Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double Hydroxide

We describe the synthesis of a composite carbon derived from zinc–aluminium-layered double hydroxides. The material was characterized by powder X-ray diffraction, Fourier transform infrared/attenuated total reflectance spectroscopy, thermogravimetric analysis–differential scanning calorimetry–mass s...

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Main Authors: Rodrigo Morais Menezes dos Santos, Rosembergue Gabriel Lima Gonçalves, Marina de Carvalho Eufrásio Pinto, Roberta Gomes Prado, Vera Regina Leopoldo Constantino, Liovando Marciano da Costa, Frederico Garcia Pinto, Jairo Tronto
Format: Article
Language:English
Published: SAGE Publishing 2013-08-01
Series:Adsorption Science & Technology
Online Access:https://doi.org/10.1260/0263-6174.31.8.711
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author Rodrigo Morais Menezes dos Santos
Rosembergue Gabriel Lima Gonçalves
Marina de Carvalho Eufrásio Pinto
Roberta Gomes Prado
Vera Regina Leopoldo Constantino
Liovando Marciano da Costa
Frederico Garcia Pinto
Jairo Tronto
author_facet Rodrigo Morais Menezes dos Santos
Rosembergue Gabriel Lima Gonçalves
Marina de Carvalho Eufrásio Pinto
Roberta Gomes Prado
Vera Regina Leopoldo Constantino
Liovando Marciano da Costa
Frederico Garcia Pinto
Jairo Tronto
author_sort Rodrigo Morais Menezes dos Santos
collection DOAJ
description We describe the synthesis of a composite carbon derived from zinc–aluminium-layered double hydroxides. The material was characterized by powder X-ray diffraction, Fourier transform infrared/attenuated total reflectance spectroscopy, thermogravimetric analysis–differential scanning calorimetry–mass spectrometry, measurement of BET specific surface area, zeta-potential analysis and scanning electron microscopy. The resulting material was used for adsorption studies with an anionic surfactant, sodium dodecylbenzenesulphonate, and a cationic surfactant, cetyltrimethylammonium bromide, as adsorbates. The adsorption of the surfactants was well described by the typical Langmuir pattern. An investigation of the influence of initial pH of a medium on surfactant adsorption showed that high pH values decrease the adsorption capacity of the adsorbent. The adsorption processes were exothermic. The results also showed that the adsorption of the two surfactants was chemical and that the kinetic models were best described by a pseudo-second-order model.
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id doaj-art-b85f4a502b0f4a29bfbdcbd5939adc23
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issn 0263-6174
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language English
publishDate 2013-08-01
publisher SAGE Publishing
record_format Article
series Adsorption Science & Technology
spelling doaj-art-b85f4a502b0f4a29bfbdcbd5939adc232025-08-20T02:44:24ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382013-08-013110.1260/0263-6174.31.8.711Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double HydroxideRodrigo Morais Menezes dos Santos0Rosembergue Gabriel Lima Gonçalves1Marina de Carvalho Eufrásio Pinto2Roberta Gomes Prado3Vera Regina Leopoldo Constantino4Liovando Marciano da Costa5Frederico Garcia Pinto6Jairo Tronto7 Institute of Science and Technology, Federal University of Viçosa, Rio Paranaíba Campus, Rio Paranaíba 38810-000, Minas Gerais, Brazil Institute of Science and Technology, Federal University of Viçosa, Rio Paranaíba Campus, Rio Paranaíba 38810-000, Minas Gerais, Brazil Institute of Science and Technology, Federal University of Viçosa, Rio Paranaíba Campus, Rio Paranaíba 38810-000, Minas Gerais, Brazil Department of Chemistry, Fuel Testing Laboratory, Institute of Science, Federal University of Minas Gerais, Avenida Antônio Carlos 6627, Belo Horizonte 31270-901, Minas Gerais, Brazil Department of Fundamental Chemistry, Institute of Chemistry, University of São Paulo, Avenida Lineus Prestes 748, São Paulo City 05508-000, São Paulo, Brazil Department of Soil, Federal University of Viçosa, Avenida Peter Henry Rolfs, Viçosa 36570-000, Minas Gerais, Brazil Institute of Science and Technology, Federal University of Viçosa, Rio Paranaíba Campus, Rio Paranaíba 38810-000, Minas Gerais, Brazil Institute of Science and Technology, Federal University of Viçosa, Rio Paranaíba Campus, Rio Paranaíba 38810-000, Minas Gerais, BrazilWe describe the synthesis of a composite carbon derived from zinc–aluminium-layered double hydroxides. The material was characterized by powder X-ray diffraction, Fourier transform infrared/attenuated total reflectance spectroscopy, thermogravimetric analysis–differential scanning calorimetry–mass spectrometry, measurement of BET specific surface area, zeta-potential analysis and scanning electron microscopy. The resulting material was used for adsorption studies with an anionic surfactant, sodium dodecylbenzenesulphonate, and a cationic surfactant, cetyltrimethylammonium bromide, as adsorbates. The adsorption of the surfactants was well described by the typical Langmuir pattern. An investigation of the influence of initial pH of a medium on surfactant adsorption showed that high pH values decrease the adsorption capacity of the adsorbent. The adsorption processes were exothermic. The results also showed that the adsorption of the two surfactants was chemical and that the kinetic models were best described by a pseudo-second-order model.https://doi.org/10.1260/0263-6174.31.8.711
spellingShingle Rodrigo Morais Menezes dos Santos
Rosembergue Gabriel Lima Gonçalves
Marina de Carvalho Eufrásio Pinto
Roberta Gomes Prado
Vera Regina Leopoldo Constantino
Liovando Marciano da Costa
Frederico Garcia Pinto
Jairo Tronto
Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double Hydroxide
Adsorption Science & Technology
title Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double Hydroxide
title_full Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double Hydroxide
title_fullStr Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double Hydroxide
title_full_unstemmed Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double Hydroxide
title_short Removal of Sodium Dodecylbenzenesulphonate and Cetyltrimethylammonium Bromide Using a Carbon Composite Derived from Modified Zn–Al-Layered Double Hydroxide
title_sort removal of sodium dodecylbenzenesulphonate and cetyltrimethylammonium bromide using a carbon composite derived from modified zn al layered double hydroxide
url https://doi.org/10.1260/0263-6174.31.8.711
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