Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational Approach

The increasing demand for advanced materials capable of withstanding high-temperature and harsh environments, such as those utilized in nuclear reactors and aerospace applications, has driven significant interest in Oxide Dispersion Strengthened (ODS) alloys. While these materials offer remarkable t...

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Main Authors: Sarah Najm Al-Challabi, Ali Samer Muhsan, Thar Mohammed Badri, Mohammad Shakir Nasif
Format: Article
Language:English
Published: Elsevier 2025-06-01
Series:Results in Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2590123025008485
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author Sarah Najm Al-Challabi
Ali Samer Muhsan
Thar Mohammed Badri
Mohammad Shakir Nasif
author_facet Sarah Najm Al-Challabi
Ali Samer Muhsan
Thar Mohammed Badri
Mohammad Shakir Nasif
author_sort Sarah Najm Al-Challabi
collection DOAJ
description The increasing demand for advanced materials capable of withstanding high-temperature and harsh environments, such as those utilized in nuclear reactors and aerospace applications, has driven significant interest in Oxide Dispersion Strengthened (ODS) alloys. While these materials offer remarkable thermomechanical properties, challenges remain in optimizing their phase stability and microstructural evolution during additive manufacturing processes such as Wire Arc Additive Manufacturing (WAAM) and Plasma Additive Manufacturing (PAM). This study addresses the gaps in the literature regarding the impact of processing parameters (temperature and scanning speed) nickel (Ni) content on the phase stability of 9Cr-ODS alloys. Using computational thermodynamics tools, including CALPHAD, the Scheil-Gulliver model, and DICTRA simulations, this study evaluates the effects of temperature (1480-1550°C), scanning speed (0.1 - 0.2 m/s), and Ni content (0.27-8%) on the formation of FCC, BCC, and carbide (M7C3) phases. Elemental distribution analysis across a 100 µm region confirms a stable FCC_L12 phase composition (100%) with no detectable M7C3_D101 phase. Thermal property analysis indicates a liquidus temperature range of 1470.27°C to 1500.67°C and a solidus temperature range of 1387.91°C to 1462.38°C, with thermal conductivity varying between 23.05 W/m·K and 27.56 W/m·K. Phase composition studies using the Scheil model reveal that at 1480°C, the FCC_L12 phase comprises 65% of the solidified structure, decreasing to 55% at 1500°C and further reducing to 45% at 1550°C, where BCC_B2 becomes dominant at 55%. These insights highlight the importance of precise control over processing parameters to optimize the mechanical and thermal performance of 9Cr-ODS alloys. The study underscores the utility of computational tools in predicting phase transformations, reducing experimental iterations, and guiding process optimization. Future research should explore advanced cooling techniques, broader parameter ranges, and the long-term stability of these alloys under cyclic thermal and mechanical loads to support their application in demanding industries like nuclear energy and aerospace.
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spelling doaj-art-b8c5735ad4e34cdc9c0ee932c0f509d42025-08-20T02:16:09ZengElsevierResults in Engineering2590-12302025-06-012610477110.1016/j.rineng.2025.104771Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational ApproachSarah Najm Al-Challabi0Ali Samer Muhsan1Thar Mohammed Badri2Mohammad Shakir Nasif3Department of Mechanical Engineering Universiti Technologi PETRONAS, Bandar Seri Iskandar, 32610, Malaysia; Corresponding authors.Department of Mechanical Engineering Universiti Technologi PETRONAS, Bandar Seri Iskandar, 32610, MalaysiaElectromechanical Engineering Department, University of Technology, Baghdad 10066, Baghdad, Iraq; Corresponding authors.Department of Mechanical Engineering Universiti Technologi PETRONAS, Bandar Seri Iskandar, 32610, MalaysiaThe increasing demand for advanced materials capable of withstanding high-temperature and harsh environments, such as those utilized in nuclear reactors and aerospace applications, has driven significant interest in Oxide Dispersion Strengthened (ODS) alloys. While these materials offer remarkable thermomechanical properties, challenges remain in optimizing their phase stability and microstructural evolution during additive manufacturing processes such as Wire Arc Additive Manufacturing (WAAM) and Plasma Additive Manufacturing (PAM). This study addresses the gaps in the literature regarding the impact of processing parameters (temperature and scanning speed) nickel (Ni) content on the phase stability of 9Cr-ODS alloys. Using computational thermodynamics tools, including CALPHAD, the Scheil-Gulliver model, and DICTRA simulations, this study evaluates the effects of temperature (1480-1550°C), scanning speed (0.1 - 0.2 m/s), and Ni content (0.27-8%) on the formation of FCC, BCC, and carbide (M7C3) phases. Elemental distribution analysis across a 100 µm region confirms a stable FCC_L12 phase composition (100%) with no detectable M7C3_D101 phase. Thermal property analysis indicates a liquidus temperature range of 1470.27°C to 1500.67°C and a solidus temperature range of 1387.91°C to 1462.38°C, with thermal conductivity varying between 23.05 W/m·K and 27.56 W/m·K. Phase composition studies using the Scheil model reveal that at 1480°C, the FCC_L12 phase comprises 65% of the solidified structure, decreasing to 55% at 1500°C and further reducing to 45% at 1550°C, where BCC_B2 becomes dominant at 55%. These insights highlight the importance of precise control over processing parameters to optimize the mechanical and thermal performance of 9Cr-ODS alloys. The study underscores the utility of computational tools in predicting phase transformations, reducing experimental iterations, and guiding process optimization. Future research should explore advanced cooling techniques, broader parameter ranges, and the long-term stability of these alloys under cyclic thermal and mechanical loads to support their application in demanding industries like nuclear energy and aerospace.http://www.sciencedirect.com/science/article/pii/S2590123025008485Additive ManufacturingPhase StabilityThermal StabilityComputational ThermodynamicsHigh-Temperature Applications
spellingShingle Sarah Najm Al-Challabi
Ali Samer Muhsan
Thar Mohammed Badri
Mohammad Shakir Nasif
Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational Approach
Results in Engineering
Additive Manufacturing
Phase Stability
Thermal Stability
Computational Thermodynamics
High-Temperature Applications
title Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational Approach
title_full Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational Approach
title_fullStr Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational Approach
title_full_unstemmed Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational Approach
title_short Phase Stability and Solidification of 9Cr-ODS Alloys for Wire Additive Manufacturing: A Computational Approach
title_sort phase stability and solidification of 9cr ods alloys for wire additive manufacturing a computational approach
topic Additive Manufacturing
Phase Stability
Thermal Stability
Computational Thermodynamics
High-Temperature Applications
url http://www.sciencedirect.com/science/article/pii/S2590123025008485
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