Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sites

Water-resistant PVA (polyvinyl alcohol) electrospun membranes with different crosslinking mechanisms were synthesized using the facile electrospinning technique. The crosslinking mechanisms were differentiated by introducing 2 different functional groups of different crosslinker agents into the mole...

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Main Authors: Ihsan Alfikro, Jorena Jorena, Octavianus Cakra Satya, Erry Koriyanti, Fiber Monado, Idha Royani
Format: Article
Language:English
Published: Ural Federal University 2024-06-01
Series:Chimica Techno Acta
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Online Access:https://chimicatechnoacta.ru/article/view/7743
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author Ihsan Alfikro
Jorena Jorena
Octavianus Cakra Satya
Erry Koriyanti
Fiber Monado
Idha Royani
author_facet Ihsan Alfikro
Jorena Jorena
Octavianus Cakra Satya
Erry Koriyanti
Fiber Monado
Idha Royani
author_sort Ihsan Alfikro
collection DOAJ
description Water-resistant PVA (polyvinyl alcohol) electrospun membranes with different crosslinking mechanisms were synthesized using the facile electrospinning technique. The crosslinking mechanisms were differentiated by introducing 2 different functional groups of different crosslinker agents into the molecular structure of the membrane. The evaluation of water resistance was conducted by both micro- and macro-structural analyses, such as Fourier Transform Infrared spectroscopy (FTIR), Scanning Electron Microscope (SEM), Energy Dispersive X-ray Spectroscopy (EDS), X-ray Diffraction (XRD), water contact angle (WCA), and immersion test. Infrared spectra confirmed the formation of new bands at around 1700 cm-1, which are acetal or ester groups, indicating the successful crosslinked process. Additionally, the lowered intensity of hydroxyl groups also signifies that the membrane is water-resistant. The XRD patterns showed the signature peak of PVA at the angle of 20°. Furthermore, the reduction in iron content, as shown by EDS spectra, was attributed to the surface imprinting process. SEM images displayed the formation of nanofibers, with mean diameters of 103 nm and interconnecting nanobead structures. The results showed that WCA was significantly enhanced, up to 91°, with minor loss in structure during water immersion test for 24 h. These findings confirm the hydrophobic characteristics of the membranes and their potential application in water-related fields.
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issn 2411-1414
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publisher Ural Federal University
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spelling doaj-art-b4583136e1ac44bbaa519e2e8898f0532025-08-20T02:02:40ZengUral Federal UniversityChimica Techno Acta2411-14142024-06-0111310.15826/chimtech.2024.11.3.015372Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sitesIhsan Alfikro0Jorena Jorena1Octavianus Cakra Satya2Erry Koriyanti3Fiber Monado4Idha Royani5Sriwijaya UniversitySriwijaya UniversitySriwijaya UniversitySriwijaya UniversitySriwijaya UniversitySriwijaya UniversityWater-resistant PVA (polyvinyl alcohol) electrospun membranes with different crosslinking mechanisms were synthesized using the facile electrospinning technique. The crosslinking mechanisms were differentiated by introducing 2 different functional groups of different crosslinker agents into the molecular structure of the membrane. The evaluation of water resistance was conducted by both micro- and macro-structural analyses, such as Fourier Transform Infrared spectroscopy (FTIR), Scanning Electron Microscope (SEM), Energy Dispersive X-ray Spectroscopy (EDS), X-ray Diffraction (XRD), water contact angle (WCA), and immersion test. Infrared spectra confirmed the formation of new bands at around 1700 cm-1, which are acetal or ester groups, indicating the successful crosslinked process. Additionally, the lowered intensity of hydroxyl groups also signifies that the membrane is water-resistant. The XRD patterns showed the signature peak of PVA at the angle of 20°. Furthermore, the reduction in iron content, as shown by EDS spectra, was attributed to the surface imprinting process. SEM images displayed the formation of nanofibers, with mean diameters of 103 nm and interconnecting nanobead structures. The results showed that WCA was significantly enhanced, up to 91°, with minor loss in structure during water immersion test for 24 h. These findings confirm the hydrophobic characteristics of the membranes and their potential application in water-related fields.https://chimicatechnoacta.ru/article/view/7743poly(vinyl)-alcoholsurface-imprintingwater resistantcrosslinkedelectrospinning
spellingShingle Ihsan Alfikro
Jorena Jorena
Octavianus Cakra Satya
Erry Koriyanti
Fiber Monado
Idha Royani
Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sites
Chimica Techno Acta
poly(vinyl)-alcohol
surface-imprinting
water resistant
crosslinked
electrospinning
title Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sites
title_full Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sites
title_fullStr Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sites
title_full_unstemmed Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sites
title_short Assessment of different crosslinked mechanisms on PVA-based membranes to achieve water resistant properties with iron imprinting sites
title_sort assessment of different crosslinked mechanisms on pva based membranes to achieve water resistant properties with iron imprinting sites
topic poly(vinyl)-alcohol
surface-imprinting
water resistant
crosslinked
electrospinning
url https://chimicatechnoacta.ru/article/view/7743
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AT jorenajorena assessmentofdifferentcrosslinkedmechanismsonpvabasedmembranestoachievewaterresistantpropertieswithironimprintingsites
AT octavianuscakrasatya assessmentofdifferentcrosslinkedmechanismsonpvabasedmembranestoachievewaterresistantpropertieswithironimprintingsites
AT errykoriyanti assessmentofdifferentcrosslinkedmechanismsonpvabasedmembranestoachievewaterresistantpropertieswithironimprintingsites
AT fibermonado assessmentofdifferentcrosslinkedmechanismsonpvabasedmembranestoachievewaterresistantpropertieswithironimprintingsites
AT idharoyani assessmentofdifferentcrosslinkedmechanismsonpvabasedmembranestoachievewaterresistantpropertieswithironimprintingsites