Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)

Indocyanine green is a great near-infrared fluorescence with good luminescent properties and important medical applications. In this paper, the theoretical spectrum and orbital model of its molecular level are established. The two most probable conformations were studied, and their energies, vibrati...

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Main Authors: Zhao Liu, Shu-Tao Wang, Yan-Song Hu, Jia-Rong You, Yong-Sheng Xv, Jun-Qiang Lei
Format: Article
Language:English
Published: Wiley 2022-01-01
Series:Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2022/4321595
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author Zhao Liu
Shu-Tao Wang
Yan-Song Hu
Jia-Rong You
Yong-Sheng Xv
Jun-Qiang Lei
author_facet Zhao Liu
Shu-Tao Wang
Yan-Song Hu
Jia-Rong You
Yong-Sheng Xv
Jun-Qiang Lei
author_sort Zhao Liu
collection DOAJ
description Indocyanine green is a great near-infrared fluorescence with good luminescent properties and important medical applications. In this paper, the theoretical spectrum and orbital model of its molecular level are established. The two most probable conformations were studied, and their energies, vibrational spectra, UV-Vis absorption spectra, frontier molecular orbitals (HOMO and LUMO), and energy gaps were obtained by density functional theory (DFT) calculations, respectively. This provides a theoretical and design basis for the development of novel dyes similar to indocyanine green dyes and a reference case for improved application methods and synthetic predesign of novel fluorescent dyes.
format Article
id doaj-art-b8fc9e12f20049b7a85bfb79f1967526
institution DOAJ
issn 2090-9071
language English
publishDate 2022-01-01
publisher Wiley
record_format Article
series Journal of Chemistry
spelling doaj-art-b8fc9e12f20049b7a85bfb79f19675262025-08-20T03:22:49ZengWileyJournal of Chemistry2090-90712022-01-01202210.1155/2022/4321595Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)Zhao Liu0Shu-Tao Wang1Yan-Song Hu2Jia-Rong You3Yong-Sheng Xv4Jun-Qiang Lei5First Hospital of Lanzhou UniversityState Key Laboratory of Applied Organic ChemistryState Key Laboratory of Applied Organic ChemistryFirst Hospital of Lanzhou UniversityFirst Hospital of Lanzhou UniversityFirst Hospital of Lanzhou UniversityIndocyanine green is a great near-infrared fluorescence with good luminescent properties and important medical applications. In this paper, the theoretical spectrum and orbital model of its molecular level are established. The two most probable conformations were studied, and their energies, vibrational spectra, UV-Vis absorption spectra, frontier molecular orbitals (HOMO and LUMO), and energy gaps were obtained by density functional theory (DFT) calculations, respectively. This provides a theoretical and design basis for the development of novel dyes similar to indocyanine green dyes and a reference case for improved application methods and synthetic predesign of novel fluorescent dyes.http://dx.doi.org/10.1155/2022/4321595
spellingShingle Zhao Liu
Shu-Tao Wang
Yan-Song Hu
Jia-Rong You
Yong-Sheng Xv
Jun-Qiang Lei
Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)
Journal of Chemistry
title Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)
title_full Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)
title_fullStr Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)
title_full_unstemmed Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)
title_short Theoretical Study on Spectrum and Luminescence Mechanism of Indocyanine Green Dye Based on Density Functional Theory (DFT)
title_sort theoretical study on spectrum and luminescence mechanism of indocyanine green dye based on density functional theory dft
url http://dx.doi.org/10.1155/2022/4321595
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