Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) Nanoparticles

In this study, magnetic binary/ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) nanoparticles were synthesized using a straightforward one-step microwave techniqu...

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Main Authors: Sanaz Chamani, Masoumeh Khatamian
Format: Article
Language:English
Published: MDPI AG 2024-11-01
Series:Chemistry Proceedings
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Online Access:https://www.mdpi.com/2673-4583/16/1/29
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author Sanaz Chamani
Masoumeh Khatamian
author_facet Sanaz Chamani
Masoumeh Khatamian
author_sort Sanaz Chamani
collection DOAJ
description In this study, magnetic binary/ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) nanoparticles were synthesized using a straightforward one-step microwave technique. To produce the Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> nanoparticles, iron (III) nitrate nonahydrate, zinc nitrate hexahydrate, and cobalt nitrate hexahydrate were used as metal sources, with urea used as the fuel and ammonium nitrate as the oxidizer. These materials were combined in an alumina crucible covered by a CuO jacket to absorb microwave energy and facilitate calcination. The thermal treatment involved placing the alumina crucible in a domestic microwave oven at 450 W for 30 min. The key strengths of this experimental strategy include its simplicity, cost-effectiveness, and rapidity, aligning with green chemistry principles. The synthesized nanoparticles were characterized using X-ray diffraction (XRD), Fourier transform infrared (FT-IR) spectroscopy, a vibrating sample magnetometer (VSM), and Brunauer–Emmett–Teller (BET) analysis. XRD analysis confirmed the presence of the pure ferrite nanocrystalline phase. Scanning electron microscopy (SEM), employed with energy-dispersive X-ray spectroscopy (EDS), was used to study the surface morphology and analyze the elemental composition. The SEM analysis revealed that the synthesized magnetic nanoparticles had particle sizes ranging from 30 to 50 nm. Furthermore, we explored the potential use of these magnetic nanoparticles as photocatalysts for degrading organic pollutants such as methylene blue in aqueous solutions.
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spelling doaj-art-b182100931ad40f1ae8a683cdfdd59e82025-08-20T03:27:13ZengMDPI AGChemistry Proceedings2673-45832024-11-011612910.3390/ecsoc-28-20248Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) NanoparticlesSanaz Chamani0Masoumeh Khatamian1Koç University Boron and Advanced Materials Applications and Research Center (KUBAM), Istanbul 34450, TurkeyInorganic Chemistry Department, Faculty of Chemistry, University of Tabriz, Tabriz 5166616471, IranIn this study, magnetic binary/ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) nanoparticles were synthesized using a straightforward one-step microwave technique. To produce the Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> nanoparticles, iron (III) nitrate nonahydrate, zinc nitrate hexahydrate, and cobalt nitrate hexahydrate were used as metal sources, with urea used as the fuel and ammonium nitrate as the oxidizer. These materials were combined in an alumina crucible covered by a CuO jacket to absorb microwave energy and facilitate calcination. The thermal treatment involved placing the alumina crucible in a domestic microwave oven at 450 W for 30 min. The key strengths of this experimental strategy include its simplicity, cost-effectiveness, and rapidity, aligning with green chemistry principles. The synthesized nanoparticles were characterized using X-ray diffraction (XRD), Fourier transform infrared (FT-IR) spectroscopy, a vibrating sample magnetometer (VSM), and Brunauer–Emmett–Teller (BET) analysis. XRD analysis confirmed the presence of the pure ferrite nanocrystalline phase. Scanning electron microscopy (SEM), employed with energy-dispersive X-ray spectroscopy (EDS), was used to study the surface morphology and analyze the elemental composition. The SEM analysis revealed that the synthesized magnetic nanoparticles had particle sizes ranging from 30 to 50 nm. Furthermore, we explored the potential use of these magnetic nanoparticles as photocatalysts for degrading organic pollutants such as methylene blue in aqueous solutions.https://www.mdpi.com/2673-4583/16/1/29microwave synthesismagnetic nanoparticlesphotocatalystorganic pollutants
spellingShingle Sanaz Chamani
Masoumeh Khatamian
Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) Nanoparticles
Chemistry Proceedings
microwave synthesis
magnetic nanoparticles
photocatalyst
organic pollutants
title Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) Nanoparticles
title_full Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) Nanoparticles
title_fullStr Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) Nanoparticles
title_full_unstemmed Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) Nanoparticles
title_short Microwave-Assisted Green Synthesis of Binary/Ternary Zn<i><sub>x</sub></i>Co<sub>1−<i>x</i></sub>Fe<sub>2</sub>O<sub>4</sub> (<i>x</i> = 0, 0.5, 1) Nanoparticles
title_sort microwave assisted green synthesis of binary ternary zn i sub x sub i co sub 1 i x i sub fe sub 2 sub o sub 4 sub i x i 0 0 5 1 nanoparticles
topic microwave synthesis
magnetic nanoparticles
photocatalyst
organic pollutants
url https://www.mdpi.com/2673-4583/16/1/29
work_keys_str_mv AT sanazchamani microwaveassistedgreensynthesisofbinaryternaryznisubxsubicosub1ixisubfesub2subosub4subixi0051nanoparticles
AT masoumehkhatamian microwaveassistedgreensynthesisofbinaryternaryznisubxsubicosub1ixisubfesub2subosub4subixi0051nanoparticles