Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling Cascade

<b>Aim</b>: Myricetin, a natural bioflavonoid, is reported as an anti-diabetic agent since it possesses the ability to inhibit α-glucosidase activity, stimulate insulin action and secretion, manage ROS, and prevent diabetes complications. Myricetin was identified as a new insulin secreta...

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Main Authors: Akhtar Ali, Zahida Memon, Abdul Hameed, Zaheer Ul-Haq, Muneeb Ali, Rahman M. Hafizur
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Biomedicines
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Online Access:https://www.mdpi.com/2227-9059/13/6/1447
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author Akhtar Ali
Zahida Memon
Abdul Hameed
Zaheer Ul-Haq
Muneeb Ali
Rahman M. Hafizur
author_facet Akhtar Ali
Zahida Memon
Abdul Hameed
Zaheer Ul-Haq
Muneeb Ali
Rahman M. Hafizur
author_sort Akhtar Ali
collection DOAJ
description <b>Aim</b>: Myricetin, a natural bioflavonoid, is reported as an anti-diabetic agent since it possesses the ability to inhibit α-glucosidase activity, stimulate insulin action and secretion, manage ROS, and prevent diabetes complications. Myricetin was identified as a new insulin secretagogue that enhances glucose-stimulated insulin secretion and seems like a better antidiabetic drug candidate. Here, we explored the insulinotropic mechanism(s) of myricetin <i>in vitro</i> in mice islets and <i>in silico</i>. <b>Methods</b>: Size-matched pancreatic islets were divided into groups and incubated in the presence or absence of myricetin and agonists/antagonists of major insulin signaling pathways. The secreted insulin was measured by ELISA. Molecular docking studies were performed with the key player of insulin secretory pathways. <b>Results</b>: Myricetin dose-dependently enhanced insulin secretion in isolated mice islets, and its insulinotropic effect was exerted at high glucose concentrations distinctly different from glibenclamide. Myricetin-induced insulin secretion was significantly inhibited using the diazoxide. Furthermore, myricetin amplified glucose-induced insulin secretion in depolarized and glibenclamide-treated islets. Myricetin showed an additive effect with forskolin- and IBMX-induced insulin secretion. Interestingly, H89, a PKA inhibitor, and MAY0132, an Epac-2 inhibitor, significantly inhibited myricetin-induced insulin secretion. The <i>in silico</i> molecular docking studies further validated these <i>in vitro</i> findings in isolated pancreatic islets. <b>Conclusions</b>: Myricetin, a potential natural insulin secretagogue, amplifies glucose-induced insulin secretion <i>via</i> the cAMP-PKA-Epac-2 signaling pathway.
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institution Kabale University
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publishDate 2025-06-01
publisher MDPI AG
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spelling doaj-art-b8052bc491ac487cb39abec97cffcb6f2025-08-20T03:27:22ZengMDPI AGBiomedicines2227-90592025-06-01136144710.3390/biomedicines13061447Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling CascadeAkhtar Ali0Zahida Memon1Abdul Hameed2Zaheer Ul-Haq3Muneeb Ali4Rahman M. Hafizur5Department of Pharmacology, Ziauddin University Karachi, Karachi 75000, PakistanDepartment of Pharmacology, Ziauddin University Karachi, Karachi 75000, PakistanZiauddin College of Molecular Medicine, Ziauddin University Karachi, Karachi 75000, PakistanDr. Panjwani Center for Molecular Medicine and Drug Research, International Center for Chemical and Biological Sciences, University of Karachi, Karachi 75270, PakistanDr. Panjwani Center for Molecular Medicine and Drug Research, International Center for Chemical and Biological Sciences, University of Karachi, Karachi 75270, PakistanDr. Panjwani Center for Molecular Medicine and Drug Research, International Center for Chemical and Biological Sciences, University of Karachi, Karachi 75270, Pakistan<b>Aim</b>: Myricetin, a natural bioflavonoid, is reported as an anti-diabetic agent since it possesses the ability to inhibit α-glucosidase activity, stimulate insulin action and secretion, manage ROS, and prevent diabetes complications. Myricetin was identified as a new insulin secretagogue that enhances glucose-stimulated insulin secretion and seems like a better antidiabetic drug candidate. Here, we explored the insulinotropic mechanism(s) of myricetin <i>in vitro</i> in mice islets and <i>in silico</i>. <b>Methods</b>: Size-matched pancreatic islets were divided into groups and incubated in the presence or absence of myricetin and agonists/antagonists of major insulin signaling pathways. The secreted insulin was measured by ELISA. Molecular docking studies were performed with the key player of insulin secretory pathways. <b>Results</b>: Myricetin dose-dependently enhanced insulin secretion in isolated mice islets, and its insulinotropic effect was exerted at high glucose concentrations distinctly different from glibenclamide. Myricetin-induced insulin secretion was significantly inhibited using the diazoxide. Furthermore, myricetin amplified glucose-induced insulin secretion in depolarized and glibenclamide-treated islets. Myricetin showed an additive effect with forskolin- and IBMX-induced insulin secretion. Interestingly, H89, a PKA inhibitor, and MAY0132, an Epac-2 inhibitor, significantly inhibited myricetin-induced insulin secretion. The <i>in silico</i> molecular docking studies further validated these <i>in vitro</i> findings in isolated pancreatic islets. <b>Conclusions</b>: Myricetin, a potential natural insulin secretagogue, amplifies glucose-induced insulin secretion <i>via</i> the cAMP-PKA-Epac-2 signaling pathway.https://www.mdpi.com/2227-9059/13/6/1447myricetininsulin secretionsulfonylureaantidiabetic drugsinsulin secretagogues
spellingShingle Akhtar Ali
Zahida Memon
Abdul Hameed
Zaheer Ul-Haq
Muneeb Ali
Rahman M. Hafizur
Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling Cascade
Biomedicines
myricetin
insulin secretion
sulfonylurea
antidiabetic drugs
insulin secretagogues
title Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling Cascade
title_full Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling Cascade
title_fullStr Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling Cascade
title_full_unstemmed Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling Cascade
title_short Myricetin Amplifies Glucose–Stimulated Insulin Secretion via the cAMP-PKA-Epac-2 Signaling Cascade
title_sort myricetin amplifies glucose stimulated insulin secretion via the camp pka epac 2 signaling cascade
topic myricetin
insulin secretion
sulfonylurea
antidiabetic drugs
insulin secretagogues
url https://www.mdpi.com/2227-9059/13/6/1447
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AT zahidamemon myricetinamplifiesglucosestimulatedinsulinsecretionviathecamppkaepac2signalingcascade
AT abdulhameed myricetinamplifiesglucosestimulatedinsulinsecretionviathecamppkaepac2signalingcascade
AT zaheerulhaq myricetinamplifiesglucosestimulatedinsulinsecretionviathecamppkaepac2signalingcascade
AT muneebali myricetinamplifiesglucosestimulatedinsulinsecretionviathecamppkaepac2signalingcascade
AT rahmanmhafizur myricetinamplifiesglucosestimulatedinsulinsecretionviathecamppkaepac2signalingcascade