT sebastianjmaerkl continuousinsitusynthesisofacompletesetoftrnassustainssteadystatetranslationinarecombinantcellfreesystem