Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray Reactor
Hydrate formation apparatus reported so far was mainly concentrated in stirred-tank batch environments. It was difficult to produce the high gas storage hydrate efficiently. Some nonstirred technology has been attracting more attention by researchers. This work proposed a new apparatus for hydrate f...
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| Format: | Article |
| Language: | English |
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Wiley
2017-01-01
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| Series: | Journal of Chemistry |
| Online Access: | http://dx.doi.org/10.1155/2017/5208915 |
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| author | Yaqin Tian Yugui Li Hongping An Jie Ren Jianfeng Su |
| author_facet | Yaqin Tian Yugui Li Hongping An Jie Ren Jianfeng Su |
| author_sort | Yaqin Tian |
| collection | DOAJ |
| description | Hydrate formation apparatus reported so far was mainly concentrated in stirred-tank batch environments. It was difficult to produce the high gas storage hydrate efficiently. Some nonstirred technology has been attracting more attention by researchers. This work proposed a new apparatus for hydrate formation by spraying water into a gaseous phase with a fine nozzle. It can get sufficient contact surface area for gas-liquid reaction. Methane hydrate formation experiments have been conducted using pure water and sodium dodecyl sulfate (SDS) aqueous solution for comparison at 277.15 K. The experiments were conducted at 7.0 and 6.0 MPa, respectively. Kinetics of methane hydrate formation have been investigated by methane consumption per mole of water and reaction rate. The mechanism of hydrate formation and kinetics property by spraying atomization were studied with the theory of crystal chemistry. |
| format | Article |
| id | doaj-art-b948ed3ffa30462ebb77ba12dab050d7 |
| institution | DOAJ |
| issn | 2090-9063 2090-9071 |
| language | English |
| publishDate | 2017-01-01 |
| publisher | Wiley |
| record_format | Article |
| series | Journal of Chemistry |
| spelling | doaj-art-b948ed3ffa30462ebb77ba12dab050d72025-08-20T03:23:12ZengWileyJournal of Chemistry2090-90632090-90712017-01-01201710.1155/2017/52089155208915Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray ReactorYaqin Tian0Yugui Li1Hongping An2Jie Ren3Jianfeng Su4College of Materials Science and Engineering, Taiyuan University of Science and Technology, Taiyuan 030024, ChinaCollege of Materials Science and Engineering, Taiyuan University of Science and Technology, Taiyuan 030024, ChinaCollege of Materials Science and Engineering, Taiyuan University of Science and Technology, Taiyuan 030024, ChinaCollege of Materials Science and Engineering, Taiyuan University of Science and Technology, Taiyuan 030024, ChinaCollege of Materials Science and Engineering, Taiyuan University of Science and Technology, Taiyuan 030024, ChinaHydrate formation apparatus reported so far was mainly concentrated in stirred-tank batch environments. It was difficult to produce the high gas storage hydrate efficiently. Some nonstirred technology has been attracting more attention by researchers. This work proposed a new apparatus for hydrate formation by spraying water into a gaseous phase with a fine nozzle. It can get sufficient contact surface area for gas-liquid reaction. Methane hydrate formation experiments have been conducted using pure water and sodium dodecyl sulfate (SDS) aqueous solution for comparison at 277.15 K. The experiments were conducted at 7.0 and 6.0 MPa, respectively. Kinetics of methane hydrate formation have been investigated by methane consumption per mole of water and reaction rate. The mechanism of hydrate formation and kinetics property by spraying atomization were studied with the theory of crystal chemistry.http://dx.doi.org/10.1155/2017/5208915 |
| spellingShingle | Yaqin Tian Yugui Li Hongping An Jie Ren Jianfeng Su Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray Reactor Journal of Chemistry |
| title | Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray Reactor |
| title_full | Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray Reactor |
| title_fullStr | Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray Reactor |
| title_full_unstemmed | Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray Reactor |
| title_short | Kinetics of Methane Hydrate Formation in an Aqueous Solution with and without Kinetic Promoter (SDS) by Spray Reactor |
| title_sort | kinetics of methane hydrate formation in an aqueous solution with and without kinetic promoter sds by spray reactor |
| url | http://dx.doi.org/10.1155/2017/5208915 |
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