High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol Electrooxidation

Abstract The urgent demand for designing highly efficient electrocatalysts for ethanol oxidation reaction (EOR) with elevated C1 selectivity, robust anti‐poisoning capability, and high mass activity presents a formidable challenge. Herein, a novel two‐dimentional (2D) high‐entropy PdRhFeCoMo metalle...

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Main Authors: Xiaohong Tan, Chenhui Wang, Jiarui Wang, Peng Wang, Yuhang Xiao, Yingying Guo, Jianpo Chen, Weidong He, Yan Li, Hao Cui, Chengxin Wang
Format: Article
Language:English
Published: Wiley 2024-12-01
Series:Advanced Science
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Online Access:https://doi.org/10.1002/advs.202409109
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author Xiaohong Tan
Chenhui Wang
Jiarui Wang
Peng Wang
Yuhang Xiao
Yingying Guo
Jianpo Chen
Weidong He
Yan Li
Hao Cui
Chengxin Wang
author_facet Xiaohong Tan
Chenhui Wang
Jiarui Wang
Peng Wang
Yuhang Xiao
Yingying Guo
Jianpo Chen
Weidong He
Yan Li
Hao Cui
Chengxin Wang
author_sort Xiaohong Tan
collection DOAJ
description Abstract The urgent demand for designing highly efficient electrocatalysts for ethanol oxidation reaction (EOR) with elevated C1 selectivity, robust anti‐poisoning capability, and high mass activity presents a formidable challenge. Herein, a novel two‐dimentional (2D) high‐entropy PdRhFeCoMo metallene (PdRhFeCoMo HEM) electrocatalyst is successfully synthesized via a mild one‐step solvothermal method. The PdRhFeCoMo HEM, characterized by intentionally designed multi‐metallic ensembles and ultra‐thin graphene‐like structures, delivers an impressive mass activity of 7.47 A mgPd+Rh−1 and specific activity of 25.5 mA cm−2. Furthermore, it can retain a mass activity of 0.56 A mgPd+Rh−1 after undergoing 20000 s of continuous testing, demonstrating outstanding resistance to poisoning. More significantly, the PdRhFeCoMo HEM demonstrates an elevated capacity for C─C bond cleavage with a superior C1 selectivity of up to 84.12%. In situ spectroscopy analysis, combined with theoretical calculations, reveals that the deliberate design of components and structures effectively regulate the electronic properties of the Pd site, thereby enhancing the adsorption of reactant and reducing the reaction barrier of the C1 pathway. Finally, a flexible solid‐state ethanol fuel cell assembled by PdRhFeCoMo HEM presents a maximum power density of 20.1 mW cm−2 and can operate continuously by repeatedly adding ethanol fuel.
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spelling doaj-art-b9a0be73e8954aa49597c8359a46c69a2024-12-27T13:00:47ZengWileyAdvanced Science2198-38442024-12-011148n/an/a10.1002/advs.202409109High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol ElectrooxidationXiaohong Tan0Chenhui Wang1Jiarui Wang2Peng Wang3Yuhang Xiao4Yingying Guo5Jianpo Chen6Weidong He7Yan Li8Hao Cui9Chengxin Wang10School of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaSchool of Materials Science and Engineering Sun Yat‐sen University Guangzhou 510275 ChinaAbstract The urgent demand for designing highly efficient electrocatalysts for ethanol oxidation reaction (EOR) with elevated C1 selectivity, robust anti‐poisoning capability, and high mass activity presents a formidable challenge. Herein, a novel two‐dimentional (2D) high‐entropy PdRhFeCoMo metallene (PdRhFeCoMo HEM) electrocatalyst is successfully synthesized via a mild one‐step solvothermal method. The PdRhFeCoMo HEM, characterized by intentionally designed multi‐metallic ensembles and ultra‐thin graphene‐like structures, delivers an impressive mass activity of 7.47 A mgPd+Rh−1 and specific activity of 25.5 mA cm−2. Furthermore, it can retain a mass activity of 0.56 A mgPd+Rh−1 after undergoing 20000 s of continuous testing, demonstrating outstanding resistance to poisoning. More significantly, the PdRhFeCoMo HEM demonstrates an elevated capacity for C─C bond cleavage with a superior C1 selectivity of up to 84.12%. In situ spectroscopy analysis, combined with theoretical calculations, reveals that the deliberate design of components and structures effectively regulate the electronic properties of the Pd site, thereby enhancing the adsorption of reactant and reducing the reaction barrier of the C1 pathway. Finally, a flexible solid‐state ethanol fuel cell assembled by PdRhFeCoMo HEM presents a maximum power density of 20.1 mW cm−2 and can operate continuously by repeatedly adding ethanol fuel.https://doi.org/10.1002/advs.202409109anti‐poisoning abilityelevated C1 selectivityethanol oxidation reactionflexible solid‐state fuel cellhigh‐entropy metallene
spellingShingle Xiaohong Tan
Chenhui Wang
Jiarui Wang
Peng Wang
Yuhang Xiao
Yingying Guo
Jianpo Chen
Weidong He
Yan Li
Hao Cui
Chengxin Wang
High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol Electrooxidation
Advanced Science
anti‐poisoning ability
elevated C1 selectivity
ethanol oxidation reaction
flexible solid‐state fuel cell
high‐entropy metallene
title High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol Electrooxidation
title_full High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol Electrooxidation
title_fullStr High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol Electrooxidation
title_full_unstemmed High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol Electrooxidation
title_short High‐Entropy PdRhFeCoMo Metallene With High C1 Selectivity and Anti‐Poisoning Ability for Ethanol Electrooxidation
title_sort high entropy pdrhfecomo metallene with high c1 selectivity and anti poisoning ability for ethanol electrooxidation
topic anti‐poisoning ability
elevated C1 selectivity
ethanol oxidation reaction
flexible solid‐state fuel cell
high‐entropy metallene
url https://doi.org/10.1002/advs.202409109
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