Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous Media

On the basis of affinity of Fe(III) ions toward functional groups of 2,6-dihydroxy benzoic acid (2,6-DHB), a charge transfer complex (CT) is formed between Fe(III) ion and 2,6-DHB in acidic media. The stoichiometry and stability constant of the complex was determined using both mole ratio and Job’s...

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Main Authors: Mohammad Saeid Hosseini, Sara Madarshahian
Format: Article
Language:English
Published: Wiley 2009-01-01
Series:E-Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2009/417303
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author Mohammad Saeid Hosseini
Sara Madarshahian
author_facet Mohammad Saeid Hosseini
Sara Madarshahian
author_sort Mohammad Saeid Hosseini
collection DOAJ
description On the basis of affinity of Fe(III) ions toward functional groups of 2,6-dihydroxy benzoic acid (2,6-DHB), a charge transfer complex (CT) is formed between Fe(III) ion and 2,6-DHB in acidic media. The stoichiometry and stability constant of the complex was determined using both mole ratio and Job’s methods. The stability constant of 1:1 complex formed in acidic media is 2.55±0.14×105 (mole ratio) or 2.70±0.12×105 (Job), in which the quantities are in agreement with together. This method was used for spectrophotometric determination of Fe(III) in aqueous media. The dynamic range and detection limit (DL) were 1.2×10-5 to 3.6×10-4 M and 1.5×10-6 M, respectively. The relative standard deviation (RSD) was found to be 0.76% in the replicate treatments (n=7) with 1.6×10-4 M Fe(III). The practical applicability of the method was confirmed using a synthetic certificated reference material (CRM) and spiked natural water samples.
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spelling doaj-art-c270e9b2e97c46d9be016087d882ea862025-08-20T03:23:15ZengWileyE-Journal of Chemistry0973-49452090-98102009-01-016498599210.1155/2009/417303Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous MediaMohammad Saeid Hosseini0Sara Madarshahian1Department of Chemistry, Faculty of Science, Birjand University, Birjand, P.O. Box 414, IranDepartment of Chemistry, Faculty of Science, Birjand University, Birjand, P.O. Box 414, IranOn the basis of affinity of Fe(III) ions toward functional groups of 2,6-dihydroxy benzoic acid (2,6-DHB), a charge transfer complex (CT) is formed between Fe(III) ion and 2,6-DHB in acidic media. The stoichiometry and stability constant of the complex was determined using both mole ratio and Job’s methods. The stability constant of 1:1 complex formed in acidic media is 2.55±0.14×105 (mole ratio) or 2.70±0.12×105 (Job), in which the quantities are in agreement with together. This method was used for spectrophotometric determination of Fe(III) in aqueous media. The dynamic range and detection limit (DL) were 1.2×10-5 to 3.6×10-4 M and 1.5×10-6 M, respectively. The relative standard deviation (RSD) was found to be 0.76% in the replicate treatments (n=7) with 1.6×10-4 M Fe(III). The practical applicability of the method was confirmed using a synthetic certificated reference material (CRM) and spiked natural water samples.http://dx.doi.org/10.1155/2009/417303
spellingShingle Mohammad Saeid Hosseini
Sara Madarshahian
Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous Media
E-Journal of Chemistry
title Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous Media
title_full Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous Media
title_fullStr Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous Media
title_full_unstemmed Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous Media
title_short Investigation of Charge Transfer Complex Formation Between Fe(III) and 2,6-Dihydroxy Benzoic Acid and its Applications for Spectrophotometric Determination of Iron in Aqueous Media
title_sort investigation of charge transfer complex formation between fe iii and 2 6 dihydroxy benzoic acid and its applications for spectrophotometric determination of iron in aqueous media
url http://dx.doi.org/10.1155/2009/417303
work_keys_str_mv AT mohammadsaeidhosseini investigationofchargetransfercomplexformationbetweenfeiiiand26dihydroxybenzoicacidanditsapplicationsforspectrophotometricdeterminationofironinaqueousmedia
AT saramadarshahian investigationofchargetransfercomplexformationbetweenfeiiiand26dihydroxybenzoicacidanditsapplicationsforspectrophotometricdeterminationofironinaqueousmedia