Carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers

Abstract Cationic polymers have emerged as promising next-generation antimicrobial agents, albeit with inherent limitations such as low potency and limited biocompatibility. Classical cationic polymers kill bacteria via physical membrane disruption. We propose a non-classical mechanism of crossing t...

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Main Authors: Chong Hui Koh, Mallikharjuna Rao Lambu, Chongyun Tan, Guangmin Wei, Zhi Yuan Kok, Kaixi Zhang, Quang Huy Nhat Vu, Muthuvel Panneerselvam, Ying Jie Ooi, Shiow Han Tan, Zheng Wang, Madhu Babu Tatina, Justin Tze Yang Ng, Aoxin Guo, Panyawut Tonanon, Tram T. Dang, Yunn-Hwen Gan, Yuguang Mu, Paula T. Hammond, Yonggui Robin Chi, Richard D. Webster, Sumod A. Pullarkat, Qingjie Li, E. Peter Greenberg, Angelika Gründling, Kevin Pethe, Mary B. Chan-Park
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-61724-y
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author Chong Hui Koh
Mallikharjuna Rao Lambu
Chongyun Tan
Guangmin Wei
Zhi Yuan Kok
Kaixi Zhang
Quang Huy Nhat Vu
Muthuvel Panneerselvam
Ying Jie Ooi
Shiow Han Tan
Zheng Wang
Madhu Babu Tatina
Justin Tze Yang Ng
Aoxin Guo
Panyawut Tonanon
Tram T. Dang
Yunn-Hwen Gan
Yuguang Mu
Paula T. Hammond
Yonggui Robin Chi
Richard D. Webster
Sumod A. Pullarkat
Qingjie Li
E. Peter Greenberg
Angelika Gründling
Kevin Pethe
Mary B. Chan-Park
author_facet Chong Hui Koh
Mallikharjuna Rao Lambu
Chongyun Tan
Guangmin Wei
Zhi Yuan Kok
Kaixi Zhang
Quang Huy Nhat Vu
Muthuvel Panneerselvam
Ying Jie Ooi
Shiow Han Tan
Zheng Wang
Madhu Babu Tatina
Justin Tze Yang Ng
Aoxin Guo
Panyawut Tonanon
Tram T. Dang
Yunn-Hwen Gan
Yuguang Mu
Paula T. Hammond
Yonggui Robin Chi
Richard D. Webster
Sumod A. Pullarkat
Qingjie Li
E. Peter Greenberg
Angelika Gründling
Kevin Pethe
Mary B. Chan-Park
author_sort Chong Hui Koh
collection DOAJ
description Abstract Cationic polymers have emerged as promising next-generation antimicrobial agents, albeit with inherent limitations such as low potency and limited biocompatibility. Classical cationic polymers kill bacteria via physical membrane disruption. We propose a non-classical mechanism of crossing the bacterial plasma membrane barrier, a step required for subsequent inhibition of intracellular targets, by cationic polymers which are carbon acids. Oligoimidazolium (OIM) carbon acids, instead of lysing bacteria, transiently deprotonate in water to form hydrophobic N-heterocyclic carbenes (NHCs) and exhibit efficient plasma membrane translocation. Only OIMs that are carbon acids have potent antibacterial activities against even colistin- and multidrug-resistant bacteria. OIM amide derivatives exhibit excellent antibacterial efficacy in murine sepsis and thigh infection models, while a polymeric version acts as a prophylactic agent against bovine mastitis, which is a global agricultural problem. This study unveils a promising path for the development of an alternative class of potent antimicrobial agents.
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series Nature Communications
spelling doaj-art-bf4fc0c09bdc4183aeffcbfcdabe425e2025-08-20T03:05:10ZengNature PortfolioNature Communications2041-17232025-07-0116111810.1038/s41467-025-61724-yCarbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymersChong Hui Koh0Mallikharjuna Rao Lambu1Chongyun Tan2Guangmin Wei3Zhi Yuan Kok4Kaixi Zhang5Quang Huy Nhat Vu6Muthuvel Panneerselvam7Ying Jie Ooi8Shiow Han Tan9Zheng Wang10Madhu Babu Tatina11Justin Tze Yang Ng12Aoxin Guo13Panyawut Tonanon14Tram T. Dang15Yunn-Hwen Gan16Yuguang Mu17Paula T. Hammond18Yonggui Robin Chi19Richard D. Webster20Sumod A. Pullarkat21Qingjie Li22E. Peter Greenberg23Angelika Gründling24Kevin Pethe25Mary B. Chan-Park26School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Biological Sciences, NTUSchool of Biological Sciences, NTUSchool of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)Infectious Diseases Translational Research Program, Department of Biochemistry, Yong Loo Lin School of Medicine, National University of Singapore (NUS)School of Biological Sciences, NTUSingapore-MIT Alliance for Research and Technology (SMART)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)Research Center of Traditional Chinese Medicine, The Affiliated Hospital to Changchun University of Chinese MedicineDepartment of Microbiology, University of Washington School of MedicineDepartment of Infectious Disease, Section of Molecular Microbiology and Centre for Bacterial Resistance Biology, Imperial College LondonCentre for Antimicrobial Bioengineering, NTUSchool of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University (NTU)Abstract Cationic polymers have emerged as promising next-generation antimicrobial agents, albeit with inherent limitations such as low potency and limited biocompatibility. Classical cationic polymers kill bacteria via physical membrane disruption. We propose a non-classical mechanism of crossing the bacterial plasma membrane barrier, a step required for subsequent inhibition of intracellular targets, by cationic polymers which are carbon acids. Oligoimidazolium (OIM) carbon acids, instead of lysing bacteria, transiently deprotonate in water to form hydrophobic N-heterocyclic carbenes (NHCs) and exhibit efficient plasma membrane translocation. Only OIMs that are carbon acids have potent antibacterial activities against even colistin- and multidrug-resistant bacteria. OIM amide derivatives exhibit excellent antibacterial efficacy in murine sepsis and thigh infection models, while a polymeric version acts as a prophylactic agent against bovine mastitis, which is a global agricultural problem. This study unveils a promising path for the development of an alternative class of potent antimicrobial agents.https://doi.org/10.1038/s41467-025-61724-y
spellingShingle Chong Hui Koh
Mallikharjuna Rao Lambu
Chongyun Tan
Guangmin Wei
Zhi Yuan Kok
Kaixi Zhang
Quang Huy Nhat Vu
Muthuvel Panneerselvam
Ying Jie Ooi
Shiow Han Tan
Zheng Wang
Madhu Babu Tatina
Justin Tze Yang Ng
Aoxin Guo
Panyawut Tonanon
Tram T. Dang
Yunn-Hwen Gan
Yuguang Mu
Paula T. Hammond
Yonggui Robin Chi
Richard D. Webster
Sumod A. Pullarkat
Qingjie Li
E. Peter Greenberg
Angelika Gründling
Kevin Pethe
Mary B. Chan-Park
Carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers
Nature Communications
title Carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers
title_full Carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers
title_fullStr Carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers
title_full_unstemmed Carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers
title_short Carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers
title_sort carbene formation as a mechanism for efficient intracellular uptake of cationic antimicrobial carbon acid polymers
url https://doi.org/10.1038/s41467-025-61724-y
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