Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogs

Unsymmetrical monocarbonyl curcumin analogs containing 1,2,3-triazole scaffold (5a-5f) have been synthesized from vanillin. 5d, which contains a carboxylic group, exhibited the highest antioxidant and cytotoxic activities, with an IC50 of 0.56 mM against DPPH and an IC50 of 38.25 ± 4.79 μM against M...

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Main Authors: Bayu Ardiansah, Ahmad Farhan, Novita Sari Nurhasanah, Mochammad Arfin Fardiansyah Nasution, Noordini M. Salleh, Kenji Mizuguchi, Antonius Herry Cahyana, Lina Mardiana
Format: Article
Language:English
Published: Elsevier 2025-06-01
Series:Case Studies in Chemical and Environmental Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2666016424004250
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author Bayu Ardiansah
Ahmad Farhan
Novita Sari Nurhasanah
Mochammad Arfin Fardiansyah Nasution
Noordini M. Salleh
Kenji Mizuguchi
Antonius Herry Cahyana
Lina Mardiana
author_facet Bayu Ardiansah
Ahmad Farhan
Novita Sari Nurhasanah
Mochammad Arfin Fardiansyah Nasution
Noordini M. Salleh
Kenji Mizuguchi
Antonius Herry Cahyana
Lina Mardiana
author_sort Bayu Ardiansah
collection DOAJ
description Unsymmetrical monocarbonyl curcumin analogs containing 1,2,3-triazole scaffold (5a-5f) have been synthesized from vanillin. 5d, which contains a carboxylic group, exhibited the highest antioxidant and cytotoxic activities, with an IC50 of 0.56 mM against DPPH and an IC50 of 38.25 ± 4.79 μM against MCF-7 cells. Docking studies revealed that 5d has high binding affinity for the tubulin protein, with predicted binding value of −10.4 kcal/mol. Additionally, in silico ADME predictions indicated that 5d demonstrates high gastrointestinal absorption and moderate intrinsic clearance. These findings indicate that the designed compounds, particularly compound 5d, could be promising for developing a new drug candidate.
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publishDate 2025-06-01
publisher Elsevier
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series Case Studies in Chemical and Environmental Engineering
spelling doaj-art-b4589b6ce59f41c4b2ae4c4d5216dae02025-08-20T02:38:23ZengElsevierCase Studies in Chemical and Environmental Engineering2666-01642025-06-011110103110.1016/j.cscee.2024.101031Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogsBayu Ardiansah0Ahmad Farhan1Novita Sari Nurhasanah2Mochammad Arfin Fardiansyah Nasution3Noordini M. Salleh4Kenji Mizuguchi5Antonius Herry Cahyana6Lina Mardiana7Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Indonesia, Depok, 16424, Indonesia; Corresponding author.Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Indonesia, Depok, 16424, IndonesiaDepartment of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Indonesia, Depok, 16424, IndonesiaInstitute for Protein Research, Osaka University, 3-2 Yamadaoka, Suita, Osaka, 565-0871, JapanDepartment of Chemistry, Faculty of Science, Universiti Malaya, 50603, Kuala Lumpur, MalaysiaInstitute for Protein Research, Osaka University, 3-2 Yamadaoka, Suita, Osaka, 565-0871, JapanDepartment of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Indonesia, Depok, 16424, IndonesiaDepartment of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Indonesia, Depok, 16424, IndonesiaUnsymmetrical monocarbonyl curcumin analogs containing 1,2,3-triazole scaffold (5a-5f) have been synthesized from vanillin. 5d, which contains a carboxylic group, exhibited the highest antioxidant and cytotoxic activities, with an IC50 of 0.56 mM against DPPH and an IC50 of 38.25 ± 4.79 μM against MCF-7 cells. Docking studies revealed that 5d has high binding affinity for the tubulin protein, with predicted binding value of −10.4 kcal/mol. Additionally, in silico ADME predictions indicated that 5d demonstrates high gastrointestinal absorption and moderate intrinsic clearance. These findings indicate that the designed compounds, particularly compound 5d, could be promising for developing a new drug candidate.http://www.sciencedirect.com/science/article/pii/S2666016424004250Curcumin analogs1,2,3-triazoleHybrid compoundsCytotoxicAntioxidant
spellingShingle Bayu Ardiansah
Ahmad Farhan
Novita Sari Nurhasanah
Mochammad Arfin Fardiansyah Nasution
Noordini M. Salleh
Kenji Mizuguchi
Antonius Herry Cahyana
Lina Mardiana
Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogs
Case Studies in Chemical and Environmental Engineering
Curcumin analogs
1,2,3-triazole
Hybrid compounds
Cytotoxic
Antioxidant
title Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogs
title_full Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogs
title_fullStr Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogs
title_full_unstemmed Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogs
title_short Dual antioxidant and cytotoxic activities of novel 1,2,3-triazole-decorated unsymmetrical monocarbonyl curcumin analogs
title_sort dual antioxidant and cytotoxic activities of novel 1 2 3 triazole decorated unsymmetrical monocarbonyl curcumin analogs
topic Curcumin analogs
1,2,3-triazole
Hybrid compounds
Cytotoxic
Antioxidant
url http://www.sciencedirect.com/science/article/pii/S2666016424004250
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