HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-

Nonahydro-closo-nonaborate anion possess the property of structural nonrigidity because of presence of three low-coordinated boron atoms. So it’s able to come into the reactions of polyhedral extension. This paper is devoted to the reactions of homoatomic polyhedral extension in nonahydrocloso-nonab...

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Main Authors: A. Yu. Bykov, N. A. Selivanov, A. P. Zhdanov, K. Yu. Zhizhin, N. T. Kuznetsov
Format: Article
Language:Russian
Published: MIREA - Russian Technological University 2016-04-01
Series:Тонкие химические технологии
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Online Access:https://www.finechem-mirea.ru/jour/article/view/17
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author A. Yu. Bykov
N. A. Selivanov
A. P. Zhdanov
K. Yu. Zhizhin
N. T. Kuznetsov
author_facet A. Yu. Bykov
N. A. Selivanov
A. P. Zhdanov
K. Yu. Zhizhin
N. T. Kuznetsov
author_sort A. Yu. Bykov
collection DOAJ
description Nonahydro-closo-nonaborate anion possess the property of structural nonrigidity because of presence of three low-coordinated boron atoms. So it’s able to come into the reactions of polyhedral extension. This paper is devoted to the reactions of homoatomic polyhedral extension in nonahydrocloso-nonaborate anion [B9H9]2- in presence of triethylaminborane complex BH3·(C2H5)3N. It was shown that mixes of [B10H10]2- and [B12H12]2- salts in various molar ratios had been formed as products. These ratios depend on proportion of reagents. In presence of excess of triethylamin borane complex the molar ratio of products is 1:1. When equimolar amount of triethyamminborane complex used, the selectivity of process shifted to formation of [B10H10]2- anion. However the formation of [B12H12]2- still occurs in this conditions but the molar ratio of [B10H10]2-:[B12H12]2- is 5:1.
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series Тонкие химические технологии
spelling doaj-art-b73c3e16108e46c4a37ed2248c0774bd2025-08-20T03:23:10ZrusMIREA - Russian Technological UniversityТонкие химические технологии2410-65932686-75752016-04-01112464910.32362/2410-6593-2016-11-2-46-4917HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-A. Yu. Bykov0N. A. Selivanov1A. P. Zhdanov2K. Yu. Zhizhin3N. T. Kuznetsov4Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of SciencesKurnakov Institute of General and Inorganic Chemistry, Russian Academy of SciencesKurnakov Institute of General and Inorganic Chemistry, Russian Academy of SciencesKurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences Moscow Technological University (Institute of Fine Chemical Technologies)Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of SciencesNonahydro-closo-nonaborate anion possess the property of structural nonrigidity because of presence of three low-coordinated boron atoms. So it’s able to come into the reactions of polyhedral extension. This paper is devoted to the reactions of homoatomic polyhedral extension in nonahydrocloso-nonaborate anion [B9H9]2- in presence of triethylaminborane complex BH3·(C2H5)3N. It was shown that mixes of [B10H10]2- and [B12H12]2- salts in various molar ratios had been formed as products. These ratios depend on proportion of reagents. In presence of excess of triethylamin borane complex the molar ratio of products is 1:1. When equimolar amount of triethyamminborane complex used, the selectivity of process shifted to formation of [B10H10]2- anion. However the formation of [B12H12]2- still occurs in this conditions but the molar ratio of [B10H10]2-:[B12H12]2- is 5:1.https://www.finechem-mirea.ru/jour/article/view/17b9h92-b10h102-b12h122-boron hydridescloso-boratespolyhedral extension
spellingShingle A. Yu. Bykov
N. A. Selivanov
A. P. Zhdanov
K. Yu. Zhizhin
N. T. Kuznetsov
HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-
Тонкие химические технологии
b9h92-
b10h102-
b12h122-
boron hydrides
closo-borates
polyhedral extension
title HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-
title_full HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-
title_fullStr HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-
title_full_unstemmed HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-
title_short HOMOATOMIC POLYHEDRAL EXTENSION IN NONAHYDRO-closo-NONABORATE ANION [B9H9]2-
title_sort homoatomic polyhedral extension in nonahydro closo nonaborate anion b9h9 2
topic b9h92-
b10h102-
b12h122-
boron hydrides
closo-borates
polyhedral extension
url https://www.finechem-mirea.ru/jour/article/view/17
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AT naselivanov homoatomicpolyhedralextensioninnonahydroclosononaborateanionb9h92
AT apzhdanov homoatomicpolyhedralextensioninnonahydroclosononaborateanionb9h92
AT kyuzhizhin homoatomicpolyhedralextensioninnonahydroclosononaborateanionb9h92
AT ntkuznetsov homoatomicpolyhedralextensioninnonahydroclosononaborateanionb9h92