Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5

Abstract The spin dynamics and electronic orders of the kagome system at different filling levels stand as an intriguing subject in condensed matter physics. By first-principles calculations and random phase approximation analyses, we investigate the spin fluctuations and superconducting instabiliti...

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Main Authors: Siqi Wu, Chenchao Xu, Xiaoqun Wang, Hai-Qing Lin, Chao Cao, Guang-Han Cao
Format: Article
Language:English
Published: Nature Portfolio 2025-02-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-56582-7
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author Siqi Wu
Chenchao Xu
Xiaoqun Wang
Hai-Qing Lin
Chao Cao
Guang-Han Cao
author_facet Siqi Wu
Chenchao Xu
Xiaoqun Wang
Hai-Qing Lin
Chao Cao
Guang-Han Cao
author_sort Siqi Wu
collection DOAJ
description Abstract The spin dynamics and electronic orders of the kagome system at different filling levels stand as an intriguing subject in condensed matter physics. By first-principles calculations and random phase approximation analyses, we investigate the spin fluctuations and superconducting instabilities in kagome phase of CsCr3Sb5 under high pressure. At the filling level slightly below the kagome flat bands, our calculations reveal strong antiferromagnetic spin fluctuations in CsCr3Sb5, together with a leading s ±-wave and a competing (d x y , $${d}_{{x}^{2}-{y}^{2}}$$ d x 2 − y 2 )-wave superconducting order. Unlike the general intuition that the flat bands are closely related to the ferromagnetic correlations, here we propose a sublattice-momentum-coupling-driven mechanism for the antiferromagnetic fluctuations enhanced from the unoccupied flat bands. The mechanism is generally applicable to kagome systems where the Fermi level intersects near the flat bands, offering a new perspective for future studies of geometrically frustrated systems.
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institution Kabale University
issn 2041-1723
language English
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publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj-art-ba8f28823db64bdca0827e912d2c13ac2025-02-09T12:45:17ZengNature PortfolioNature Communications2041-17232025-02-011611810.1038/s41467-025-56582-7Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5Siqi Wu0Chenchao Xu1Xiaoqun Wang2Hai-Qing Lin3Chao Cao4Guang-Han Cao5School of Physics, Zhejiang UniversitySchool of Physics, Hangzhou Normal UniversitySchool of Physics, Zhejiang UniversitySchool of Physics, Zhejiang UniversitySchool of Physics, Zhejiang UniversitySchool of Physics, Zhejiang UniversityAbstract The spin dynamics and electronic orders of the kagome system at different filling levels stand as an intriguing subject in condensed matter physics. By first-principles calculations and random phase approximation analyses, we investigate the spin fluctuations and superconducting instabilities in kagome phase of CsCr3Sb5 under high pressure. At the filling level slightly below the kagome flat bands, our calculations reveal strong antiferromagnetic spin fluctuations in CsCr3Sb5, together with a leading s ±-wave and a competing (d x y , $${d}_{{x}^{2}-{y}^{2}}$$ d x 2 − y 2 )-wave superconducting order. Unlike the general intuition that the flat bands are closely related to the ferromagnetic correlations, here we propose a sublattice-momentum-coupling-driven mechanism for the antiferromagnetic fluctuations enhanced from the unoccupied flat bands. The mechanism is generally applicable to kagome systems where the Fermi level intersects near the flat bands, offering a new perspective for future studies of geometrically frustrated systems.https://doi.org/10.1038/s41467-025-56582-7
spellingShingle Siqi Wu
Chenchao Xu
Xiaoqun Wang
Hai-Qing Lin
Chao Cao
Guang-Han Cao
Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5
Nature Communications
title Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5
title_full Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5
title_fullStr Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5
title_full_unstemmed Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5
title_short Flat-band enhanced antiferromagnetic fluctuations and superconductivity in pressurized CsCr3Sb5
title_sort flat band enhanced antiferromagnetic fluctuations and superconductivity in pressurized cscr3sb5
url https://doi.org/10.1038/s41467-025-56582-7
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AT haiqinglin flatbandenhancedantiferromagneticfluctuationsandsuperconductivityinpressurizedcscr3sb5
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