Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic Excitation

This study establishes for the first time a P2D-coupled non-ideal double-layer capacitor model (P2D-CNIC), which can be used for mechanism analysis under high-frequency periodic signal excitation. The novelty of this work is the consideration of the generally neglected electric double-layer capacita...

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Main Authors: Zhihao Wang, Xingzhen Zhou, Bingxiang Sun, Weige Zhang, Xiaojia Su, Jinkai Shi, Qinhe Huang
Format: Article
Language:English
Published: American Association for the Advancement of Science (AAAS) 2024-01-01
Series:Space: Science & Technology
Online Access:https://spj.science.org/doi/10.34133/space.0129
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author Zhihao Wang
Xingzhen Zhou
Bingxiang Sun
Weige Zhang
Xiaojia Su
Jinkai Shi
Qinhe Huang
author_facet Zhihao Wang
Xingzhen Zhou
Bingxiang Sun
Weige Zhang
Xiaojia Su
Jinkai Shi
Qinhe Huang
author_sort Zhihao Wang
collection DOAJ
description This study establishes for the first time a P2D-coupled non-ideal double-layer capacitor model (P2D-CNIC), which can be used for mechanism analysis under high-frequency periodic signal excitation. The novelty of this work is the consideration of the generally neglected electric double-layer capacitance and its dispersion effects, especially the capacitance of the solid electrolyte interface (SEI) film. The dispersion effect of the model is verified by a periodic current excitation signal and the corresponding phase change in the voltage response. Under sinusoidal alternating current (AC) excitation, a comparative analysis was conducted between the traditional P2D model, the traditional P2D model coupled with the ideal double-layer capacitor (P2D-CIC), and the proposed P2D-CNIC mechanism model. Furthermore, three models were evaluated under periodic short-circuit pulse discharge conditions to verify the accuracy and reliability of P2D-CNIC. The simulation results are used to analyze the dominant order of faradaic and non-Faraday processes under sinusoidal AC excitation, thereby providing insights into the internal mechanism analysis of lithium batteries under high-frequency cycling conditions.
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issn 2692-7659
language English
publishDate 2024-01-01
publisher American Association for the Advancement of Science (AAAS)
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series Space: Science & Technology
spelling doaj-art-bb259051df5c4971bcf8cdbbfd7bcc232025-08-20T01:55:19ZengAmerican Association for the Advancement of Science (AAAS)Space: Science & Technology2692-76592024-01-01410.34133/space.0129Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic ExcitationZhihao Wang0Xingzhen Zhou1Bingxiang Sun2Weige Zhang3Xiaojia Su4Jinkai Shi5Qinhe Huang6National Active Distribution Network Technology Research Center (NANTEC), Beijing Jiaotong University, Beijing 100044, ChinaNational Active Distribution Network Technology Research Center (NANTEC), Beijing Jiaotong University, Beijing 100044, ChinaNational Active Distribution Network Technology Research Center (NANTEC), Beijing Jiaotong University, Beijing 100044, ChinaNational Active Distribution Network Technology Research Center (NANTEC), Beijing Jiaotong University, Beijing 100044, ChinaNational Active Distribution Network Technology Research Center (NANTEC), Beijing Jiaotong University, Beijing 100044, ChinaNational Active Distribution Network Technology Research Center (NANTEC), Beijing Jiaotong University, Beijing 100044, ChinaNational Active Distribution Network Technology Research Center (NANTEC), Beijing Jiaotong University, Beijing 100044, ChinaThis study establishes for the first time a P2D-coupled non-ideal double-layer capacitor model (P2D-CNIC), which can be used for mechanism analysis under high-frequency periodic signal excitation. The novelty of this work is the consideration of the generally neglected electric double-layer capacitance and its dispersion effects, especially the capacitance of the solid electrolyte interface (SEI) film. The dispersion effect of the model is verified by a periodic current excitation signal and the corresponding phase change in the voltage response. Under sinusoidal alternating current (AC) excitation, a comparative analysis was conducted between the traditional P2D model, the traditional P2D model coupled with the ideal double-layer capacitor (P2D-CIC), and the proposed P2D-CNIC mechanism model. Furthermore, three models were evaluated under periodic short-circuit pulse discharge conditions to verify the accuracy and reliability of P2D-CNIC. The simulation results are used to analyze the dominant order of faradaic and non-Faraday processes under sinusoidal AC excitation, thereby providing insights into the internal mechanism analysis of lithium batteries under high-frequency cycling conditions.https://spj.science.org/doi/10.34133/space.0129
spellingShingle Zhihao Wang
Xingzhen Zhou
Bingxiang Sun
Weige Zhang
Xiaojia Su
Jinkai Shi
Qinhe Huang
Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic Excitation
Space: Science & Technology
title Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic Excitation
title_full Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic Excitation
title_fullStr Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic Excitation
title_full_unstemmed Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic Excitation
title_short Model Construction and Dominant Mechanism Analysis of Li-Ion Batteries under Periodic Excitation
title_sort model construction and dominant mechanism analysis of li ion batteries under periodic excitation
url https://spj.science.org/doi/10.34133/space.0129
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