Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packaging

Abstract Growing global concern about plastic packaging waste has led to the development of eco-friendly polymer composites. Each year, hundreds of millions of metric tons of plastic are discarded, highlighting the need for green packaging solutions. In this study, composites based on PLA and TK wer...

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Main Authors: Ektinai Jansri, Narongchai O-Charoen, Pattarawit Rukthong, Khanittha Charoenlarp, Porawan Naksang, Nattaya Vuthiganond, Piyaporn Kampeerapappun
Format: Article
Language:English
Published: Springer 2025-08-01
Series:Discover Sustainability
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Online Access:https://doi.org/10.1007/s43621-025-01719-3
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author Ektinai Jansri
Narongchai O-Charoen
Pattarawit Rukthong
Khanittha Charoenlarp
Porawan Naksang
Nattaya Vuthiganond
Piyaporn Kampeerapappun
author_facet Ektinai Jansri
Narongchai O-Charoen
Pattarawit Rukthong
Khanittha Charoenlarp
Porawan Naksang
Nattaya Vuthiganond
Piyaporn Kampeerapappun
author_sort Ektinai Jansri
collection DOAJ
description Abstract Growing global concern about plastic packaging waste has led to the development of eco-friendly polymer composites. Each year, hundreds of millions of metric tons of plastic are discarded, highlighting the need for green packaging solutions. In this study, composites based on PLA and TK were prepared at different compositions using a twin-screw extruder and hot compression molding. Traditionally used for sun protection and skincare, TK contains bioactive compounds with anti-inflammatory, antioxidant, and antibacterial effects. A higher TK content in the composite led to a reduction in tensile strength (approximately 21.3% at 10% TK content) and impact strength (around 15.1% at 10% TK content) compared to the composite without TK, and also resulted in a rougher surface morphology. DSC data indicated that the addition of TK increased the PLA matrix's degree of crystallinity and glass transition temperature. The color of PLA/TK composites became yellower and darker with increased TK content and demonstrated UV protection properties. Moreover, the antibacterial activity of the TK powder was determined against S. aureus and E. coli (Gram-positive and Gram-negative, respectively). TK powder demonstrated more potent antibacterial activity inhibiting S. aureus than E. coli bacteria. In contrast, antibacterial tests showed no activity in the composite material, including PLA and PLA with TK composites at various concentrations. Despite this, the findings suggest that PLA/TK composites hold promise for packaging applications, offering biodegradability, enhanced tensile modulus, and UV protective properties.
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institution Kabale University
issn 2662-9984
language English
publishDate 2025-08-01
publisher Springer
record_format Article
series Discover Sustainability
spelling doaj-art-bffe8d2bee4a4fe8ae4db09dfba4880a2025-08-20T03:42:45ZengSpringerDiscover Sustainability2662-99842025-08-016112010.1007/s43621-025-01719-3Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packagingEktinai Jansri0Narongchai O-Charoen1Pattarawit Rukthong2Khanittha Charoenlarp3Porawan Naksang4Nattaya Vuthiganond5Piyaporn Kampeerapappun6Division of Polymer Materials Technology, Faculty of Agricultural Product Innovation and Technology, Srinakharinwirot UniversityDepartment of Materials and Metallurgical Engineering, Faculty of Engineering, Rajamangala University of Technology ThanyaburiDepartment of Pharmaceutical Technology, Faculty of Pharmacy, Srinakharinwirot UniversityFaculty of Textile Industries, Rajamangala University of Technology KrungthepDepartment of Food Science and Technology, Faculty of Home Economics Technology, Rajamangala University of Technology KrungthepDivision of Materials and Textile Technology, Faculty of Science and Technology, Thammasat University, Rangsit CenterFaculty of Textile Industries, Rajamangala University of Technology KrungthepAbstract Growing global concern about plastic packaging waste has led to the development of eco-friendly polymer composites. Each year, hundreds of millions of metric tons of plastic are discarded, highlighting the need for green packaging solutions. In this study, composites based on PLA and TK were prepared at different compositions using a twin-screw extruder and hot compression molding. Traditionally used for sun protection and skincare, TK contains bioactive compounds with anti-inflammatory, antioxidant, and antibacterial effects. A higher TK content in the composite led to a reduction in tensile strength (approximately 21.3% at 10% TK content) and impact strength (around 15.1% at 10% TK content) compared to the composite without TK, and also resulted in a rougher surface morphology. DSC data indicated that the addition of TK increased the PLA matrix's degree of crystallinity and glass transition temperature. The color of PLA/TK composites became yellower and darker with increased TK content and demonstrated UV protection properties. Moreover, the antibacterial activity of the TK powder was determined against S. aureus and E. coli (Gram-positive and Gram-negative, respectively). TK powder demonstrated more potent antibacterial activity inhibiting S. aureus than E. coli bacteria. In contrast, antibacterial tests showed no activity in the composite material, including PLA and PLA with TK composites at various concentrations. Despite this, the findings suggest that PLA/TK composites hold promise for packaging applications, offering biodegradability, enhanced tensile modulus, and UV protective properties.https://doi.org/10.1007/s43621-025-01719-3BiocompositePackaging materialSustainabilityThanakaPolylactic acid
spellingShingle Ektinai Jansri
Narongchai O-Charoen
Pattarawit Rukthong
Khanittha Charoenlarp
Porawan Naksang
Nattaya Vuthiganond
Piyaporn Kampeerapappun
Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packaging
Discover Sustainability
Biocomposite
Packaging material
Sustainability
Thanaka
Polylactic acid
title Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packaging
title_full Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packaging
title_fullStr Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packaging
title_full_unstemmed Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packaging
title_short Effect of thanaka powder (TK) content on the structural and functional properties of polylactic acid/TK composites for sustainable packaging
title_sort effect of thanaka powder tk content on the structural and functional properties of polylactic acid tk composites for sustainable packaging
topic Biocomposite
Packaging material
Sustainability
Thanaka
Polylactic acid
url https://doi.org/10.1007/s43621-025-01719-3
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