Comprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3

The mechanical, electronic and thermodynamic properties of alloy carbide ε -Fe _3 Cr _4 C _3 under varying temperature and pressure were systematically investigated using first-principles calculations and the quasi-harmonic Debye model. ε -Fe _3 Cr _4 C _3 maintains thermodynamic and mechanical stab...

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Main Authors: Zixuan Xie, Tingping Hou, Junwen Duan, Xuan Liang, Yihang Zheng, Tao Yu, Gengping Jiang, Tianliang Zhao
Format: Article
Language:English
Published: IOP Publishing 2025-01-01
Series:Materials Research Express
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Online Access:https://doi.org/10.1088/2053-1591/adee7f
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author Zixuan Xie
Tingping Hou
Junwen Duan
Xuan Liang
Yihang Zheng
Tao Yu
Gengping Jiang
Tianliang Zhao
author_facet Zixuan Xie
Tingping Hou
Junwen Duan
Xuan Liang
Yihang Zheng
Tao Yu
Gengping Jiang
Tianliang Zhao
author_sort Zixuan Xie
collection DOAJ
description The mechanical, electronic and thermodynamic properties of alloy carbide ε -Fe _3 Cr _4 C _3 under varying temperature and pressure were systematically investigated using first-principles calculations and the quasi-harmonic Debye model. ε -Fe _3 Cr _4 C _3 maintains thermodynamic and mechanical stability across the investigated pressure range. Increasing pressure enhances its thermodynamic stability and reduces elastic anisotropy. The electron density distribution indicates stronger metallic bonds under high pressure, providing an explanation for the increased Young’s modulus. Concurrently, the rise in Debye temperature implies enhanced interatomic bonding forces, correlating with improved toughness and hardness. Ultimately, the sample of ε -Fe _3 Cr _4 C _3 was prepared through mechanical alloying and sintering. The experimentally measured hardness is in basic agreement with the theoretical predictions. This work lays essential theoretical foundations for understanding and predicting the properties of ε -Fe _3 Cr _4 C _3 in high pressure and high temperature applications.
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institution Kabale University
issn 2053-1591
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publisher IOP Publishing
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series Materials Research Express
spelling doaj-art-bc883d241d0b4ed897ecfc749b2926702025-08-20T03:30:52ZengIOP PublishingMaterials Research Express2053-15912025-01-0112707651310.1088/2053-1591/adee7fComprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3Zixuan Xie0Tingping Hou1https://orcid.org/0000-0003-3411-5351Junwen Duan2Xuan Liang3Yihang Zheng4Tao Yu5Gengping Jiang6Tianliang Zhao7The State Key Laboratory for Refractories and Metallurgy, Joint International Research Laboratory of Refractories and Metallurgy, Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, International Research Institute for Steel Technology, Collaborative Innovation Center for Advanced Steels, Wuhan University of Science and Technology , Wuhan, 430081, People’s Republic of ChinaThe State Key Laboratory for Refractories and Metallurgy, Joint International Research Laboratory of Refractories and Metallurgy, Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, International Research Institute for Steel Technology, Collaborative Innovation Center for Advanced Steels, Wuhan University of Science and Technology , Wuhan, 430081, People’s Republic of ChinaThe State Key Laboratory for Refractories and Metallurgy, Joint International Research Laboratory of Refractories and Metallurgy, Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, International Research Institute for Steel Technology, Collaborative Innovation Center for Advanced Steels, Wuhan University of Science and Technology , Wuhan, 430081, People’s Republic of ChinaThe State Key Laboratory for Refractories and Metallurgy, Joint International Research Laboratory of Refractories and Metallurgy, Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, International Research Institute for Steel Technology, Collaborative Innovation Center for Advanced Steels, Wuhan University of Science and Technology , Wuhan, 430081, People’s Republic of ChinaThe State Key Laboratory for Refractories and Metallurgy, Joint International Research Laboratory of Refractories and Metallurgy, Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, International Research Institute for Steel Technology, Collaborative Innovation Center for Advanced Steels, Wuhan University of Science and Technology , Wuhan, 430081, People’s Republic of ChinaKey Laboratory of Photochemical Materials and Devices, Ministry of Education, School of Optoelectronic Material and Technology, Jianghan University , Wuhan, 430056, People’s Republic of ChinaThe State Key Laboratory for Refractories and Metallurgy, Joint International Research Laboratory of Refractories and Metallurgy, Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, International Research Institute for Steel Technology, Collaborative Innovation Center for Advanced Steels, Wuhan University of Science and Technology , Wuhan, 430081, People’s Republic of ChinaThe State Key Laboratory for Refractories and Metallurgy, Joint International Research Laboratory of Refractories and Metallurgy, Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, International Research Institute for Steel Technology, Collaborative Innovation Center for Advanced Steels, Wuhan University of Science and Technology , Wuhan, 430081, People’s Republic of ChinaThe mechanical, electronic and thermodynamic properties of alloy carbide ε -Fe _3 Cr _4 C _3 under varying temperature and pressure were systematically investigated using first-principles calculations and the quasi-harmonic Debye model. ε -Fe _3 Cr _4 C _3 maintains thermodynamic and mechanical stability across the investigated pressure range. Increasing pressure enhances its thermodynamic stability and reduces elastic anisotropy. The electron density distribution indicates stronger metallic bonds under high pressure, providing an explanation for the increased Young’s modulus. Concurrently, the rise in Debye temperature implies enhanced interatomic bonding forces, correlating with improved toughness and hardness. Ultimately, the sample of ε -Fe _3 Cr _4 C _3 was prepared through mechanical alloying and sintering. The experimentally measured hardness is in basic agreement with the theoretical predictions. This work lays essential theoretical foundations for understanding and predicting the properties of ε -Fe _3 Cr _4 C _3 in high pressure and high temperature applications.https://doi.org/10.1088/2053-1591/adee7fhigh temperaturehigh pressuremechanical propertiesthermodynamic propertieselectronic propertiesalloy carbide
spellingShingle Zixuan Xie
Tingping Hou
Junwen Duan
Xuan Liang
Yihang Zheng
Tao Yu
Gengping Jiang
Tianliang Zhao
Comprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3
Materials Research Express
high temperature
high pressure
mechanical properties
thermodynamic properties
electronic properties
alloy carbide
title Comprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3
title_full Comprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3
title_fullStr Comprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3
title_full_unstemmed Comprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3
title_short Comprehensive insights into the structural, mechanical, electronic and thermodynamic properties of ε-Fe3Cr4C3
title_sort comprehensive insights into the structural mechanical electronic and thermodynamic properties of ε fe3cr4c3
topic high temperature
high pressure
mechanical properties
thermodynamic properties
electronic properties
alloy carbide
url https://doi.org/10.1088/2053-1591/adee7f
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